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Quantum simulators based on cold atomic gases can provide an ideal platform to study the microscopic mechanisms behind intriguing properties of solid materials and further explore novel exotic phenomena inaccessible by chemical synthesis.…

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

Ionization of an atom or molecule presents surprising richness beyond our current understanding: strong-field ionization with low-frequency fields recently revealed unexpected kinetic energy structures (1, 2). A solid grasp on electron…

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

Quantum Physics · Physics 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

We discuss a method of solving the time dependent Schrodinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997)] to calculate…

Atomic Physics · Physics 2014-05-19 Armin Scrinzi , Bernard Piraux

The electronic structure of electron doped iron-arsenide superconductors Ba(Fe1- xCox)2As2 has been measured with Angle Resolved Photoemission Spectroscopy. The data reveal a marked photon energy dependence of points in momentum space where…

We formulate a three-dimensional semi-classical model to treat three-electron escape dynamics in a strongly-driven linear triatomic molecule, HeH$_{2}^{+}$. Our model includes the Coulomb singularities. Hence, to avoid unphysical…

Atomic Physics · Physics 2021-04-21 M. B. Peters , V. P. Majety , A. Emmanouilidou

For the description of nonsequential double ionization (NSDI) of rare-gas atoms by a strong linearly polarized laser field, the quantum-mechanical $S$-matrix diagram that incorporates rescattering impact ionization is evaluated in the…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu , H. Schomerus , W. Becker

Photoelectron spectra obtained from the ab initio solution of the time-dependent Schr\"odinger equation can be in striking disagreement with predictions by the strong-field approximation (SFA) not only at low energy but also around twice…

Atomic Physics · Physics 2016-12-14 Th. Keil , S. V. Popruzhenko , D. Bauer

Here, we report on the nonlinear ionization of argon atoms in the short wavelength regime using ultraintense x rays from the European XFEL. After sequential multiphoton ionization, high charge states are obtained. For photon energies that…

We present an ab initio study of the nonsequential strong-field ionization dynamics of a model two-electron atom with helium character. Single- and double-ionization events are characterized and displayed using detector signals extracted at…

Atomic Physics · Physics 2023-06-14 Daniel Younis , Joseph H. Eberly

We extend a recently developed three-dimensional semiclassical model [\href{https://journals.aps.org/pra/abstract/10.1103/PhysRevA.109.033106}{Phys. Rev. \textbf{A} 109, 033106 (2024)}] to study multielectron ionization and the formation of…

Atomic Physics · Physics 2026-02-17 Georgios Petros Katsoulis , Agapi Emmanouilidou

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

Double ionization processes triggered by intense linearly polarized laser fields have revealed the paramount role of electron-electron collisions. It has been shown that the correlated dynamics of such electronic collisions can be modeled…

Atomic Physics · Physics 2011-05-03 Francois Mauger , Cristel Chandre , Turgay Uzer

The Gamma Factory (GF) initiative aims at the construction of a unique experimental tool exploiting resonant interaction of light with ultra-relativistic partially stripped ions (PSI) stored in circular accelerators at CERN. Resonant…

Atomic Physics · Physics 2022-05-31 J. Bieroń , M. W. Krasny , W. Płaczek , S. Pustelny

Strong-field ionization generally produces ions in a superposition of ionic eigenstates. This superposition is generally not fully coherent und must be described in terms of a density matrix. A recent experiment [E. Goulielmakis et al.,…

Atomic Physics · Physics 2015-05-27 Robin Santra , Vladislav S. Yakovlev , Thomas Pfeifer , Zhi-Heng Loh

We analyzed the two-dimensional (2D) electron momentum distributions of high-energy photoelectrons of atoms in an intense laser field using the second-order strong field approximation (SFA2). The SFA2 accounts for the rescattering of the…

Atomic Physics · Physics 2009-11-13 Zhangjin Chen , Toru Morishita , Anh-Thu Le , C. D. Lin

We investigate the physical processes in which an electron, upon return to its parent ion, promotes a second electron to an excited state, from which it subsequently tunnels. Employing the strong-field approximation and saddle-point…

Atomic Physics · Physics 2015-05-13 T. Shaaran , C. Figueira de Morisson Faria

We introduce soft recollisions in laser-matter interaction. They are characterized by the electron missing the ion upon recollision in contrast to the well-known head-on collisions responsible for high-harmonic generation or above-threshold…

Atomic Physics · Physics 2015-03-19 Alexander Kästner , Ulf Saalmann , Jan M. Rost
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