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Fulfilling the potential of the colloidal semiconductor quantum dots (QDs) in electrically driven applications remains a challenge largely since operation of such devices involves charged QDs with drastically different photo-physical…

Colloidal semiconductor quantum dots are robust emitters implemented in numerous prototype and commercial optoelectronic devices. However, active fluorescence color tuning, achieved so far by electric-field induced Stark effect, has been…

Mesoscale and Nanoscale Physics · Physics 2023-05-16 Yonatan Ossia , Adar Levi , Yossef E. Panfil , Somnath Koley , Einav Scharf , Nadav Chefetz , Sergei Remennik , Atzmon Vakahi , Uri Banin

Hexagonal boron nitride is a van der Waals material that hosts visible-wavelength quantum emitters at room temperature. However, experimental identification of the quantum emitters' electronic structure is lacking, and key details of their…

Creation of defect with predetermined optical, chemical and other characteristics is a powerful tool to enhance the functionalities of materials. Herewith, we utilize density functional theory to understand the microscopic mechanisms of…

Materials Science · Physics 2022-08-31 P. Huang , M. Grzeszczyk , K. Vaklinova , K. Watanabe , T. Taniguchi , K. S. Novoselov , M. Koperski

Precise control over the electronic and optical properties of defect centers in solid-state materials is necessary for their applications as quantum sensors, transducers, memories, and emitters. In this study, we demonstrate, from first…

Quantum Physics · Physics 2021-05-07 Derek S. Wang , Susanne F. Yelin , Johannes Flick

We study the carbon dimer defect in a hexagonal boron-nitride monolayer using the GW and Bethe-Salpeter many-body perturbation theories within a finite size cluster approach. While quasiparticle energies converge very slowly with system…

Mesoscale and Nanoscale Physics · Physics 2021-10-04 Michael Winter , Manon H. E. Bousquet , Denis Jacquemin , Ivan Duchemin , Xavier Blase

The research focuses on the explanation of a phenomenon observed in the spectra of electron nuclear resonance (ENDOR) pertaining to nitrogen atoms adjacent to the boron vacancy (VB) defect in hexagonal boron nitride (hBN). The phenomenon is…

Materials Science · Physics 2025-02-13 G. V. Mamin , E. V. Dmitrieva , F. F. Murzakhanov , I. N. Gracheva , V. A. Soltamov , M. R. Gafurov

Neutral silicon vacancy (SiV0) centers in diamond are promising candidates for quantum networks because of their excellent optical properties and long spin coherence times. However, spin-dependent fluorescence in such defects has been…

Spin-dependent optical transitions are attractive for a plethora of applications in quantum technologies. Here we report on utilization of high quality ring resonators fabricated from TiO2 to enhance the emission from negatively charged…

Hexagonal boron nitride (hBN) is a wide band gap material with both strong excitonic light emission in the ultraviolet and strong exciton-phonon coupling. Luminescence experiments performed on the recently synthesized monolayer form (m-hBN)…

Materials Science · Physics 2023-02-28 Pierre Lechifflart , Fulvio Paleari , Davide Sangalli , Claudio Attaccalite

Quantum emitters in layered materials are promising candidates for applications in nanophotonics. Here we present a technique based on charge transfer to graphene for measuring the charge transition levels ($\rm E_t$) of fluorescent defects…

Materials Science · Physics 2019-07-02 Zai-Quan Xu , Noah Mendelson , John A. Scott , Chi Li , Igor Aharonovich , Milos Toth

Ultraviolet (UV) quantum emitters in hexagonal boron nitride (hBN) have generated considerable interest due to their outstanding optical response. Recent experiments have identified a carbon impurity as a possible source of UV single photon…

Quantum Physics · Physics 2021-11-19 Song Li , Anton Pershin , Gergő Thiering , Péter Udvarhelyi , Adam Gali

Recent observation of quantum emitters in monolayers of hexagonal boron nitride (h-BN) has provided a novel platform for optomechanical experiments where the single-photon emitters can couple to the motion of freely suspended h-BN membrane.…

Quantum Physics · Physics 2019-01-17 Mehdi Abdi , Martin B. Plenio

Single photon emitter (SPE) sources are important building blocks for photonics-based quantum technologies. Recently, the highly bright and versatile SPEs from the two-dimensional insulator material hexagonal boron nitride (hBN) have…

Mesoscale and Nanoscale Physics · Physics 2021-08-05 Yifeng Chen , Su Ying Quek

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

Atomic Physics · Physics 2021-06-02 Yimeng Wang , Chris H. Greene

A fundamental building block in nano-photonics is the ability to directionally excite highly squeezed optical mode dynamically, particularly with an electrical bias. Such capabilities would enable the active manipulation of light…

Optics · Physics 2018-02-26 Yuyu Jiang , Xiao Lin , Tony Low , Baile Zhang , Hongsheng Chen

The strong excitonic emission at 5.75 eV of hexagonal boron nitride (h-BN) makes this material one of the most promising candidate for light emitting devices in the far ultraviolet (UV). However, single excitons occur only in perfect…

Intense "blue-green" phosphorescence is commonly observed in near colourless lab-grown high-pressure high-temperature (HPHT) diamonds following optical excitation at or above the indirect bandgap. We have employed a holistic combination of…

Materials Science · Physics 2023-06-06 Jiahui Zhao , Ben L. Green , Ben G. Breeze , Mark E. Newton

The defect-mediated hexagonal boron nitride (hBN) supercell display the visible optical spectra and electronic characteristics. The defects in the hBN supercell include the atomic vacancy, antisite, antisite vacancy, and substitution of a…

Materials Science · Physics 2019-12-13 Sheng Yu , Bagher Tabibi , Qiliang Li , Felix Jaetae Seo

In recent years, mono-layers and multi-layers of hexagonal boron nitride (hBN) have been demonstrated as host materials for localized atomic defects that can be used as emitters for ultra-bright, non-classical light. The origin of the…

Quantum Physics · Physics 2019-07-18 Alexander Bommer , Christoph Becher