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Understanding the electronic structure of actinide materials is crucial for both fundamental research and nuclear applications. The partially filled 5f shells exhibit complex behavior due to strong correlations and ligand hybridization,…

We have investigated the electronic structure of Ba3InIr2O9 within the density-functional theory (DFT) using the generalized gradient approximation while considering strong Coulomb correlations (GGA+$U$) in the framework of the fully…

Strongly Correlated Electrons · Physics 2025-02-26 D. A. Kukusta , L. V. Bekenov , V. N. Antonov

Resonant Inelastic X-ray Scattering (RIXS) was used to measure the local electronic structure in few-layer exfoliated flakes of the van der Waals antiferromagnet NiPS$_3$. The resulting spectra show a systematic softening and broadening of…

Strongly Correlated Electrons · Physics 2024-02-09 M. F. DiScala , D. Staros , A. de la Torre , A. Lopez , D. Wong , C. Schulz , M. Bartkowiak , B. Rubenstein , K. W. Plumb

The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and…

Mesoscale and Nanoscale Physics · Physics 2022-10-27 Nanna Zhou Hagström , Michael Schneider , Nico Kerber , Alexander Yaroslavtsev , Erick Burgos Parra , Marijan Beg , Martin Lang , Christian M. Günther , Boris Seng , Fabian Kammerbauer , Horia Popescu , Matteo Pancaldi , Kumar Neeraj , Debanjan Polley , Rahul Jangid , Stjepan B. Hrkac , Sheena K. K. Patel , Sergei Ovcharenko , Diego Turenne , Dmitriy Ksenzov , Christine Boeglin , Igor Pronin , Marina Baidakova , Clemens von Korff Schmising , Martin Borchert , Boris Vodungbo , Kai Chen , Chen Luo , Florin Radu , Leonard Müller , Miriam Martínez Flórez , André Philippi-Kobs , Matthias Riepp , Wojciech Roseker , Gerhard Grübel , Robert Carley , Justine Schlappa , Benjamin Van Kuiken , Rafael Gort , Laurent Mercadier , Naman Agarwal , Loïc Le Guyader , Giuseppe Mercurio , Martin Teichmann , Jan Torben Delitz , Alexander Reich , Carsten Broers , David Hickin , Carsten Deiter , James Moore , Dimitrios Rompotis , Jinxiong Wang , Daniel Kane , Sandhya Venkatesan , Joachim Meier , Florent Pallas , Tomasz Jezynski , Maximilian Lederer , Djelloul Boukhelef , Janusz Szuba , Krzysztof Wrona , Steffen Hauf , Jun Zhu , Martin Bergemann , Ebad Kamil , Thomas Kluyver , Robert Rosca , Michał Spirzewski , Markus Kuster , Monica Turcato , David Lomidze , Andrey Samartsev , Jan Engelke , Matteo Porro , Stefano Maffessanti , Karsten Hansen , Florian Erdinger , Peter Fischer , Carlo Fiorini , Andrea Castoldi , Massimo Manghisoni , Cornelia Beatrix Wunderer , Eric E. Fullerton , Oleg G. Shpyrko , Christian Gutt , Cecilia Sanchez-Hanke , Hermann A. Dürr , Ezio Iacocca , Hans T. Nembach , Mark W. Keller , Justin M. Shaw , Thomas J. Silva , Roopali Kukreja , Hans Fangohr , Stefan Eisebitt , Mathias Kläui , Nicolas Jaouen , Andreas Scherz , Stefano Bonetti , Emmanuelle Jal

Resonant soft X-ray scattering (RSXS) is a powerful technique for probing both spatial and electronic structures within solid-state systems. We present a newly developed RSXS capability at beamline 13-3 of the Stanford Synchrotron Radiation…

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

We report on the Cu 1s resonant inelastic X-ray scattering (RIXS) of Cu-O one-dimensional (1D) strongly correlated insulator systems with contrasting atomic arrangements, namely edge-sharing CuGeO3 and corner-sharing Sr2CuO3. Owing to good…

Strongly Correlated Electrons · Physics 2009-11-11 S. Suga , S. Imada , A. Higashiya , A. Shigemoto , S. Kasai , M. Sing , H. Fujiwara , A. Sekiyama , A. Yamasaki , C. Kim , T. Nomura , J. Igarashi , M. Yabashi , T. Ishikawa

