Related papers: Efficient and robust chiral resolution by composit…
In this work, we propose a composite pulses scheme by modulating phases to achieve high fidelity population transfer in three-level systems. To circumvent the obstacle that not enough variables are exploited to eliminate the systematic…
In this work, we exploit the idea of composite pulses to achieve robust population inversion in a three-level quantum system. The scheme is based on the modulation of the coupling strength, while the other physical parameters remain…
Recent advances in engineering and control of nanoscale quantum sensors have opened new paradigms in precision metrology. Unfortunately, hardware restrictions often limit the sensor performance. In nanoscale magnetic resonance probes, for…
Attosecond science is an emerging topic where chirality plays a central role. Here we demonstrate subjecting iodoacetylene, a geometrically achiral molecule, to a pair of simulated non-ionizing ultrafast circularly polarized laser pulses at…
We introduce chiral rotational spectroscopy: a new technique that enables the determination of the orientated optical activity pseudotensor components $B_{XX}$, $B_{YY}$ and $B_{ZZ}$ of chiral molecules, in a manner that reveals the…
We implement an ensemble quantum counting algorithm on three NMR spectrometers with 1H resonance frequencies of 500, 600 and 750 MHz. At higher frequencies, the results deviate markedly from naive theoretical predictions. These systematic…
The control of qubit states is often impeded by systematic control errors. Compensating pulse sequences have emerged as a resource efficient method for quantum error reduction. In this review, we discuss compensating composite pulse…
We consider pulses of finite duration for coherent control in the presence of classical noise. We derive the corrections to ideal, instantaneous pulses for the case of general decoherence (spin-spin relaxation and spin-lattice relaxation)…
Many chirality-sensitive light-matter interactions are governed by chiral electron dynamics. Therefore, the development of advanced technologies harnessing chiral phenomena would critically benefit from measuring and controlling chiral…
Circular dichroism (CD), arising from spin-selective light-matter interactions controlled by chirality, is critical for advanced applications such as chiral imaging and ultrasensitive biosensing. However, CD of chiral natural materials is…
This PhD thesis is a first step towards the control of the quantum corrections in the Resonance Chiral Theory, the suggested framework to handle QCD in the resonance region. After a theoretical introduction, Chapter 3 is devoted to…
Using a model methane-like chiral system, we theoretically demonstrate a possibility to access photoelectron circular dichroism (PECD) by a single experiment with two overlapping laser pulses of carrier frequencies $\omega$ and $2\omega$,…
Four-dimensional imaging of charge migration is crucial to the understanding of several ubiquitous processes in nature. The present work focuses on imaging of charge migration in an oriented epoxypropane: a chiral molecule. A linearly…
Composite pulses, which produce ultrabroadband, ultranarrowband and ultrapassband $x$-, $y$-) rotations by $\theta = \pi$ on the Bloch-Poincar\'e sphere, are presented. The first class plays a role for design of achromatic polarisation…
Chiral emission, where the handedness of a transition dipole determines the direction in which a photon is emitted, has recently been observed from atoms and quantum dots coupled to nanophotonic waveguides. Here, we consider the case of…
Electronic circular dichroism (ECD) spectroscopy captures the chiroptical response of molecules, enabling absolute configuration assignment that is vital for enantioselective synthesis and drug design. The practical use of ECD spectra in…
State-selective enantiomeric excess is realized using microwave-driven coherent population transfer. The method selectively promotes either R or S molecules to a higher rotational state by phase-controlled microwave pulses that drive…
The chiral anomaly is a fundamental property of quantum chromodynamics (QCD). It governs the transition amplitudes for processes involving an odd number of Goldstone bosons of chiral symmetry breaking. In case of the coupling of three pions…
We study corrections to the Heisenberg interaction between several lateral, single-electron quantum dots. We show, using exact diagonalization, that three-body chiral terms couple triangular configurations to external sources of flux rather…
We present an improvement to the cross resonance gate realized with the addition of resonant, target rotary pulses. These pulses, applied directly to the target qubit, are simultaneous to and in phase with the echoed cross resonance pulses.…