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Active optical waveguides combine light source and waveguides together in an individual component, which are essential for the integrated photonic chips. Although 1D luminescent materials based optical waveguides were extensively…

Organic-inorganic halide perovskite solar cells have recently attracted much attention due to their low-cost fabrication, flexibility, and high-power conversion efficiency. The reduction from three- to two-dimension (2D) promises an…

Materials Science · Physics 2018-07-24 Rahul Singh , Prashant Singh , Ganesh Balasubramanian

Carrier multiplication by singlet exciton fission enhances photovoltaic conversion efficiencies in organic solids. This decay of one singlet exciton into two triplet states promises to overcome the Shockley-Queisser limit as up to two…

Materials Science · Physics 2016-12-16 K. Kolata , S. Marquardt , N. W. Rosemann , A. Mager , A. Hansmann , U. Höfer , R. Berger , T. Breuer , G. Witte , S. Chatterjee

We experimentally investigate the lateral diffusion of dipolar excitons in coupled quantum wells in two (2D) and one (1D) dimensions. In 2D, the exciton expansion obeys non-linear temporal dynamics due to the repulsive dipole pressure at a…

Mesoscale and Nanoscale Physics · Physics 2009-02-02 X. P. Vogele , D. Schuh , W. Wegscheider , J. P. Kotthaus , A. W. Holleitner

Using transient fluorescent spectra at time-zero, we develop a density-resolved fluorescent spectroscopic method for investigating photoproducts in CH3NH3PbI3 perovskite and related photophysics. The density dependent dynamical co-existence…

Materials Science · Physics 2016-11-22 Wei Wang , Yu Li , Xiangyuan Wang , Yanping Lv , Shufeng Wang , Kai Wang , Yantao Shi , Lixin Xiao , Zhijian Chen , Qihuang Gong

Exciton polaritons, hybrid quasiparticles with part-light part-matter nature in semiconductor microcavities, are extensively investigated for striking phenomena such as polariton condensation and quantum emulation. These phenomena have…

Materials Science · Physics 2022-07-27 Tingting Wang , Zhihao Zang , Yuchen Gao , Chao Lyu , Kai Peng , Kenji Watanabe , Takashi Taniguchi , Xiaoze Liu , Wei Bao , Yu Ye

Exciton-phonon interactions govern the optical response of semiconductors, yet disentangling multiple coupling channels in lead halide perovskites remains challenging. We investigate CsPbBr3 microcrystals using photoluminescence, Raman and…

Mesoscale and Nanoscale Physics · Physics 2026-02-19 Pradeepa H. L. , Sagnik Chatterjee , Sayantan Patra , Swapneswar Bisoi , Saqlain Mushtaq , Hardeep , Akshay Singh , Ashish Arora , Atikur Rahman

We present a many-body theory for exciton-trion-polaritons in doped two-dimensional materials. Exciton-trion-polaritons are robust coherent hybrid excitations involving excitons, trions, and photons. Signatures of these polaritons have been…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Farhan Rana , Okan Koksal , Minwoo Jung , Gennady Shvets , A. Nick Vamivakas , Christina Manolatou

Exciton dynamics, lifetimes and scattering are directly related to the exciton dispersion, or bandstructure. While electron and phonon bandstructures are well understood and can be easily calculated from first principles, the exciton…

Materials Science · Physics 2021-10-04 Diana Y. Qiu , Galit Cohen , Dana Novichkova , Sivan Refaely-Abramson

Organic-inorganic halide perovskite solar cells have attracted much attention due to their low-cost fabrication, flexibility, and high-power conversion efficiency. More recent efforts show that the reduction from three- to two-dimensions…

Materials Science · Physics 2021-09-03 Rahul Singh , Prashant Singh , Ganesh Balasubramania

We show that exciton-type transport in certain materials can be dramatically modified by their inclusion in an optical cavity: the modification of the electromagnetic vacuum mode structure introduced by the cavity leads to transport via…

Quantum Physics · Physics 2015-05-22 Johannes Schachenmayer , Claudiu Genes , Edoardo Tignone , Guido Pupillo

While exciton relaxation in transition metal dichalcogenides (TMDs) has been intensively studied, spatial exciton propagation has received only little attention - in spite of being a key process for optoelectronics and having already shown…

Mesoscale and Nanoscale Physics · Physics 2020-01-23 Roberto Rosati , Raül Perea-Causín , Samuel Brem , Ermin Malic

Low-dimensional materials differ from their bulk counterpart in many respects. In particular, the screening of the Coulomb interaction is strongly reduced, which can have important consequences such as the significant increase of exciton…

We demonstrate room temperature optical trapping and generation of high-order angular harmonics in exciton-polariton condensates in a monocrystalline CsPbBr$_3$ perovskite-filled microcavity. Using an annular nonresonant excitation profile…

The interplay of optics, dynamics and transport is crucial for the design of novel optoelectronic devices, such as photodetectors and solar cells. In this context, transition metal dichalcogenides (TMDs) have received much attention. Here,…

Mesoscale and Nanoscale Physics · Physics 2019-11-04 Raul Perea-Causin , Samuel Brem , Roberto Rosati , Roland Jago , Marvin Kulig , Jonas D. Ziegler , Jonas Zipfel , Alexey Chernikov , Ermin Malic

Two-dimensional (2D) heterostructures (HS) formed by transition-metal dichalcogenide (TMDC) monolayers offer a unique platform for the study of intralayer and interlayer excitons as well as moir\'e-pattern-induced features. Particularly,…

Mesoscale and Nanoscale Physics · Physics 2021-11-15 Mohammed Adel Aly , Manan Shah , Lorenz Maximilian Schneider , Kyungnam Kang , Martin Koch , Eui-Hyeok Yang , Arash Rahimi-Iman

Lead halide perovskites show remarkable performance when used in photovoltaic and optoelectronic devices. However, the peculiarities of light-matter interactions in these materials in general are far from being fully explored experimentally…

Other Condensed Matter · Physics 2022-02-24 A. V. Trifonov , S. Grisard , A. N. Kosarev , I. A. Akimov , D. R. Yakovlev , J. Höcker , V. Dyakonov , M. Bayer

Efficient energy transport is highly desirable for organic semiconductor (OSC) devices such as photovoltaics, photodetectors, and photocatalytic systems. However, photo-generated excitons in OSC films mostly occupy highly localized states…

Halide double perovskites with alternating silver and pnictogen cations are an emerging family of photoabsorber materials with robust stability and band gaps in the visible range. However, the nature of optical excitations in these systems…

Materials Science · Physics 2021-02-12 Raisa-Ioana Biega , Marina R. Filip , Linn Leppert , Jeffrey B. Neaton

Two-dimensional (2D) halide perovskites feature a versatile structure, which not only enables the fine-tuning of their optoelectronic properties but also makes them appealing as model systems to investigate the fundamental properties of…