Related papers: Cesium $nD_{J}$+$6S_{1/2}$ Rydberg molecules and t…
We present a depletion imaging technique to map out the spatial and temporal dependency of the density distribution of an ultracold gas of Rydberg atoms. Locally resolved absorption depletion, observed through differential ground state…
Alkaline earth Rydberg atoms are very promising tools for quantum technologies. Their highly excited outer electron provides them with the remarkable properties of Rydberg atoms and, notably, with a huge coupling to external fields or to…
We employ two-photon spectroscopy to study the vibrational states of the triplet ground state potential ($a^3\Sigma^+$) of the $^{23}$Na$^{6}$Li molecule. Pairs of Na and Li atoms in an ultracold mixture are photoassociated into an excited…
The resonant transfer of energy from the inversion sublevels in NH$_3$ to He atoms in triplet Rydberg states with principal quantum number $n=38$ has been controlled using electric fields below 15 V/cm in intrabeam collisions at…
Polarisation labelling spectroscopy technique was employed to study the 3$^{1}\Pi_{u}$ state of Cs$_2$ molecule. The main equlibrium constants are $T_e=20684.60$cm$^{-1}$, $\omega_e=30.61$cm$^{-1}$ and $R_e=5.27$\r{A}. Vibrational levels…
We present a study of the Rydberg spectrum in $^{39}K$ for $nS$ and $nD_{3/2}$ series connected to $5^2P_{1/2}$ using two-photon spectroscopy based on EIT in a heated vapor cell. We observed some 80 transitions from $5P_{1/2}$ to Rydberg…
We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar…
Photoassociation of ultracold atoms induced by chirped picosecond pulses is analyzed in a non-perturbative treatment by following the wavepackets dynamics on the ground and excited surfaces. The initial state is described by a Boltzmann…
This work reports on the real-time detection of internal-state dynamics of cold Rb$^{87}$ atoms being excited to the $30D_{5/2}$ Rydberg state via two-photon excitation. A mesoscopic cloud of atoms is overlapped with the mode volume of a…
The matter-antimatter asymmetry cannot be explained by the Standard Model (SM) of elementary particle physics. According to A. Sakharov, additional sources of $\mathcal{CP}$-Violating phenomena are needed to understand the matter-antimatter…
Novel equations for the electric dipole polarizability $\alpha_{_{E1}}$ of low-lying excited states in atomic nuclei -- and the related $(-2)$ moment of the total photo-absorption cross section, $\sigma_{_{-2}}$ -- are inferred in terms of…
We develop and study quantum and semi-classical models of Rydberg-atom spectroscopy in amplitude-modulated optical lattices. Both initial- and target-state Rydberg atoms are trapped in the lattice. Unlike in any other spectroscopic scheme,…
A fascinating aspect of Rydberg atoms is their ability to form huge but very weakly bound molecules with a ground state atom, only held together by a scattering process between the latter and the Rydberg electron. Beyond the usual way of…
Rydberg molecules, Rydberg-atom or Rydberg-molecule, are an essential ingredient of cold molecular sciences. However, due to the richness of Rydberg-neutral interactions, new kinds of Rydberg molecules and binding mechanisms are still to be…
Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…
A highly sensitive, general, and preferably nondestructive technique to detect polar molecules would greatly advance a number of fields, in particular quantum science with cold and ultracold molecules. Here, we propose using resonant energy…
H$_3^{2+}$ is a one-electron system with three positive nuclei and is known to be unstable in its electronic ground-state. We examine an analogous one-electron system composed of a $^{87}$Rb Rydberg atom interacting with a pair of cations…
We recently reported the formation of ultracold LiCs molecules in the rovibrational ground state X1Sigma+,v''=0,J''=0 [J. Deiglmayr et al., PRL 101, 133004 (2008)]. Here we discuss details of the experimental setup and present a thorough…
We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…
We investigate triatomic molecules that consist of two ground state atoms and a highly excited Rydberg atom, bound at large internuclear distances of thousands of \AA ngstroms. In the molecular state the Rydberg electron is in a…