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We review the problem of spin decoherence of magnetic atoms deposited on a surface. Recent breakthroughs in scanning tunnelling microscopy (STM) make it possible to probe the spin dynamics of individual atoms, either isolated or integrated…

Mesoscale and Nanoscale Physics · Physics 2017-02-14 F. Delgado , J. Fernández-Rossier

The nuclear spin of a phosphorus atom in silicon has been used as a quantum bit in various quantum-information experiments. It has been proposed that this nuclear-spin qubit can be efficiently controlled by an ac electric field, when…

Mesoscale and Nanoscale Physics · Physics 2019-10-02 Bence Hetényi , Péter Boross , András Pályi

The parametric excitation of spin waves by coherent surface acoustic waves is demonstrated experimentally in metallic magnetic thin film structures. The involved magnon modes are analyzed with micro-focused Brillouin light scattering…

Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…

The detection of ensembles of spins under ambient conditions has revolutionized the biological, chemical, and physical sciences through magnetic resonance imaging and nuclear magnetic resonance. Pushing sensing capabilities to the…

Mesoscale and Nanoscale Physics · Physics 2013-04-05 M. S. Grinolds , S. Hong , P. Maletinsky , L. Luan , M. D. Lukin , R. L. Walsworth , A. Yacoby

Two-dimensional Nuclear Magnetic Resonance (NMR) is essential in molecular structure determination. The Nitrogen-Vacancy (NV) center in diamond has been proposed and developed as an outstanding quantum sensor to realize NMR in nanoscale. In…

We present experimental results which demonstrate that nuclear magnetic resonance spectroscopy is capable of efficiently emulating many of the capabilities of quantum computers, including unitary evolution and coherent superpositions, but…

Quantum Physics · Physics 2009-10-30 David G. Cory , Mark D. Price , Timothy F. Havel

We report on Fourier spectroscopy experiments performed with near-surface nitrogen-vacancy centers in a diamond chip. By detecting the free precession of nuclear spins rather than applying a multipulse quantum sensing protocol, we are able…

Quantum Physics · Physics 2016-05-18 J. M. Boss , K. Chang , J. Armijo , K. Cujia , T. Rosskopf , J. R. Maze , C. L. Degen

Sensors based on spin qubits in 2D crystals offer the prospect of nanoscale sensing volumes, where the close proximity of the sensor and source could provide access to otherwise inaccessible signals. For AC magnetometry, the sensitivity and…

Materials Science · Physics 2024-03-14 Charlie J. Patrickson , Simon Baber , Blanka B. Gaál , Andrew J. Ramsay , Isaac J. Luxmoore

Echo-based spectroscopy of the superhyperfine interaction of an electronic spin with nuclear spins in its surroundings enables detailed insights into the microscopic magnetic environment of spins in solids. Still, it is an outstanding…

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

We consider an electronic spin, such as a nitrogen-vacancy (NV) center in diamond, weakly coupled to a large number (bath) of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase (multiple rotary echo). We…

Mesoscale and Nanoscale Physics · Physics 2015-03-25 V. V. Mkhitaryan , F. Jelezko , V. V. Dobrovitski

Magnetic resonance imaging is a three-dimensional imaging technique, where a gradient of the magnetic field is used to interrogate spin resonances with spatial resolution. The application of this technique to probe the coherence of atoms…

Quantum Physics · Physics 2025-02-24 Mateusz Mazelanik , Adam Leszczyński , Tomasz Szawełło , Michał Parniak

The small mass and high coherence of nanomechanical resonators render them the ultimate force probe, with applications ranging from biosensing and magnetic resonance force microscopy, to quantum optomechanics. A notorious challenge in these…

Quantum Physics · Physics 2017-07-18 Yeghishe Tsaturyan , Andreas Barg , Eugene S. Polzik , Albert Schliesser

Dielectric interfaces critical for metal-oxide-semiconductor (MOS) electronic devices, such as the Si/SiO$_2$ MOS field effect transistor (MOSFET), possess trap states that can be visualized with electrically-detected spin resonance…

Materials Science · Physics 2020-08-21 Nicholas J. Harmon , James P. Ashton , Patrick M. Lenahan , Michael E. Flatté

The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

Spin noise spectroscopy has become a widespread technique to extract information on spin dynamics in atomic and solid-state systems, in a potentially non-invasive way, through the optical probing of spin fluctuations. Here we experimentally…

Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

We study the vibrational motion of membrane resonators upon strong drive in the strongly nonlinear regime. By imaging the vibrational state of rectangular siliconnitride membrane resonators and by analyzing the frequency response using…

Mesoscale and Nanoscale Physics · Physics 2019-04-24 Fan Yang , Felix Rochau , Jana Huber , Alexandre Brieussel , Gianluca Rastelli , Eva M. Weig , Elke Scheer

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson