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Among all materials, mono-crystalline diamond has one of the highest measured thermal conductivities, with values above 2000 W/m/K at room temperature. This stems from momentum-conserving `normal' phonon-phonon scattering processes…

We investigate the lifetime of indirect excitons in extremely high purity diamond grown by the chemical vapor deposition method. A clear correlation is found between the lifetime and small strain (magnitude $< $10$^{-4}$) assessed using…

Materials Science · Physics 2020-11-25 K. Konishi , I. Akimoto , J. Isberg , N. Naka

The discovery of lead free all-inorganic alloyed double perovskites have revolutionized photovoltaic research, showing promising light emitting efficiency and its tunability. However, detailed studies regarding optical, exciton, polaron and…

Materials Science · Physics 2021-10-26 Manjari Jain , Manish Kumar , Preeti Bhumla , Saswata Bhattacharya

The coherent manipulation of excitons in bulk semiconductors via the lattice degrees of freedom is key to the development of acousto-optic and acousto-excitonic devices. Wide-bandgap transition metal oxides exhibit strongly bound excitons…

Time-resolved spectroscopy provides the main tool for analyzing the dynamics of excitonic energy transfer in light-harvesting complexes. To infer time-scales and effective coupling parameters from experimental data requires to develop…

Chemical Physics · Physics 2018-11-28 Tobias Kramer , Mirta Rodriguez , Yaroslav Zelinskyy

We report a combined theoretical/experimental study of dynamic screening of excitons in media with frequency-dependent dielectric functions. We develop an analytical model showing that interparticle interactions in an exciton are screened…

Mesoscale and Nanoscale Physics · Physics 2017-03-16 Andrey R. Klots , Benjamin Weintrub , Dhiraj Prasai , Daniel Kidd , Kalman Varga , Kirill A. Velizhanin , Kirill I. Bolotin

We apply an intense infrared laser pulse in order to perturb the electronic and vibrational states in the three-dimensional charge density wave material 1$T$-VSe$_2$. Ultrafast snapshots of the light-induced hot carrier dynamics and…

In this report we review recent experimental results on photoexcited carrier relaxation dynamics on high temperature superconductors (HTSC) probed by a femtosecond time-resolved optical spectroscopy, and compare the results with the data…

Superconductivity · Physics 2015-06-24 Jure Demsar , Dragan Mihailovic , Viktor V. Kabanov

Carrier multiplication by singlet exciton fission enhances photovoltaic conversion efficiencies in organic solids. This decay of one singlet exciton into two triplet states promises to overcome the Shockley-Queisser limit as up to two…

Materials Science · Physics 2016-12-16 K. Kolata , S. Marquardt , N. W. Rosemann , A. Mager , A. Hansmann , U. Höfer , R. Berger , T. Breuer , G. Witte , S. Chatterjee

Charge neutrality and their expected itinerant nature makes excitons potential transmitters of information. However, exciton mobility remains inaccessible to traditional optical experiments that only create and detect excitons with…

The ground state of two-dimensional (2D) electron systems with equal low densities of electrons and holes in nearby layers is an exciton fluid. We show that a reservoir for excitons can be established by contacting the two layers separately…

Mesoscale and Nanoscale Physics · Physics 2018-08-10 Ming Xie , Allan H. MacDonald

Theory predicts peculiar features for excited-state dynamics in one dimension (1D) that are difficult to be observed experimentally. Single-walled carbon nanotubes (SWNTs) are an excellent approximation to 1D quantum confinement, due to…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Giancarlo Soavi , Francesco Scotognella , Daniele Viola , Timo Hefner , Tobias Hertel , Giulio Cerullo , Guglielmo Lanzani

Excitation and charge transfer in low-energy O+H collisions is studied; it is a problem of importance for modelling stellar spectra and obtaining accurate oxygen abundances in late-type stars including the Sun. The collisions have been…

Solar and Stellar Astrophysics · Physics 2018-02-28 P. S. Barklem

Transform-limited photon emission from quantum emitters is essential for high-fidelity entanglement generation. In this study, we report the coherent optical property of a single negatively-charged lead-vacancy (PbV) center in diamond.…

Nitrogen-vacancy (NV) centers in diamond are reliable single-photon emitters, with applications in quantum technologies and metrology. Two charge states are known for NV centers: NV$^0$ and NV$^-$, with the latter being mostly studied due…

Optics · Physics 2019-12-23 Magdalena Solà-Garcia , Sophie Meuret , Toon Coenen , Albert Polman

We present systematic studies of the transient dynamics of GaAs by ultrafast time-resolved optical reflectivity. In photo excited non-equilibrium states, we found a sign reverse in transient reflectivity spectra $\Delta R/R$ (t $>$ 0), from…

Strongly Correlated Electrons · Physics 2018-05-25 X. C. Nie , H. Y. Liu , Xiu Zhang , Peng Gu , Hai-Ying Song , Fan Li , Jian-Qiao Meng , Yu-Xia Duin , Shi-Bing Liu

Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…

Excited states of the of the double-stranded DNA model (A)$_{12}\cdot$(T)_{12} were calculated in the framework of the exciton theory. The off-diagonal elements of the exciton matrix were calculated using the transition densities and ideal…

Soft Condensed Matter · Physics 2009-11-13 Arkadiusz Czader , Eric R. Bittner

The perturbation of a semiconductor from the thermodynamic equilibrium often leads to the display of nonlinear dynamics and formation of spatiotemporal patterns due to the spontaneous generation of competing processes. Here, we describe the…

Materials Science · Physics 2019-09-16 Ebrahim Najafi , Amir Jafari , Bolin Liao , Ahmed Zewail

Two-dimensional transition metal dichalcogenides (TMDCs) are promising materials for next-generation optoelectronic devices, yet their implementation is hindered by limited sample stability and challenges in forming reliable electrical…

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