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Excitons, bound electron-hole pairs, in Two-Dimensional Hybrid Organic Inorganic Perovskites (2D HOIPs) are capable of forming hybrid light-matter states known as exciton-polaritons (E-Ps) when the excitonic medium is confined in an optical…

Presence of excitons significantly influence the optoelectronic properties and potential applications of materials. Using combined theoretical and experimental tools, we investigate the absorption spectra of $d^0$ double perovskite oxides…

Exciton-polaritons are unique quasiparticles with hybrid properties of an exciton and a photon, opening ways to realize ultrafast strongly nonlinear systems and inversion-free lasers based on Bose-Einstein polariton condensation. However,…

Perovskites have been the focus of attention due to their multitude of outstanding optoelectronic properties and structural versatility. Two-dimensional halide perovskite such as (C_6H_5C_2H_4NH_3)_2PbI_4, or simply PEPI, forms natural…

Materials Science · Physics 2021-03-04 Tanjung Krisnanda , Qiannan Zhang , Kevin Dini , David Giovanni , Timothy C. H. Liew , Tze Chien Sum

Perovskite microwires are promising candidates for integrated photonic systems due to their strong nonlinear optical response and inherent waveguiding capabilities. In this study, we focus on the directional emission properties of…

The surface chemistry and inter-connectivity within perovskite nanocrystals play a critical role in determining the electronic interactions. They manifest in the Coulomb screening of electron-hole correlations and the carrier relaxation…

Two-dimensional (2D) transition metal dichalcogenides (TMDC) and their moir\'e interfaces have been demonstrated for correlated electron states, including Mott insulators and electron/hole crystals commensurate with moir\'e superlattices.…

Mesoscale and Nanoscale Physics · Physics 2024-01-08 Yusong Bai , Yiliu Li , Song Liu , Yinjie Guo , Jordan Pack , Jue Wang , Cory R. Dean , James Hone , X. -Y. Zhu

Understanding the fine structure of excitons is crucial for optoelectronic and quantum photonic applications of lead halide perovskites. It is demonstrated that polarization-sensitive photon echo spectroscopy in magnetic field provides a…

Halide double perovskites are an emerging class of semiconductors with tremendous chemical and electronic diversity. While their bandstructure features can be understood from frontier-orbital models, chemical intuition for optical…

Materials Science · Physics 2023-09-04 Raisa-Ioana Biega , Yinan Chen , Marina R. Filip , Linn Leppert

Lead-halide perovskite nanocrystals (PNCs) exhibit unique optoelectronic properties, many of which originate from a purported bright-triplet exciton fine-structure. A major impediment to measuring this fine-structure is inhomogeneous…

Mesoscale and Nanoscale Physics · Physics 2022-03-09 Albert Liu

In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek

The growing interest in exciton-polaritons has driven the need to manipulate their motion and engineer their band structures to the forefront of contemporary research. This study explores the band structures that emerge from a spatially…

Optics · Physics 2025-10-09 Xingran Xu , Chunyu Jia , Xin-Xin Yang

Perovskites have attracted much attention due to their remarkable optical properties. While it is well established that excitons dominate their optical response, the impact of higher excitonic states and formation of phonon sidebands in…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 David Feldstein , Raul Perea-Causin , Shuli Wang , Mateusz Dyksik , Kenji Watanabe , Takashi Taniguchi , Paulina Plochocka , Ermin Malic

To assess the potential optoelectronic applications of metal-halide perovskites, it is critical to have a detailed understanding of the nature, strength, and dynamics of the interactions between carriers and the polar lattices. Here, we…

Materials Science · Physics 2022-10-28 Xing He , Naveen Kumar Tailor , Soumitra Satapathi , Jakoah Brgoch , Ding-Shyue Yang

Determining the nature of the optical excited state (excitons or free carriers) in nanostructured materials is crucial for device design, as optoelectronic and photovoltaic technologies require different considerations regarding the…

We study theoretically the exciton Bose-Einstein condensation and exciton vortices in a two-dimensional (2D) perovskite (PEA)2PbI4 monolayer. Combining the first-principles calculations and the Keldysh model, the exciton binding energy of…

Mesoscale and Nanoscale Physics · Physics 2020-11-06 Yingda Chen , Dong Zhang , Kai Chang

We investigate the two-pulse photon echo response of excitons in the mixed lead halide perovskite crystal \sample in dependence on the excitation intensity and polarization of the incident laser pulses. Using spectrally narrow picosecond…

As the bound state of two oppositely charged particles, excitons emerge from optically excited semiconductors as the electronic analogue of a hydrogen atom. In the two-dimensional (2D) case, realized either in quantum well systems or truly…

Optics · Physics 2022-05-13 Tobias Graß , Utso Bhattacharya , Julia Sell , Mohammad Hafezi

Cesium lead bromide (CsPbBr$_3$) is a representative material of the emerging class of lead halide perovskite semiconductors that possess remarkable optoelectronic properties. Its optical properties in the vicinity of the band gap energy…

We theoretically investigate the spin structure and spin dynamics of excitons in bulk lead halide perovskite semiconductors with cubic, tetragonal, and orthorhombic crystal symmetry. The exciton spin structure and its modification by an…

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