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The effective conductivity determines the reciprocal of the transport resistance, the dominant loss of fill factor in organic solar cells. We experimentally determine the dependence of effective conductivity on its electron and hole…

Materials Science · Physics 2025-08-18 Chen Wang , Toni Seiler , Doyoung Sun , Safa Shoaee , Maria Saladina , Carsten Deibel

The effect of hydrodynamic interactions on the free-solution electrophoresis of polyelectrolytes is investigated with coarse-grained molecular dynamics simulations. By comparing the results to simulations with switched-off hydrodynamic…

Soft Condensed Matter · Physics 2009-11-13 Kai Grass , Christian Holm

The dependence of DNA assemblies conductance on relative humidity is investigated theoretically. Following earlier suggestions, we consider the ionic conductivity through the layers of water adsorbed by DNA molecules. The increase in…

Chemical Physics · Physics 2015-05-14 J. M. Leveritt , S. Tesar , C. Dibaya , R. Shrestha , A. L. Burin

When electrolyte solutions are confined in micro- and nanochannels their conductivity is significantly different from those in a bulk phase. Here we revisit the theory of this phenomenon by focusing attention on the reduction in the ion…

Soft Condensed Matter · Physics 2023-11-08 Olga I. Vinogradova , Elena F. Silkina

We present a theory for the equilibrium structure of polyelectrolyte solutions. The main element is a simple, new optimization scheme that allows theories such as the random phase approximation (RPA) to handle the harsh repulsive forces…

Soft Condensed Matter · Physics 2009-11-10 James P. Donley , David R. Heine , David T. Wu

Interplay of Coulomb interaction energy, free ion entropy, and conformational elasticity is a fascinating aspect in polyelectrolytes (PEs). We develop a theory for complexation of two oppositely charged PEs, a process known to be the…

Soft Condensed Matter · Physics 2022-09-15 Soumik Mitra , Arindam Kundagrami

We fabricate electric double-layer field-effect transistor (EDL-FET) devices on mechanically exfoliated few-layer graphene. We exploit the large capacitance of a polymeric electrolyte to study the transport properties of three, four and…

Mesoscale and Nanoscale Physics · Physics 2017-01-11 E. Piatti , S. Galasso , M. Tortello , J. R. Nair , C. Gerbaldi , D. Daghero , M. Bruna , S. Borini , R. S. Gonnelli

A simple theory of the fluid state of a charged colloidal suspension is proposed. The full free energy of a polyelectrolyte solution is calculated. It is found that the counterions condense onto the polyions forming clusters composed of one…

Soft Condensed Matter · Physics 2009-10-30 Yan Levin , Marcia C. Barbosa , M. N. Tamashiro

The interaction between polyelectrolyte and ionic surfactant is of great importance in different areas of chemistry and biology. In this paper we present a theory of polyelectrolyte ionic-surfactant solutions. The new theory successfully…

Condensed Matter · Physics 2009-10-31 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

Bioelectrochemical systems are electrochemical cells that rely on conductive biofilms covering an electrode. We consider the example of a microbial fuel cell, and we derive a dynamic model of ion transport, biochemical reactions and…

In a solid, transport of electricity can occur via negative electrons or via positive holes. In the normal state of superconducting materials experiments show that transport is usually dominated by $dressed$ $positive$ $hole$ $carriers$.…

Superconductivity · Physics 2008-05-19 J. E. Hirsch

In a previous paper [S. Ghosal, Phys. Rev. E 74, 041901 (2006)] a hydrodynamic model for determining the electrophoretic speed of a polyelectrolyte through an axially symmetric slowly varying nanopore was presented in the limit of a…

Chemical Physics · Physics 2011-11-10 Sandip Ghosal

During the past few decades, several new classes of superconductors have been discovered. Most of these do not appear to be related to traditional superconductors. As a consequence, it is felt by many that for these materials,…

Superconductivity · Physics 2015-05-28 M. R. Norman

We calculate the inelastic lifetime of an electron quasiparticle due to Coulomb interactions in an electron liquid at low (or zero) temperature in two and three spatial dimensions. The contribution of "exchange" processes is calculated…

Strongly Correlated Electrons · Physics 2009-11-10 Zhixin Qian , Giovanni Vignale

Based on a recent proposal [O.P. Sushkov, Phys. Rev. B 64, 155319 (2001)], we relate the quantum conductance through a sample in which electrons are strongly correlated to the persistent current of a large ring, composed of the sample and a…

Strongly Correlated Electrons · Physics 2009-11-07 Rafael A. Molina , Dietmar Weinmann , Rodolfo A. Jalabert , Gert-Ludwig Ingold , Jean-Louis Pichard

Measurements of the capillary-driven thinning and breakup of fluid filaments are widely used to extract extensional rheological properties of complex materials. For viscoelastic (e.g., polymeric) fluids, the determination of the longest…

Soft Condensed Matter · Physics 2025-03-19 Vincenzo Calabrese , Amy Q. Shen , Simon J. Haward

Conductivity models for warm dense matter inform simulations of planetary structure and fusion experiments. State-of-the-art conductivity calculations based on density functional theory approximate many-body physics and neglect…

We study the flow of an electrically charged fluid through an elastic and porous medium. A three continuum model consisting of an elastic solid, a viscous fluid, and a mobile charge continuum is used. The relevant laws of physics are…

Soft Condensed Matter · Physics 2024-03-19 Jiashi Yang

Fluid dynamics is one of the cornerstones of modern physics and has recently found applications in the transport of electrons in solids. In most solids electron transport is dominated by extrinsic factors, such as sample geometry and…

We study the chemical potential of water as a function of charge based on perturbation theory. By calculating the electrostatic-energy fluctuations of two states (fully charged and uncharged) we are able to determine accurate values for the…

chem-ph · Physics 2008-02-03 Gerhard Hummer , Lawrence R. Pratt , Angel E. Garcia