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We calculate the two-photon absorption in bulk and single layer hexagonal boron nitride (hBN) both by an ab-initio real-time Bethe-Salpeter approach and by a the real-space solution of the excitonic problem in tight-binding formalism. The…

Materials Science · Physics 2018-10-17 Claudio Attaccalite , Myrta Grüning , Hakim Amara , Sylvain Latil , François Ducastelle

Controlling and manipulating individual quantum systems in solids underpins the growing interest in development of scalable quantum technologies. Recently, hexagonal boron nitride has garnered significant attention in quantum photonic…

Substitutional carbon defects in hexagonal boron nitride (hBN) are prominent single photon emitters (SPEs), and their potential for spin activity ($S\geq1$) is particularly intriguing. While studies have largely focused on intra-layer…

Materials Science · Physics 2025-06-03 Ignacio Chacon , Andrea Echeverri , Carlos Cardenas , Francisco Munoz

The active driving of the electron spin of a color center is known as a method for the hyperpolarization of the surrounding nuclear spin bath and to initialize a system with large number of spins. Here, we investigate the efficiency of this…

Quantum Physics · Physics 2023-08-15 F. T. Tabesh , M. Fani , J. S. Pedernales , M. B. Plenio , M. Abdi

Control over the charge states of color centers in solids is necessary in order to fully utilize them in quantum technologies. However, the microscopic charge dynamics of deep defects in wide-bandgap semiconductors are complex, and much…

Mesoscale and Nanoscale Physics · Physics 2021-09-08 A. Gardill , I. Kemeny , M. C. Cambria , Y. Li , H. T. Dinani , A. Norambuena , J. R. Maze , V. Lordi , S. Kolkowitz

We investigate optical nonlinearities that are induced and enhanced due to the strong phonon resonance in hexagonal boron nitride. We predict and observe large sub-picosecond duration signals due to four-wave mixing (FWM) during resonant…

Hyperbolic phonon polaritons (HPhPs) in hexagonal boron nitride (hBN) enable the direct manipulation of mid-infrared light at nanometer scales, many orders of magnitude below the free-space light wavelength. High resolution monochromated…

We propose that the carbon dimer defect in hexagonal boron nitride gives rise to the ubiquitous narrow luminescence band with a zero-phonon line of 4.08 eV (usually labeled the 4.1 eV band). Our first-principles calculations are based on…

Hexagonal boron nitride (hBN) is an emerging two dimensional material for quantum photonics owing to its large bandgap and hyperbolic properties. Here we report a broad range of multicolor room temperature single photon emissions across the…

The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…

In the case of Li-intercalated hexagonal boron nitride bilayer (Li-hBN), the vertex corrections of electron-phonon interaction cannot be omitted. This is evidenced by the very high value of the ratio $\lambda\omega_{D}/\varepsilon_{F}\sim…

Superconductivity · Physics 2020-01-24 K. A. Szewczyk , I. A. Domagalska , A. P. Durajski , R. Szczęśniak

We present comprehensive optical studies of recently discovered single photon sources in boron nitride, which appear in form of narrow lines emitting centres. Here, we aim to compactly characterise their basic optical properties, including…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Maciej Koperski , Karol Nogajewski , Marek Potemski

Color centers in h-BN are among the brightest emission centers known yet the origins of these emission centers are not well understood. Here, using first-principles calculations in combination with the generating function method, we…

Materials Science · Physics 2021-08-17 Christopher Linderälv , Witlef Wieczorek , Paul Erhart

Monolayer transition metal dichalcogenide semiconductors, with versatile experimentally accessible exciton species, offer an interesting platform for investigating the interaction between excitons and a Fermi sea of charges. Using hexagonal…

Mesoscale and Nanoscale Physics · Physics 2020-08-18 Thomas Goldstein , Yueh-Chun Wu , Shao-Yu Chen , Takashi Taniguchi , Kenji Watanabe , Kalman Varga , Jun Yan

We theoretically analyze the carrier capture and distribution among the available energy levels of a symmetric semiconductor quantum dot under continuous-wave excitation resonant with the barrier energy levels. At low temperature all the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 G. Pistone , S. Savasta , O. Di Stefano , G. Martino , R. Girlanda , S. Portolan

Polarons can control carrier mobility and can also be used in the design of quantum devices. Although much effort has been directed into investigating the nature of polarons, observation of defect-related polarons is challenging due to…

Materials Science · Physics 2024-09-11 Takuto Ichikawa , Junjie Guo , Paul Fons , Dwi Prananto , Toshu An , Muneaki Hase

The optical emission spectra of semiconducting transition-metal dichalcogenide monolayers highlight fascinating recombination processes of charged excitons (trions). When charge tunable WSe$_2$ monolayers are moderately doped with…

Mesoscale and Nanoscale Physics · Physics 2025-01-22 V. Jindal , K. Mourzidis , A. Balocchi , C. Robert , P. Li , D. Van Tuan , L. Lombez , D. Lagarde , P. Renucci , T. Taniguchi , K. Watanabe , H. Dery , X. Marie

The positively charged nitrogen vacancy (NV+) centre in diamond has been traditionally treated as a dark state due to the experimental lack of an optical signature. Recent computational studies have shown that it is possible for the NV+…

Mesoscale and Nanoscale Physics · Physics 2022-01-05 Akib Karim , Igor Lyskov , Salvy P. Russo , Alberto Peruzzo

In this work, robustness of controlled density of optical states in doubly driven artificial atoms is studied under phonon dissipation. By using both perturbative and polaron approaches, we investigate the influence of carrier-phonon…

Quantum Physics · Physics 2020-10-07 David F. Macias-Pinilla , Hanz Y. Ramírez

Low temperature photoluminescence spectra of a color center in hexagonal boron nitride are analyzed. The acoustic phonon sideband can be described by a deformation coupling proportional to strain to a phonon bath that is effectively two…

Mesoscale and Nanoscale Physics · Physics 2019-09-25 P. Khatri , I. J. Luxmoore , A. J. Ramsay