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The bottleneck for an attosecond science experiment is concluded to be the lack of a high-peak-power isolated attosecond pulse source. Therefore, currently, generating an intense attosecond pulse would be one of the highest priority goals.…

The generation of gigawatt-class isolated attosecond pulses (IAPs) is vital for attosecond pump-probe experiments. In such experiments, the temporal duration of IAPs must be determined quickly and accurately. In this study, we developed a…

The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of…

Optics · Physics 2025-11-03 Kaito Nishimiya , Rambabu Rajpoot , Eiji J Takahashi

The development of high-energy, high-power, multi-octave light-transients is currently subject of intense research driven by emerging applications in attosecond spectroscopy and coherent control. We report on a phase-stable, multi-octave…

Efficient supercontinuum (SC) generation featuring high spectral intensity across a large bandwidth requires high peak powers of several megawatt from pulsed lasers. Under these conditions and at multi-kilohertz (kHz) repetition rates, the…

We have produced a soft x-ray supercontinuum with a pulse energy of 0.24-$\mu$J using high-order harmonics from a multiterawatt, 10-Hz, stable, three-channel waveform synthesizer [Sci. Adv. eaay2802 (2020)]. We report here an attosecond…

Optics · Physics 2022-03-24 Bing Xue , Katsumi Midorikawa , Eiji J. Takahashi

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…

This study demonstrates the potential to generate a soft X-ray single-cycle attosecond pulse using a single-cycle mid-infrared pulse from the advanced dual-chirped optical parametric amplification. Supercontinuum high harmonic (HH) spectrum…

Optics · Physics 2024-10-07 Kaito Nishimiya , Feng Wang , Pengfei Lan , Eiji J. Takahashi

Providing phase stable laser light is important to extend the interrogation time of optical clocks towards many seconds and thus achieve small statistical uncertainties. We report a laser system providing more than 50 uW phase-stabilized UV…

The generation of attosecond pulses (1 as=10-18 s) has enabled real-time observation and manipulation of coherent electron dynamics, yet their low peak power has hindered the development of advanced attosecond pump-probe spectroscopy and…

Optics · Physics 2026-04-23 Lihui Meng , Lu Xu , Xusheng Zhu , Lixin He , Zan Nie , Pengfei Lan , Peixiang Lu

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

A source of ultrashort pulses of light in the 2 {\mu}m region was constructed using supercontinuum broadening from an erbium mode-locked laser. The output spectrum spanned 1000 nm to 2200 nm with an average power of 250 mW. A pulse width of…

Optics · Physics 2017-07-26 Andrew Klose , Gabriel Ycas , Daniel L. Maser , Scott A. Diddams

An optical parametric chirped pulse amplifier fully based on Yb lasers at 500 kHz is described. Passive optical-synchronization is achieved between a fiber laser-pumped white-light and a 515 nm pump produced with a 200 W picosecond Yb:YAG…

We demonstrate the highest flux tabletop source of coherent soft X-rays to date, driven by a single-stage 10 mJ Ti:sapphire regenerative amplifier at 1 kHz. We first down-convert the laser to 1.3 um using a parametric amplifier, before…

Controlling femtosecond optical pulses with temporal precision better than one cycle of the carrier field has a profound impact on measuring and manipulating interactions between light and matter. We explore pulses that are carved from a…

Attosecond photoelectron spectroscopy is often performed with interferometric experimental setups that require outstanding stability. We demonstrate and characterize in detail an actively stabilized, versatile, high spectral resolution…

The generation of high power coherent soft X-ray pulses of sub-100 as duration and 10 nm wavelength using beams from a GeV energy plasma wakefield accelerator has been recently investigated in Ref. [arXiv:2011.07163]. As a future upgrade to…

Accelerator Physics · Physics 2024-01-17 Rafi Hessami , Jenny Morgan , River Robles , Kirk A. Larsen , Agostino Marinelli , Claudio Emma

The availability of electromagnetic pulses with controllable field waveform and extremely short duration, even below a single optical cycle, is imperative to fully harness strong-field processes and to gain insight into ultrafast…

We report a multi-channel optical frequency synthesizer developed to generate extremely stable continuous wave lasers directly out of the optical comb of an Er-doped fiber oscillator. Being stabilized to a high-finesse cavity with a…

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