Related papers: Clocking Auger Electrons
Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…
Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…
Typically, in Self-Amplified Spontaneous Emission Free Electron Laser (SASE FEL) based short-pulse schemes, pulse duration is limited by FEL coherence time. For hard X-ray FELs, coherence time is in a few hundred attosecond range while for…
Time-resolved X-ray absorption spectroscopy (tr-XAS) has been shown to be a versatile measurement technique for investigating non-equilibrium dynamics. Novel X-ray free electron laser (XFEL) facilities like the European XFEL offer increased…
In the field of chemistry, where nuclear motion has traditionally been a focal point, we now explore the ultra-rapid electronic motion spanning attoseconds to femtoseconds, demonstrating that it is equally integral and relevant to the…
This Letter of Intent describes LUXE (Laser Und XFEL Experiment), an experiment that aims to use the high-quality and high-energy electron beam of the European XFEL and a powerful laser. The scientific objective of the experiment is to…
Self-action nonlinearity is a key aspect -- either as a foundational element or a detrimental factor -- of several optical spectroscopies and photonic devices. Supercontinuum generation, wavelength converters and chirped pulse amplification…
Irradiation of solid surfaces with intense ultrashort laser pulses represents a unique way of depositing energy into materials. It allows to realize states of extreme electronic excitation and/or very high temperature and pressure, and to…
Free-electron lasers (FELs) can now generate temporally short, high power x-ray pulses of unprecedented brightness, even though their longitudinal coherence is relatively poor. The longitudinal coherence can be potentially improved by…
The LUXE experiment (Laser Und XFEL Experiment) is an experiment in planning at DESY Hamburg using the electron beam of the European XFEL (Eu.XFEL). LUXE is intended to study collisions between a high-intensity optical laser pulse and 16.5…
Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…
The ability to arbitrarily dial in amplitudes and phases enables the fundamental quantum state operations pioneered for microwaves and then infrared and visible wavelengths during the second half of the last century. Self-seeded X-ray…
The LUXE experiment aims at studying high-field QED in electron-laser and photon-laser interactions, with the 16.5 GeV electron beam of the European XFEL and a laser beam with power of up to 350 TW. The experiment will measure the spectra…
Using attoscience, we study the electron correlations responsible for Auger decay in krypton atoms. The Auger decay is induced by a pulse train or a twin pulse composed of subpulses of attosecond duration. During the Auger decay an optical…
In single particle coherent x-ray diffraction imaging experiments, performed at x-ray free-electron lasers (XFELs), samples are exposed to intense x-ray pulses to obtain single-shot diffraction patterns. The high intensity induces…
We demonstrate a novel method to measure the temporal evolution of electric fields with optical frequencies. Our technique is based on the detection of transient currents in air plasma. These directional currents result from sub-cycle…
The life-times due to Auger-electron emission for a hole on a deep electronic shell of neutral and charged sodium clusters are studied for different sizes. We consider spherical clusters and calculate the Auger-transition probabilities…
Understanding and controlling microscopic dynamics across spatial and temporal scales has driven major progress in science and technology over the past several decades. While ultrafast laser-based techniques have enabled probing nanoscale…
X-ray free-electron lasers (XFELs) with megahertz repetition rate can provide novel insights into structural dynamics of biological macromolecule solutions. However, very high dose rates can lead to beam-induced dynamics and structural…
X-ray Free Electron Lasers (XFEL) are the most advanced pulsed x-ray sources. Their extraordinary pulse parameters promise unique applications. Indeed, several new methods have been developed at XFEL-s. However, no methods are known, which…