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We excite YbF molecules to low-lying vibrational levels of the $A^2\Pi_{1/2}$ state, and of the nearby perturber state sometimes called [18.6]0.5. By dispersing the fluorescence, we measure branching ratios for the radiative decay to…

Atomic Physics · Physics 2015-06-18 I. J. Smallman , F. Wang , T. C. Steimle , M. R. Tarbutt , E. A. Hinds

The fluorescence spectrum resulting from laser excitation of the A^{2}\Pi_{1/2} - X^{2}\Sigma^{+} (0,0) band of ytterbium monofluoride, YbF, has been recorded and analyzed to determine the Franck-Condon factors. The measured values are…

Valuable dynamical and structural information about neat liquid DMSO at ambient conditions can be obtained through study of low frequency vibrations in the far infrared (FIR), that is, terahertz regime. For DMSO, collective excitations as…

Chemical Physics · Physics 2017-09-13 Milan Hazra , Biman Bagchi

Vibrational branching ratios in the B$^2\Sigma^+$ -- X$^2\Sigma^+$ and A$^2\Pi$ -- X$^2\Sigma^+$ optical-cycling transitions of BaH molecules are investigated using measurements and {\it ab initio} calculations. The experimental values are…

Atomic Physics · Physics 2019-08-13 K. Moore , I. C. Lane , R. L. McNally , T. Zelevinsky

We observed the $A^1\Sigma^+\sim b^3\Pi\to a^3\Sigma^+/X^1\Sigma^+$ laser-induced fluorescence (LIF) spectra of the RbCs molecule excited from the ground $X^1\Sigma^+$ state by the Ti:Sapphire laser. The LIF radiation from the common…

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

Aims: We measure transition probabilities for Cr II transitions from the z ^4H_J, z ^2D_J, y ^4F_J, and y ^4G_J levels in the energy range 63000 to 68000 cm^{-1}. Methods: Radiative lifetimes were measured using time-resolved laser-induced…

Solar and Stellar Astrophysics · Physics 2015-05-14 J. Gurell , H. Nilsson , L. Engstrom , H. Lundberg , R. Blackwell-Whitehead , K. E. Nielsen , S. Mannervik

Time resolved detection of laser induced fluorescence from pulsed excitation of electronic states in barium monofluoride (BaF) molecules has been performed in order to determine the lifetimes of the $A^2\Pi_{1/2}$ and $A^2\Pi_{3/2}$ states.…

Molecules containing a lanthanide atom have sets of electronic states arising from excitation of an inner-shell electron. These states have received little attention, but are thought to play an important role in laser cooling of such…

Atomic Physics · Physics 2024-05-28 S. Popa , S. Schaller , A. Fielicke , J. Lim , B. G. Sartakov , M. R. Tarbutt , G. Meijer

A wide variety of feed gases are used to generate low-temperature plasmas for the microelectronics and the sustainability applications. These plasmas often have a complex combination of reactive and non-reactive species which may have…

This work reports new experimental radiative lifetimes and calculated oscillator strengths for transitions of astrophysical interest in singly ionized cobalt. More precisely, nineteen radiative lifetimes in Co+ have been measured with the…

Solar and Stellar Astrophysics · Physics 2016-10-02 P. Quinet , V. Fivet , P. Palmeri , L. Engstrom , H. Hartman , H. Lundberg , H. Nilsson

Extensive information, such as ion temperature and wave-particle interactions, can be obtained by direct measurement of ion distribution functions using laser-induced fluorescence (LIF). This nonintrusive plasma diagnostic provides an…

Plasma Physics · Physics 2019-04-24 F. Chu , F. Skiff

When optically excited, iodine absorbs in the 490- to 650-nm visible region of the spectrum and, after radiative relaxation, it displays an emission spectrum of discrete vibrational bands at moderate resolution. This makes laser-induced…

Physics Education · Physics 2015-07-10 S. B. Bayram , M. V. Freamat

We measure the upper state lifetime and two ratios of vibrational branching fractions f_{v'v} on the B^{3}\Pi_{1}(v') - X^{1}\Sigma^{+}(v) transition of TlF. We find the B state lifetime to be 99(9) ns. We also determine that the…

Atomic Physics · Physics 2013-05-30 L. R. Hunter , S. K. Peck , A. S. Greenspon , S. Saad Alam , D. DeMille

New branching fraction measurements based primarily on data from a cross dispersed echelle spectrometer are reported for 84 lines of Co II. The branching fractions for 82 lines are converted to absolute atomic transition probabilities using…

Solar and Stellar Astrophysics · Physics 2018-10-10 J. E. Lawler , T. Feigenson , C. Sneden , J. J. Cowan , G. Nave

Vacuum-ultraviolet (VUV) photoabsorption spectra were recorded of the $A\,{}^2\Sigma^+(v'=0)\leftarrow{}X\,{}^2\Pi(v''=0)$, $D\,{}^2\Sigma^-(v'=0)\leftarrow{}X\,{}^2\Pi(v''=0)$ and $D\,{}^2\Sigma^-(v'=1)\leftarrow{}X\,{}^2\Pi(v''=0)$ bands…

We have performed high resolution spectroscopy of rubidium with a single mode continuous wave distributed feedback (DFB) laser diode. The saturation spectrum of the D_2-line of 85Rb and 87Rb was recorded with a resolution close to the…

Atomic Physics · Physics 2015-06-26 S. Kraft , A. Deninger , Ch. Truck , J. Fortagh , F. Lison , C. Zimmermann

We report lifetime measurements of the 6 levels in the 3d6(5D)4d e6G term in Fe ii at an energy of 10.4 eV, and f -values for 14 transitions from the investigated levels. The lifetimes were measured using time-resolved laser-induced…

Solar and Stellar Astrophysics · Physics 2016-10-31 H. Hartman , H. Nilsson , L. Engström , H. Lundberg

This work reports new experimental radiative lifetimes and calculated oscillator strengths for transitions from 3d8 4d levels of astrophysical interest in singly ionized nickel. Radiative lifetimes of seven high-lying levels of even parity…

Solar and Stellar Astrophysics · Physics 2017-04-12 H. Hartman , L. Engstrom , H. Lundberg , H. Nilsson , P. Quinet , V. Fivet , P. Palmeri , G. Malcheva , K. Blagoev

Alkaline earth monoalkoxide free radicals (MORs) have molecular properties conducive to direct laser cooling to sub-millikelvin temperatures. Using dispersed laser induced fluorescence (DLIF) measurements from a pulsed supersonic molecular…

Atomic Physics · Physics 2019-05-22 Ivan Kozyryev , Timothy C. Steimle , Phelan Yu , Duc-Trung Nguyen , John M. Doyle
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