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Element- and site-specific resonant inelastic x-ray scattering spectroscopy (RIXS) is employed to investigate electron correlation effects in {$\rm NaV_2O_5$}. In contrast to single photon techniques, RIXS at the vanadium $L_3$ edge is able…

Strongly Correlated Electrons · Physics 2009-11-07 G. P. Zhang , T. A. Callcott , G. T. Woods , L. Lin , Brian Sales , D. Mandrus , J. He

I present a tractable theory for the Resonant Inelastic X-ray Scattering (RIXS) spectral function of magnons. The low-energy transition operator is written as a product of local spin operators times fundamental x-ray absorption spectra.…

Strongly Correlated Electrons · Physics 2011-07-05 M. W. Haverkort

We report measurements of the non-resonant inelastic x-ray scattering (NRIXS) from the O 1s orbitals in ice Ih, and also report calculations of the corresponding spectra for ice Ih and several other phases of water ice. We find that the…

Materials Science · Physics 2008-01-15 T. T. Fister , K. P. Nagle , F. D. Vila , G. T. Seidler , C. Hamner , J. O. Cross , J. J. Rehr

Because chemical reactions on/in cosmic ice dust grains covered by amorphous solid water (ASW) play important roles in generating a variety of molecules, many experimental and theoretical studies have focused on the chemical processes…

Astrophysics of Galaxies · Physics 2021-01-11 Masashi Tsuge , Naoki Watanabe

Resonant inelastic x-ray scattering (RIXS) has become a very powerful experimental technique to probe a broad range of intrinsic elementary excitations, for example, from low energy phonons and (bi-)magnons to high energy $d$-$d$,…

Strongly Correlated Electrons · Physics 2019-06-20 Y. L. Wang , G. Fabbris , M. P. M. Dean , G. Kotliar

We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

Strongly Correlated Electrons · Physics 2013-05-29 J. N. Hancock , G. Chabot-Couture , Y. Li , G. Petrakovskii , K. Ishii , I. Jarrige , J. Mizuki , T. P. Devereaux , M. Greven

Recent experiments show that indirect resonant inelastic X-ray scattering (RIXS) is a new probe of spin dynamics. Here I derive the cross-section for magnetic RIXS and determine the momentum dependent four-spin correlation function that it…

Strongly Correlated Electrons · Physics 2015-06-25 Jeroen van den Brink

Nonresonant inelastic x-ray scattering (NIXS) is a possible tool to detect charge excitations in electron systems. In addition, multipole transitions at high-momentum-transfer region open a new possibility to determine orbital-selective…

Strongly Correlated Electrons · Physics 2015-11-11 Kenji Tsutsui , Eiji Kaneshita , Takami Tohyama

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting…

Strongly Correlated Electrons · Physics 2012-12-27 C. J. Jia , C. -C. Chen , A. P. Sorini , B. Moritz , T. P. Devereaux

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

We present calculations for resonant inelastic x-ray scattering (RIXS) in edge-shared copper oxide systems, such as CuGeO$_{3}$ and Li$_{2}$CuO$_{2}$, appropriate for hard x-ray scattering where the photoexcited electron lies above oxygen…

Strongly Correlated Electrons · Physics 2009-11-13 F. Vernay , B. Moritz , I. Elfimov , J. Geck , D. Hawthorn , T. P. Devereaux , G. A. Sawatzky

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…

Strongly Correlated Electrons · Physics 2019-11-20 A. M. Tsvelik , R. M. Konik , N. V. Prokof'ev , I. S. Tupitsyn

We propose a method for realizing true, real-space imaging of charge dynamics in a periodic system, with angstrom spatial resolution and attosecond time resolution. In this method, inelastic x-ray scattering (IXS) is carried out with a…

Strongly Correlated Electrons · Physics 2015-06-05 Yu Gan , Anshul Kogar , Peter Abbamonte

Resonant Inelastic X-ray scattering (RIXS) is a synchrotron-based spectroscopy that has seen growing interest across a range of scientific disciplines beyond fundamental physics. The interpretation of experimental RIXS data requires…

We develop a formalism to study indirect resonant inelastic x-ray scattering (RIXS) in systems with itinerant electrons, accounting for the attraction between valence electrons and the positively-charged core hole exactly, and apply this…

Strongly Correlated Electrons · Physics 2014-07-16 David Benjamin , Israel Klich , Eugene Demler

Excitons in a complex organic molecular crystal were studied by inelastic x-ray scattering (IXS) for the first time. The dynamic dielectric response function is measured over a large momentum transfer region, from which an exciton…

Other Condensed Matter · Physics 2007-05-23 K. Yang , L. P. Chen , Y. Q. Cai , N. Hiraoka , S. Li , J. F. Zhao , D. W. Shen , H. F. Song , H. Tian , L. H. Bai , Z. H. Chen , Z. G. Shuai , D. L. Feng

Continued improvement of the energy resolution of resonant inelastic x-ray scattering (RIXS) spectrometers is crucial for fulfilling the potential of this technique in the study of electron dynamics in materials of fundamental and…

Instrumentation and Detectors · Physics 2017-09-11 Jungho Kim , D. Casa , Ayman Said , Richard Krakora , B. J. Kim , Elina Kasman , Xianrong Huang , T. Gog

Resonant (elastic) soft x-ray scattering (RSXS) offers a unique element, site, and valence specific probe to study spatial modulations of charge, spin, and orbital degrees of freedom in solids on the nanoscopic length scale. It cannot only…

Materials Science · Physics 2013-04-12 J. Fink , E. Schierle , E. Weschke , J. Geck

We report on the Cu 1s resonant inelastic X-ray scattering (RIXS) of Cu-O one-dimensional (1D) strongly correlated insulator systems with contrasting atomic arrangements, namely edge-sharing CuGeO3 and corner-sharing Sr2CuO3. Owing to good…

Strongly Correlated Electrons · Physics 2009-11-11 S. Suga , S. Imada , A. Higashiya , A. Shigemoto , S. Kasai , M. Sing , H. Fujiwara , A. Sekiyama , A. Yamasaki , C. Kim , T. Nomura , J. Igarashi , M. Yabashi , T. Ishikawa