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Related papers: Strong-field ionization of complex molecules

200 papers

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant…

Atomic Physics · Physics 2018-10-03 J. Fedyk , A. B. Voitkiv , C. Müller

We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

We present a combined experimental and theoretical study on strong-field ionization of a three-dimensionally oriented asymmetric top molecule, benzonitrile (C$_7$H$_5$N), by circularly polarized, nonresonant femtosecond laser pulses. Prior…

Signatures of the Coulomb corrections in the photoelectron momentum distribution during laser-induced ionization of atoms or ions in tunneling and multiphoton regimes are investigated analytically in the case of an one-dimensional problem.…

The nondipole under-the-barrier dynamics of the electron during strong-field tunneling ionization is investigated, examining the role of the Coulomb field of the atomic core. The common analysis in the strong field approximation is…

Atomic Physics · Physics 2022-04-06 Pei-Lun He , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Strong-field ionization by counter-rotating two-color laser fields produces quantum interference between photoelectrons emitted on the leading and trailing edges of the laser field oscillations. We show that in chiral molecules, this…

We analyze atomic photoelectron momentum distributions induced by bichromatic and monochromatic laser fields within the strong field approximation (SFA), separable Coulomb-Volkov approximation (SCVA), and ab initio treatment. We focus on…

Atomic Physics · Physics 2009-06-11 Denys I. Bondar , Michael Spanner , Wing-Ki Liu , Gennady L. Yudin

In strong-field ionization interferences between electron trajectories create a variety of interference structures in the final momentum distributions. Among them, the interferences between electron pathways that are driven directly to the…

The combination of photoelectron spectroscopy and ultrafast light sources is on track to set new standards for detailed interrogation of dynamics and reactivity of molecules. A crucial prerequisite for further progress is the ability to not…

Nondipole effects are ubiquitous and crucial in light-matter interaction. However, they are too weak to be directly observed. In strong-field physics, motion of electrons is mainly confined in transverse plane of light fields, which…

Atomic Physics · Physics 2023-03-07 Yankun Dou , Yiqi Fang , Peipei Ge , Yunquan Liu

We present a novel approach to calculating strong field ionization dynamics of multielectron molecular targets. Adopting a multielectron wavefunction ansatz based on field-free ab initio neutral and ionic multielectron states, a set of…

Atomic Physics · Physics 2015-05-14 Michael Spanner , Serguei Patchkovskii

We extend the semiclassical two-step model [Phys. Rev. A 94, 013415 (2016)] to include a multielectron polarization-induced dipole potential. Using this model we investigate the imprints of multielectron effects in the momentum…

Atomic Physics · Physics 2018-08-22 N. I. Shvetsov-Shilovski , M. Lein , L. B. Madsen

We investigate the role of nuclear motion and strong-field-induced electronic couplings during the double ionization of deuterated water using momentum-resolved coincidence spectroscopy. By examining the three-body dicationic dissociation…

We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

Recollision processes are fundamental to strong-field physics and attoscience, thus models connecting recolliding trajectories to quantum amplitudes are a crucial part in furthering understanding of these processes. We report developments…

Atomic Physics · Physics 2023-11-06 Mads Brøndum Carlsen , Emil Hansen , Lars Bojer Madsen , Andrew Stephen Maxwell

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we…

Atomic Physics · Physics 2020-02-19 Benjamin Willenberg , Jochen Maurer , Benedikt W. Mayer , Ursula Keller

We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…

Atomic Physics · Physics 2013-06-26 M. F. Ciappina , J. A. Pérez-Hernández , T. Shaaran , L. Roso , M. Lewenstein

Interaction of a strong laser pulse with matter transfers not only energy but also linear momentum of the photons. Recent experimental advances have made it possible to detect the small amount of linear momentum delivered to the…

Atomic Physics · Physics 2022-12-19 Xiaodan Mao , Hongcheng Ni , Xiaochun Gong , Joachim Burgdörfer , Jian Wu