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We demonstrate control over attosecond pulse generation and shaping by numerically optimizing the synthesis of few-cycle to sub-cycle driver waveforms. The optical waveform synthesis takes place in an ultrabroad spectral band covering the…

Optics · Physics 2014-09-15 E. Balogh , B. Bódi , V. Tosa , E. Goulielmakis , K. Varjú , P. Dombi

A laser was designed and constructed with the goal of producing ultra-short pulses at a high repetition rate as needed for certain applications of multi-photon microscopy. With pure prism-based dispersion compensation repetition rates of up…

Optics · Physics 2007-05-23 J. Sawinski , D. Debarre , W. Denk

High energy terahertz pulses are produced by optical rectification (OR) in organic crystals DAST and DSTMS by a Ti:sapphire amplifier system centered at 0.8 microns. The simple scheme provides broadband spectra between 1 and 5 THz, when…

Optics · Physics 2015-06-17 B. Monoszlai , C. Vicario , M. Jazbinsek , C. P. Hauri

We report the generation of a multi-octave supercontinuum spanning from 350 nm to 1700 nm with exceptional spectral flatness and high conversion efficiency to both the visible and near infrared region, by pumping a methane-filled…

We demonstrate a versatile technique for generating continuously wavelength-tunable laser waveforms, with mJ pulse energies and ultrashort pulse durations down to few-cycle in the ultraviolet C and visible spectral ranges. Using the…

We demonstrate a broad, flat, visible supercontinuum spectrum that is generated by a dispersion-engineered tapered photonic crystal fiber pumped by a 1 GHz repetition rate turn-key Ti:sapphire laser outputting $\sim$ 30 fs pulses at 800 nm.…

Instrumentation and Methods for Astrophysics · Physics 2018-10-29 Aakash Ravi , Matthias Beck , David F. Phillips , Albrecht Bartels , Dimitar Sasselov , Andrew Szentgyorgyi , Ronald L. Walsworth

We present a solid-state laser system that generates over 200 mW of continuous-wave, narrowband light, tunable from 316.3 nm - 317.7 nm and 318.0 nm - 319.3 nm. The laser is based on commercially available fiber amplifiers and optical…

We present a laser source delivering waveform-controlled 1.5-cycle pulses that can be focused to relativistic intensity at 1 kHz repetition rate. These pulses are generated by nonlinear compression of high-temporal-contrast sub-25\,fs…

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

Atomic and Molecular Clusters · Physics 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…

We report here an experimental setup to perform three-pulse pump-probe measurements over a wide wavelength and temperature range. By combining two pump pulses in the visible (650-900 nm) and mid-IR (5-20 $\mu$m) range, with a broadband…

We demonstrate a novel technique for producing high-order harmonics with designer spectral combs in the extreme ultraviolet-soft X-ray range for resonance applications using spectrally controlled visible lasers. Our approach enables…

The advancement of the ultrafast pulse shaping and waveform synthesis allowed to coherently control the atomic and electronic motions in matter. The temporal resolution of the waveform synthesis is inversely proportional to the broadening…

Optics · Physics 2024-06-04 Husain Alqattan , Dandan Hui , Vladimir Pervak , Mohammed Th. Hassan

High-energy, carrier-envelope phase (CEP)-stable, sub-cycle, mid-infrared (mid-IR) pulses can provide unique opportunities of exploring phase-sensitive strong-field light-matter interactions in atoms, molecules, and solids. In the mid-IR…

Supercontinuum (SC) light source has advanced ultrafast laser spectroscopy in condensed matter science, biology, physics, and chemistry. Compared to the frequently used photonic crystal fibers and bulk materials, femtosecond laser…

Laser pulses with a duration of one femtosecond or shorter can be generated both in the IR-VIS and in the extreme UV, but the deep UV is a spectral region where such extremely short pulses have not yet been demonstrated. Here, a method for…

Optics · Physics 2019-01-24 Jan Reislöhner , Christoph Leithold , Adrian N. Pfeiffer

Many experiments in biological and medical sciences currently use multiphoton microscopy as a core imaging technique. To date, solid-state lasers are most commonly used as excitation beam sources. However, the most demanding applications…

Phase-matched harmonic conversion of visible laser light into soft x-rays was demonstrated. The recently developed technique of guided-wave frequency conversion was used to upshift light from 800 nanometers to the range from 17 to 32…

Novel table-top sources of extreme-ultraviolet light based on high-harmonic generation yield unique insight into the fundamental properties of molecules, nanomaterials, or correlated solids, and enable advanced applications in imaging or…

Full coherent soft X-ray attosecond pulses are now available through high-order harmonic generation (HHG); however, its insufficient output energy hinders various applications, such as attosecond-scale soft X-ray nonlinear experiments, the…