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We report on a novel method for photo-association of strongly polar trilobite Rydberg molecules. This exotic ultralong-range dimer, consisting of a ground-state atom bound to the Rydberg electron via electron-neutral scattering, inherits…

We present measurements of hyperfine structure (HFS) of the $nP_J$ Rydberg states for large principal quantum number $n$ range ($n=41-55$) employing the microwave spectroscopy in an ultra-cold cesium Rydberg ensemble. A microwave field with…

Atomic Physics · Physics 2024-10-15 Rong Song , Jingxu Bai , Zhenhua Li , Yuechun Jiao , Suotang Jia , Jianming Zhao

We present precise measurements of the quantum defects of cesium $n$F$_J$ Rydberg levels. We employ high-precision microwave spectroscopy of $(n+2)\mathrm{D}_{5/2}\rightarrow n\mathrm{F}_{5/2,7/2}$ transitions for $n=45$ to 50 in a…

Atomic Physics · Physics 2023-08-10 Jingxu Bai , Yuechun Jiao , Rong Song , Jiabei Fan , Jianming Zhao , Suotang Jia , Georg Raithe

The lifetimes and decay channels of ultralong-range Rydberg molecules created in a dense BEC are examined by monitoring the time evolution of the Rydberg population using field ionization. Studies of molecules with values of principal…

Spectroscopic measurements of the rotational distribution of $^{84}$Sr and $^{86}$Sr 5sns $^1S_0$ ultralong-range Rydberg molecular dimers created via photoassociation in a cold gas are reported. The dimers are produced by two-photon…

Atomic Physics · Physics 2024-06-14 C. Wang , Y. Lu , S. K. Kanungo , F. B. Dunning , T. C. Killian , S. Yoshida

A proof-of-principle electron electric dipole moment (e-EDM) experiment using slow cesium atoms, nulled magnetic fields, and electric field quantization has been performed. With the ambient magnetic fields seen by the atoms reduced to less…

Atomic Physics · Physics 2008-11-26 Jason M. Amini , Charles T. Munger , Harvey Gould

Applicability of Rydberg atoms to quantum computers is examined from experimental point of view. In many theoretical proposals appeared recently, excitation of atoms into highly excited Rydberg states was considered as a way to achieve…

Quantum Physics · Physics 2007-05-23 Igor I. Ryabtsev , Denis B. Tretyakov , Ilya I. Beterov

We discuss the realization of mesoscopic phases of dipolar gases relevant to current experiments with cold polar molecules and Rydberg atoms confined to two dimensions. We predict the existence of superfluid clusters, mesoscopic…

Quantum Gases · Physics 2009-04-20 G. Pupillo , A. Micheli , M. Boninsegni , I. Lesanovsky , P. Zoller

Double-resonant photoexcitation of nitric oxide in a molecular beam creates a dense ensemble of $50f(2)$ Rydberg states, which evolves to form a plasma of free electrons trapped in the potential well of an NO$^+$ spacecharge. The plasma…

Chemical Physics · Physics 2015-05-27 N. Saquet , J. P. Morrison , M. Schulz-Weiling , H. Sadeghi , J. Yiu , C. J. Rennick , E. R. Grant

We characterize the two-photon excitation of an ultracold gas of Rubidium atoms to Rydberg states analysing the induced atomic losses from an optical dipole trap. Extending the duration of the Rydberg excitation to several ms, the ground…

Atomic Physics · Physics 2015-06-03 T. M. Weber , T. Niederprüm , T. Manthey , P. Langer , V. Guarrera , G. Barontini , H. Ott

The Standard Model (SM) of Particle Physics is not capable to account for the apparent matter-antimatter asymmetry of our Universe. Physics beyond the SM is required and is either probed by employing highest energies (e.g., at LHC), or by…

Nuclear Experiment · Physics 2019-05-01 Frank Rathmann , Nikolai N. Nikolaev

We introduce four new molecules -- YbRb, YbCs, YbSr$^+$, and YbBa$^+$ -- that may prove fruitful in experimental searches for the electric dipole moment (EDM) of the electron. These molecules can, in principle, be prepared at extremely low…

Atomic Physics · Physics 2015-05-13 Edmund R. Meyer , John L. Bohn

We present a comprehensive study of the diverse properties of heteronuclear Rydberg molecules, placing a special emphasis on those composed of the light alkali atoms, Li, Na, and K. Electron-atom scattering phase shifts, which determine the…

Atomic Physics · Physics 2019-02-13 Matthew T. Eiles

The electric dipole moment (EDM) of paramagnetic atoms is sensitive to the intrinsic EDM contribution from that of its constituent electrons and a scalar--pseudo-scalar (S-PS) electron-nucleus interactions. The electron EDM and the S-PS EDM…

Atomic Physics · Physics 2008-07-16 H. S. Nataraj , B. K. Sahoo , B. P. Das , D. Mukherjee

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

Atoms excited to electronically high-lying Rydberg states decay to low-energy states through spontaneous emission processes. We investigate the impact of a static electric field on the superradiant emission process between Rydberg…

Atomic Physics · Physics 2024-11-18 Yunhui He , Jingxu Bai , Yuechun Jiao , Weibin Li , Jianming zhao

Resonant energy transfer (RET), between equal parity 1s65s$^3\mathrm{S}_1$ and 1s66s$^3\mathrm{S}_1$ Rydberg levels in helium has been observed in low-temperature ($\sim80$ mK) collisions with ammonia molecules which undergo inversion…

Atomic Physics · Physics 2026-05-21 J. Zou , R. R. W. Wang , R. González-Férez , H. R. Sadeghpour , S. D. Hogan

We propose a novel scheme to efficiently tune the scattering length of two colliding ground-state atoms by off-resonantly coupling the scattering-state to an excited Rydberg-molecular state using laser light. For the s-wave scattering of…

Quantum Gases · Physics 2017-10-04 Nóra Sándor , Rosario González-Férez , Paul S. Julienne , Guido Pupillo

Long-range $(n+2)D_{5/2} \, nF_J$ Rydberg macro-dimers are observed in an ultracold cesium Rydberg gas for $39\leq n\leq48$. Strong dipolar "flip" ($\langle D_{5/2} F_{5/2} \vert \hat{V}_{dd} \vert F_{5/2} D_{5/2} \rangle$, $\langle D_{5/2}…

Atomic Physics · Physics 2024-11-05 Jingxu Bai , Yuechun Jiao , Rong Song , Georg Raithel , Suotang Jia , Jianming Zhao

The permanent electric dipole moment (EDM) of the ground state of potassium has been found by measuring the electric susceptibility. We find d(K)=(1.58 plus or minus 0.19(stat) plus or minus 0.13(syst)) times 10-8 e.cm and the induced EDM,…

General Physics · Physics 2011-06-28 Pei-Lin You
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