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The reactivity of interstellar carbon atoms (C) on the water-dominated ices is one of the possible ways to form interstellar complex organic molecules (iCOMs). In this work, we report a quantum chemical study of the coupling reaction of C…

Astrophysics of Galaxies · Physics 2023-10-24 Stefano Ferrero , Cecilia Ceccarelli , Piero Ugliengo , Mariona Sodupe , Albert Rimola

The mobility of lighter species on the surface of interstellar dust grains plays a crucial role in forming simple through complex molecules. Carbon monoxide is one of the most abundant molecules, its surface diffusion on the grain surface…

Astrophysics of Galaxies · Physics 2022-03-30 Kinsuk Acharyya

CO2 is one of the dominant components of the interstellar ice. Recent observations show CO2 exists more abundantly in polar (H2O-dominated) ice than in apolar (H2O-poor) ice. CO2 ice formation is primarily attributed to the reaction between…

Astrophysics of Galaxies · Physics 2023-09-06 Germán Molpeceres , Joan Enrique-Romero , Yuri Aikawa

Carbon ($^3$P) atom is a reactive species that, according to laboratory experiments and theoretical calculations, condensates with interstellar ice components. This fact is of uttermost importance for the chemistry in the interstellar…

Astrophysics of Galaxies · Physics 2023-07-19 Stefano Ferrero , Cecilia Ceccarelli , Piero Ugliengo , Mariona Sodupe , Albert Rimola

Major components of ices on interstellar grains in molecular clouds - water and carbon oxides - occur at various optical depths. This implies that selective desorption mechanisms are at work. An astrochemical model of a contracting low-mass…

Astrophysics of Galaxies · Physics 2015-06-23 Juris Kalvans

We report new computational and experimental evidence of an efficient and astrochemically relevant formation route to formaldehyde (H$_2$CO). This simplest carbonylic compound is central to the formation of complex organics in cold…

The mobility of atoms, molecules and radicals in icy grain mantles regulate ice restructuring, desorption, and chemistry in astrophysical environments. Interstellar ices are dominated by H2O, and diffusion on external and internal (pore)…

The interaction of carbon atoms with solid carbon monoxide (CO) is a fundamental process in astrochemistry, influencing the formation of complex organic molecules in interstellar environments. This study investigates the adsorption and…

Astrophysics of Galaxies · Physics 2025-09-23 Masashi Tsuge , Germán Molpeceres , Ryota Ichimura , Hideko Nomura , Kenji Furuya , Naoki Watanabe

The successive addition of H atoms to CO in the solid phase has been hitherto regarded as the primary route to form methanol in dark molecular clouds. However, recent Monte Carlo simulations of interstellar ices alternatively suggested the…

Astrophysics of Galaxies · Physics 2022-06-15 Julia C. Santos , Ko-Ju Chuang , Thanja Lamberts , Gleb Fedoseev , Sergio Ioppolo , Harold Linnartz

We sought to determine which are the main hydrogenation paths of acetaldehyde (CH3CHO). As a partially unsaturated molecule, CH3CHO can have links with more hydrogenated species, like ethanol (C2H5OH) or with more unsaturated ones, like…

Astrophysics of Galaxies · Physics 2025-02-26 Germán Molpeceres , Thanh Nguyen , Yasuhiro Oba , Naoki Watanabe

The formation pathways of sulfur-bearing species in the interstellar medium are crucial to understand astrochemical processes in cold molecular clouds and to gain new insights about the sulfur budget in these regions. We aim to explore the…

Astrophysics of Galaxies · Physics 2026-02-20 N. Rani , S. Vogt-Geisse , S. Bovino

Solid state astrochemical reaction pathways have the potential to link the formation of small nitrogen-bearing species, like NH3 and HNCO, and prebiotic molecules, specifically amino acids. To date, the chemical origin of such small…

Astrophysics of Galaxies · Physics 2017-05-26 Gleb Fedoseev , Sergio Ioppolo , Dongfeng Zhao , Thanja Lamberts , Harold Linnartz

Complex organic molecules (COMs) have been observed not only in the hot cores surrounding low- and high- mass protostars, but also in cold dark clouds. Therefore, it is interesting to understand how such species can be formed without the…

Astrophysics of Galaxies · Physics 2016-06-06 K. -J. Chuang , G. Fedoseev , S. Ioppolo , E. F. van Dishoeck , H. Linnartz

The interstellar medium (ISM) is all but empty. To date, more than 300 molecules have already been discovered. Because of the extremely low temperature, the gas-phase chemistry is dominated by barrierless exothermic reactions of radicals…

Astrophysics of Galaxies · Physics 2025-06-03 Tobe Vorsselmans , Erik C. Neyts

With the advent of JWST ice observations, dedicated studies on the formation reactions of detected molecules are becoming increasingly important. One of the most interesting molecules in interstellar ice is CO$_2$. Despite its simplicity,…

Astrophysics of Galaxies · Physics 2024-10-22 Atsuki Ishibashi , Germán Molpeceres , Hiroshi Hidaka , Yasuhiro Oba , Thanja Lamberts , Naoki Watanabe

The chemical network governing interstellar sulfur has been the topic of unrelenting discussion for the past decades due to the conspicuous discrepancy between its expected and observed abundances in different interstellar environments.…

Astrophysics of Galaxies · Physics 2024-07-16 Julia C. Santos , Joan Enrique-Romero , Thanja Lamberts , Harold Linnartz , Ko-Ju Chuang

In the coldest (10--20 K) regions of the interstellar medium, the icy surfaces of interstellar grains serve as solid-state supports for chemical reactions. Among their plausible roles, that of third body is advocated, in which the reaction…

Astrophysics of Galaxies · Physics 2023-03-01 Stefano Ferrero , Stefano Pantaleone , Cecilia Ceccarelli , Piero Ugliengo , Mariona Sodupe , Albert Rimola

Explaining the formation pathways of amides on ice-grain mantels is crucial to understanding the prebiotic chemistry in an interstellar medium. In this computational study, we explore different radical-neutral formation pathways for some of…

Astrophysics of Galaxies · Physics 2024-07-10 Gabriela Silva-Vera , Giulia M. Bovolenta , Namrata Rani , Sebastian Vera , Stefan Vogt-Geisse

Molecular clouds are the cold regions of the Milky Way where stars form. They are enriched by rather complex molecules. Many of these molecules are believed to be synthesized on the icy surfaces of the interstellar submicron-sized dust…

Astrophysics of Galaxies · Physics 2020-07-08 Stefano Pantaleone , Joan Enrique-Romero , Cecilia Ceccarelli , Piero Ugliengo , Nadia Balucani , Albert Rimola

On the surface of icy dust grains in the dense regions of the interstellar medium a rich chemistry can take place. Due to the low temperature, reactions that proceed via a barrier can only take place through tunneling. The reaction H +…

Astrophysics of Galaxies · Physics 2017-08-31 Thanja Lamberts , Johannes Kästner