Related papers: RIXS Reveals Hidden Local Transitions of the Aqueo…
Recent debates on the oxygen redox behaviors in battery electrodes have triggered a pressing demand for the reliable detection and understanding of non-divalent oxygen states beyond conventional absorption spectroscopy. Here, enabled by…
Resonant inelastic x-ray scattering (RIXS) has become a powerful tool in the study of the electronic structure of condensed matter. Although the linewidths of many RIXS features are narrow, the experimental broadening can often hamper the…
Effective symmetry-based transition operators for resonant inelastic X-ray scattering (RIXS) are derived that show how the scattering between different states depends on the polarization of the incoming and outgoing X-rays. In spherical…
Resonant inelastic x-ray scattering (RIXS) has become a prominent technique to study quasiparticle excitations. With advances in polarization analysis capabilities at different facilities, RIXS offers exceptional potential for investigating…
Water (H2O) ice is ubiquitous component of the universe, having been detected in a variety of interstellar and Solar System environments where radiation plays an important role in its physico-chemical transformations. Although the radiation…
X-ray absorption spectroscopy (XAS) is a powerful experimental technique to probe the local order in materials with core electron excitations. Experimental interpretation requires supporting theoretical calculations. For water, these…
We analyze resonant inelastic x-ray scattering (RIXS) at the Cu K edge in a typical orbital-ordered compound KCuF3 on the basis of a microscopic theory. Spectral shape and its dependence on polarization direction and momentum transfer of…
With the advancement of synchrotron radiation and free-electron laser, X-ray quantum optics has emerged as a novel frontier for exploring light-matter interactions at high photon energies. A significant challenge in this field is achieving…
We describe a new method for imaging ultrafast dynamics in condensed matter using inelastic x-ray scattering (IXS). We use the concepts of causality and irreversibility to construct a general solution to the inverse scattering problem (or…
We derive general expressions for resonant inelastic x-ray scattering (RIXS) operators for $t_{2g}$ orbital systems, which exhibit a rich array of unconventional magnetism arising from unquenched orbital moments. Within the fast collision…
We propose a novel way to image dynamical properties of nonstationary electron systems using ultrafast resonant x-ray scattering. Employing a rigorous theoretical analysis within the framework of quantum electrodynamics, we demonstrate that…
While hydroxyl radicals ($\cdot$OH) play an important role as potent oxidizing agents in various plasma applications, their high reactivity confines them to a thin layer at the plasma-liquid interface, posing challenges in comprehending the…
Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$ spectral and…
The hydroxyl radical (OH) is found in various environments within the interstellar medium (ISM) of the Milky Way and external galaxies, mostly either in diffuse interstellar clouds or in the warm, dense environments of newly formed low-mass…
We present the fingerprints of dynamic Jahn-Teller effect in resonant inelastic x-ray scattering (RIXS) spectra of K$_2$RuCl$_6$. We determined the dynamic Jahn-Teller model Hamiltonian of an embedded Ru$^{4+}$ ion using post Hartree-Fock…
We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…
We show that, contrary to common lore, in resonant inelastic x-ray scattering (RIXS) at the copper L- and M-edge direct spin-flip scattering is in principle allowed. We demonstrate how this possibility can be exploited to probe the momentum…
An inelastic X-ray scattering experiment has been performed in liquid aluminum with the purpose of studying the collective excitations at wavevectors below the first sharp diffraction peak. The high instrumental resolution (up to 1.5 meV)…
Valence band electronic structure of mixed uranium oxides (UO2, U4O9, U3O7, U3O8, UO3) has been studied by the resonant inelastic X-ray scattering (RIXS) technique at the U M5 edge and by computational methods. We show here that the RIXS…
Recent experiments on La$_2$CuO$_4$ suggest that indirect resonant inelastic X-ray scattering (RIXS) might provide a probe for transversal spin dynamics. We present in detail a systematic expansion of the relevant magnetic RIXS cross…