We report on the most complete investigation to date of the 4f-electron properties at the gamma-alpha transition in elemental Ce by resonant inelastic x-ray scattering (RIXS). The Ce 2p3d-RIXS spectra were measured directly in the bulk…

Strongly Correlated Electrons · Physics 2016-08-16 Jean-Pascal Rueff , Jean-Paul Itié , M. Taguchi , C. F. Hague , J. -M. Mariot , R. Delaunay , J. -P. Kappler , N. Jaouen

The Cu K-edge resonant inelastic x-ray scattering (RIXS) spectrum in one-dimensional insulating cuprates is theoretically examined by using the exact diagonalization technique for the extended one-dimensional Hubbard model with nearest…

Strongly Correlated Electrons · Physics 2016-08-31 K. Tsutsui , T. Tohyama , S. Maekawa

Using a novel ultrahigh resolution ($\Delta E \sim 0.1\,$eV) setup to measure electronic features in x-ray Thomson scattering (XRTS) experiments at the European XFEL in Germany, we have studied the collective plasmon excitation in aluminium…

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

We present a novel derivation of resonant inelastic x-ray scattering (RIXS) which yields an expression for the RIXS cross section in terms of emission pathways between intermediate and final many-body states. Thereby electron-hole…

Materials Science · Physics 2020-10-14 Christian Vorwerk , Francesco Sottile , Claudia Draxl

Periodic structures of phases with orientational order of molecules, but homogenous electron density distribution: a short pitch cholesteric, blue phase and twist-bend nematic phase, were probed by a resonant soft x-ray scattering (RSoXS)…

Soft Condensed Matter · Physics 2017-04-19 Mirosław Salamończyk , Nataša Vaupotič , Damian Pociecha , Cheng Wang , Chenhui Zhu , Ewa Gorecka

The detection of inelastically scattered soft X-rays with high energy resolution usually requires large grating spectrometers. Recently, photoelectron spectrometry for analysis of X-rays (PAX) has been rediscovered for modern spectroscopy…

We present a study of resonant inelastic X-ray scattering (RIXS) spectra collected at the rare-earth $L$ edges of divalent hexaborides YbB$_6$ and EuB$_6$. In both systems, RIXS-active features are observed at two distinct resonances…

Resonant inelastic x-ray scattering (RIXS) has become a very powerful experimental technique to probe a broad range of intrinsic elementary excitations, for example, from low energy phonons and (bi-)magnons to high energy $d$-$d$,…

Strongly Correlated Electrons · Physics 2019-06-20 Y. L. Wang , G. Fabbris , M. P. M. Dean , G. Kotliar

Element- and site-specific resonant inelastic x-ray scattering spectroscopy (RIXS) is employed to investigate electron correlation effects in {$\rm NaV_2O_5$}. In contrast to single photon techniques, RIXS at the vanadium $L_3$ edge is able…

Strongly Correlated Electrons · Physics 2009-11-07 G. P. Zhang , T. A. Callcott , G. T. Woods , L. Lin , Brian Sales , D. Mandrus , J. He

Resonant X-ray scattering (RXS) is a spectroscopy where both the power of site selective diffraction and the power of local absorption spectroscopy regarding atomic species are combined. By virtue of the dependence on the core level state…

Materials Science · Physics 2007-11-12 Yves Joly , Elena S. Nazarenko , José-Emilio Lorenzo , Sergio Di Matteo , Calogero R. Natoli

We theoretically demonstrate that a resonant inelastic x-ray scattering (RIXS) with a sizable momentum transfer can be utilized to study valence band dispersion for broad band materials. We take RIXS at the Si K edge of 3C-SiC as a typical…

Materials Science · Physics 2009-09-21 Yunori Nisikawa , Muneharu Ibuki , Manabu Usuda

We present calculations for resonant inelastic x-ray scattering (RIXS) in edge-shared copper oxide systems, such as CuGeO$_{3}$ and Li$_{2}$CuO$_{2}$, appropriate for hard x-ray scattering where the photoexcited electron lies above oxygen…

Strongly Correlated Electrons · Physics 2009-11-13 F. Vernay , B. Moritz , I. Elfimov , J. Geck , D. Hawthorn , T. P. Devereaux , G. A. Sawatzky