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The structural degrees of freedom of a material are the various distortions most straightforwardly activated by external stimuli. A highly successful design strategy in materials chemistry involves controlling these individual distortions…

Materials Science · Physics 2020-11-30 Hanna L. B. Boström , Andrew L. Goodwin

The defect-activity in halide perovskites remains a critical factor for the application in optoelectronics. The imperfections (vacancies, anti-sites, interstitials) formed in the lattice of the halide perovskites were considered as a main…

In hybrid perovskites, the organic molecules and inorganic frameworks exhibit distinct static and dynamic characteristics. Their coupling will lead to unprecedented phenomena, which have attracted wide research interests. In this paper, we…

Materials Science · Physics 2022-09-28 Ping Tuo , Lei Li , Xiaoxu Wang , Bo Xu , Jianhui Chen , Zhicheng Zhong , Fu-Zhi Dai

We report the results of comprehensive study of the critical dynamics of the prototype perovskite antiferroelectric PbZrO$_3$. The combination of inelastic X-ray and diffuse X-ray scattering techniques and Brillouin light scattering was…

We report observation of coherent oscillations in the relaxation dynamics of an exciton-polariton condensate driven by parametric scattering processes. As a result of the interbranch scattering scheme and the nonlinear polariton-polariton…

Quantum entanglement between the spin, orbital, and lattice degrees of freedom in condensed matter systems can emerge due to an interplay between spin-orbit and vibronic interactions. Heavy transition metal ions decorated on a face-centered…

Neutron scattering investigations were carried out in PbMg$_{1/3}$Ta$_{2/3}$O$_3$ and BaMg$_{1/3}$Ta$_{2/3}$O$_3$ complex perovskites. The crystal structure of both compounds does not show any phase transition in the temperature range 1.5…

Materials Science · Physics 2007-05-23 S. N. Gvasaliya , B. Roessli , D. Sheptyakov , S. G. Lushnikov , T. A. Shaplygina

We report a strongly temperature dependent luminescence Stokes shift in the electronic spectra of both hybrid and inorganic lead-bromide perovskite single crystals. This behavior stands in stark contrast to that exhibited by more…

Materials Science · Physics 2018-04-05 Yinsheng Guo , Omer Yaffe , Trevor D. Hull , Jonathan S. Owen , David R. Reichman , Louis E. Brus

We study the non-equilibrium structural dynamics of the incommensurate and nearly-commensurate charge-density wave phases in 1T-TaS$_2$. Employing ultrafast low-energy electron diffraction (ULEED) with 1 ps temporal resolution, we…

Electronic properties and lattice vibrations are supposed to be strongly correlated in metal-halide perovskites, due to the "soft" fluctuating nature of their crystal lattice. Thus, unveiling electron-phonon coupling dynamics upon…

We demonstrate a novel approach to the structural and electronic property modification of perovskites, focusing on Pr$_2$CuO$_4$, an undoped parent compound of a class of electron-doped copper-oxide superconductors. Currents were passed…

Lead-free antiferroelectric perovskite $\rm AgNbO_3$ is nowadays attracting extensive research interests due to its promising applications in energy storage. Although great progress has been made in optimizing the material performance,…

Materials Science · Physics 2025-11-18 Huazhang Zhang , Konstantin Shapovalov , Safari Amisi , Philippe Ghosez

The lattice dynamics of coesite has been studied by a combination of diffuse x-ray scattering, inelastic x-ray scattering and an ab initio lattice dynamics calculation. The combined technique gives access to the full lattice dynamics in…

Real-time dynamics of charge density and lattice displacements is studied during photoinduced ionic-to-neutral phase transitions by using a one-dimensional extended Peierls-Hubbard model with alternating potentials for the one-dimensional…

Materials Science · Physics 2009-11-07 Naoyuki Miyashita , Makoto Kuwabara , Kenji Yonemitsu

Perovskite materials are at the forefront of modern materials science due to their exceptional structural, electronic, and optical properties. The controlled fabrication of perovskite nanostructures is crucial for enhancing their…

The bandgap tunability of mixed-halide perovskites makes them promising candidates for light emitting diodes and tandem solar cells. However, illuminating mixed-halide perovskites results in the formation of segregated phases enriched in a…

In two-dimensional hybrid organic-inorganic metal-halide perovskites, the intrinsic optical lineshape reflects multiple excitons with distinct binding energies, each dressed differently by the hybrid lattice. Given this complexity, a…

We report structural evidence of dynamic reorganization in vortex matter in clean NbSe$_2$ by joint small angle neutron scattering and ac-susceptibility measurements. The application of oscillatory forces in a transitional region near the…

Superconductivity · Physics 2015-08-12 M. Marziali Bermúdez , M. R. Eskildsen , M. Bartkowiak , G. Nagy , V. Bekeris , G. Pasquini

Spintronics in halide perovskites has drawn significant attention in recent years, due to highly tunable spin-orbit fields and intriguing interplay with lattice symmetry. Spin lifetime -- a key parameter that determines the applicability of…

Materials Science · Physics 2023-10-25 Junqing Xu , Kejun Li , Uyen N. Huynh , Jinsong Huang , Ravishankar Sundararaman , Valy Vardeny , Yuan Ping

Some layered silicates are composed of positive ions, surrounded by layers of ions with opposite sign. Mica muscovite is a particularly interesting material, because there exist fossil and experimental evidence for nonlinear excitations…

Pattern Formation and Solitons · Physics 2018-08-28 Juan F. R. Archilla , Yaroslav Zolotaryuk , Yuriy A. Kosevich , Yusuke Doi