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Related papers: Strong-field ionization of complex molecules

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The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…

Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the…

Atomic Physics · Physics 2016-02-22 Xiaohong Song , Cheng Lin , Zhihao Sheng , Peng Liu , Zhangjin Chen , Weifeng Yang , Shilin Hu , C. D. Lin , Jing Chen

Strong-field photoelectron holography denotes the interference of various electron paths in laser-induced ionization of atoms, leading to interference patterns in the final momentum distribution. For a quantitative description of holography…

Atomic Physics · Physics 2019-08-28 Simon Brennecke , Manfred Lein

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

When a strong laser pulse induces the ionization of an atom, momentum conservation dictates that the absorbed photons transfer their momentum $p_{\gamma}=E_{\gamma}/c$ to the electron and its parent ion. Even after 30 years of studying…

Ionization of an atom or molecule presents surprising richness beyond our current understanding: strong-field ionization with low-frequency fields recently revealed unexpected kinetic energy structures (1, 2). A solid grasp on electron…

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of…

Atomic Physics · Physics 2019-03-27 N. I. Shvetsov-Shilovski , M. Lein , K. Tőkési

We present a semiclassical two-step model for strong-field ionization that accounts for path interferences of tunnel-ionized electrons in the ionic potential beyond perturbation theory. Within the framework of a classical trajectory…

We present an ab initio study of the nonsequential strong-field ionization dynamics of a model two-electron atom with helium character. Single- and double-ionization events are characterized and displayed using detector signals extracted at…

Atomic Physics · Physics 2023-06-14 Daniel Younis , Joseph H. Eberly

Photoelectron momentum distributions from strong-field ionization of carbonyl sulfide with 800 nm central-wavelength laser pulses at various peak intensities from $4.6$ to $13\times10^{13}$ W/cm$^2$ were recorded and analyzed regarding…

We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…

Strong field ionization provides a unique mean to address complex dynamics of an electron in competing Coulomb and laser fields. Recent streak camera experiment (K\"ubel, et al., Phys. Rev. Lett. 119, 183201) analyzed asymmetries in the…

We investigate the photoionization dynamics of atoms subjected to intense, ultrashort laser pulses through the use of quantum trajectories. This method provides a unique and consistent framework for examining electron dynamics within a…

Atomic Physics · Physics 2024-08-01 Taylor Moon , Klaus Bartschat , Nicolas Douguet

We report on the unambiguous observation of the sub-cycle ionization bursts in sequential strong-field double ionization of H$_2$ and their disentanglement in molecular frame photoelectron angular distributions. This observation was made…

Interaction of a strong laser pulse with matter transfers not only energy but also linear momentum of the photons. Recent experimental advances have made it possible to detect the small amount of linear momentum delivered to the…

We investigate the effects of the multielectron polarization of the ion described by the induced dipole potential in photoelectron momentum distributions produced in ionization of the CO molecule by a strong laser field. We present results…

Atomic Physics · Physics 2024-04-23 Mahmoud Abu-samha , L. B. Madsen , N. I. Shvetsov-Shilovski

Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

The dynamics of light-matter interactions in the realm of strong-field ionization has been a focal point and has attracted widespread interest. We present the eTraj.jl program package, designed to implement established…

Atomic Physics · Physics 2025-02-28 Mingyu Zhu , Hongcheng Ni , Jian Wu

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

Atomic Physics · Physics 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

We demonstrate that quantum light statistics can be used to control strong-field ionization at the tunneling step. Using a bichromatic linearly polarized field composed of a strong coherent driver and a weak bright squeezed vacuum (BSV), we…

Quantum Physics · Physics 2026-04-15 G. Singh , T. Rook , J. Rivera-Dean , C. Figueira de Morisson Faria
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