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Solid-phase photo-processes involving icy dust grains greatly affect the chemical evolution of the interstellar medium by leading to the formation of complex organic molecules and by inducing photodesorption. So far, the focus of laboratory…

Context. Recent Monte Carlo simulations and laboratory studies of interstellar ices have proposed an alternative pathway involving the radical-molecule H-atom abstraction reaction in the overall mechanism of methanol (CH3OH) formation in…

Astrophysics of Galaxies · Physics 2026-01-14 K. -Y. Huang , E. Méndez-Robayo , S. Viti , Mario -A. Higuera -G

We investigate the formation and evolution of interstellar dust-grain ices under dark-cloud conditions, with a particular emphasis on CO2. We use a three-phase model (gas/surface/mantle) to simulate the coupled gas--grain chemistry,…

Astrophysics of Galaxies · Physics 2015-05-28 Robin T. Garrod , Tyler Pauly

We present the results of astrochemical modeling of complex organic molecules (COMs) in the ice and gas of the prestellar core L1544 with the recently updated MONACO rate equations-based model. The model includes, in particular,…

Observations of star forming environments revealed that the abundances of some deuterated interstellar molecules are markedly larger than the cosmic D/H ratio of 10-5. Possible reasons for this pointed to grain surface chemistry. How- ever,…

Solar and Stellar Astrophysics · Physics 2015-05-28 S. Cazaux , P. Caselli , M. Spaans

Context. Among the most significant chemical functional groups of interstellar molecules are the class of nitriles, which are proposed as key prebiotic molecules due to their chemical connection to the peptide bond after hydrolysis. CN…

Astrophysics of Galaxies · Physics 2025-07-16 Joan Enrique-Romero , Thanja Lamberts

Context. The molecular composition of interstellar ice mantles is defined by gas-grain processes in molecular clouds, with the main components being $H_2O$, $CO$, and $CO_2$. $CH_3OH$ ice is detected towards the denser regions, where large…

Astrophysics of Galaxies · Physics 2021-08-25 B. Müller , B. M. Giuliano , M. Goto , P. Caselli

Interstellar complex organic molecules (COMs) are commonly observed during star formation, and are proposed to form through radical chemistry in icy grain mantles. Reactions between ions and neutral molecules in ices may provide an…

Instrumentation and Methods for Astrophysics · Physics 2016-10-05 Jennifer B. Bergner , Karin I. Oberg , Mahesh Rajappan , Edith C. Fayolle

Context. In dense clouds, hydrogenation reactions on icy dust grains are key in the formation of molecules, like formaldehyde, methanol, and complex organic molecules (COMs). These species form through the sequential hydrogenation of CO…

Solar and Stellar Astrophysics · Physics 2018-09-28 K. -J. Chuang , G. Fedoseev , D. Qasim , S. Ioppolo , E. F. van Dishoeck , H. Linnartz

Methane is one of the simplest stable molecules that is both abundant and widely distributed across space. It is thought to have partial origin from interstellar molecular clouds, which are near the beginning of the star formation cycle.…

Solar and Stellar Astrophysics · Physics 2020-04-16 D. Qasim , G. Fedoseev , K. -J. Chuang , J. He , S. Ioppolo , E. F. van Dishoeck , H. Linnartz

Recent astronomical observations have shown that interstellar complex organic molecules (COMs) exist even in cold environments ($\sim$10 K), while various interstellar COMs have conventionally been detected in the hot gas ($\gtrsim$ 100 K)…

Astrophysics of Galaxies · Physics 2023-08-11 Yu Komatsu , Kenji Furuya

We present a computational study into the adsorption properties of CO$_2$ on amorphous and crystalline water surfaces under astrophysically relevant conditions. Water and carbon dioxide are two of the most dominant species in the icy…

Astrophysics of Galaxies · Physics 2017-09-13 L. J. Karssemeijer , G. A. de Wijs , H. M. Cuppen

Peptide bonds (N-C=O) play a key role in metabolic processes since they link amino acids into peptide chains or proteins. Recently, several molecules containing peptide-like bonds have been detected across multiple environments in the…

Solar and Stellar Astrophysics · Physics 2017-12-27 David Quénard , Izaskun Jiménez-Serra , Serena Viti , Jon Holdship , Audrey Coutens

Formaldehyde (H2CO) is one of the most abundant molecules observed in the icy mantle covering interstellar grains. Studying its evolution can contribute to our understanding of the formation of complex organic molecules in various…

Astrophysics of Galaxies · Physics 2020-09-14 Lei Song , Johannes Kästner

The geometrical structures of singlet or triplet NCH3 molecules adsorbing on Cu(110) surface with presence of Cu adatoms have been determined by first-principle calculation method. The two distinguishable structures match the patterns of…

Materials Science · Physics 2016-06-28 Po-Tuan Chen

Methanol and formaldehyde are two simple organic molecules that are ubiquitously detected in the interstellar medium. An origin in the solid phase and a subsequent nonthermal desorption into the gas phase is often invoked to explain their…

Astrophysics of Galaxies · Physics 2016-04-20 R. Martín-Doménech , G. M. Muñoz Caro , G. A. Cruz-Díaz

The recent unexpected detection of terrestrial complex organic molecules in the cold (~ 10 K) gas has cast doubts on the commonly accepted formation mechanisms of these species. Standard gas-phase mechanisms are inefficient and tend to…

Astrophysics of Galaxies · Physics 2016-03-02 Aurore Bacmann , Alexandre Faure

The simultaneous detection of organic molecules of the form C$_2$H$_{\text{n}}$O, such as ketene (CH$_2$CO), acetaldehyde (CH$_3$CHO), and ethanol (CH$_3$CH$_2$OH), toward early star-forming regions offers hints of shared chemical history.…

Astrophysics of Galaxies · Physics 2021-06-16 K. -J. Chuang , G. Fedoseev , C. Scirè , G. A. Baratta , C. Jäger , Th. Henning , H. Linnartz , M. E. Palumbo

New insights into the formation of interstellar formamide, a species of great relevance in prebiotic chemistry, are provided by electronic structure and kinetic calculations for the reaction NH2 + H2CO -> NH2CHO + H. Contrarily to what…

Astrophysics of Galaxies · Physics 2015-08-19 V. Barone , C. Latouche , D. Skouteris , F. Vazart , N. Balucani , C. Ceccarelli , B. Lefloch

N-bearing molecules (like N2H+ or NH3) are excellent tracers of high-density, low-temperature regions like dense cloud cores and could shed light into snowlines in protoplanetary disks and the chemical evolution of comets. However,…

Astrophysics of Galaxies · Physics 2023-12-01 S. Kakkenpara Suresh , F. Dulieu , J. Vitorino , P. Caselli