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Using an approximate time-dependent density functional theory method, we calculate the absorption and luminescence spectra for hydrogen passivated silicon nanoscale structures with large aspect ratio. The effect of electron confinement in…

Materials Science · Physics 2009-09-27 Y. Wang , R. Q. Zhang , Th. Frauenheim , T. A. Niehaus

Long-lived exciton coherences have been recently observed in photosynthetic complexes via ultrafast spectroscopy, opening exciting possibilities for the study and design of coherent exciton transport. Yet, ambiguity in the spectroscopic…

Photoluminescence is commonly used to identify the electronic structure of individual nanotubes. But, nanotubes naturally occur in bundles. Thus, we investigate photoluminescence of nanotube bundles. We show that their complex spectra are…

Materials Science · Physics 2015-05-13 P. H. Tan , A. G. Rozhin , T. Hasan , P. Hu , V. Scardaci , W. I. Milne , A. C. Ferrari

Two-dimensional halide perovskite nanoplatelets (NPLs) have exceptional light-emitting properties, including wide spectral tunability, ultrafast radiative decays, high quantum yields (QY), and oriented emission. To realize efficient…

We investigate exciton bound-state formation and crystallization effects in two-dimensional electron-hole bilayers. Performing unbiased path integral Monte Carlo simulations all quantum and Coulomb correlation effects are treated on first…

Strongly Correlated Electrons · Physics 2012-11-30 J. Schleede , A. Filinov , M. Bonitz , H. Fehske

We construct a theory for Bose-Einstein condensation of light in nano-fabricated semiconductor microcavities. We model the semiconductor by one conduction and one valence band which consist of electrons and holes that interact via a Coulomb…

Quantum Gases · Physics 2016-07-27 A. -W. de Leeuw , E. C. I. van der Wurff , R. A. Duine , D. van Oosten , H. T. C. Stoof

Solution-processed light-emitting diodes (LEDs) are appealing for their potential in the low-cost fabrication of large-area devices. However, the limited performance of solution-processed blue LEDs, particularly their short operation…

Generation of energetic (hot) electrons is an intrinsic property of any plasmonic nanostructure under illumination. Simultaneously, a striking advantage of metal nanocrystals over semiconductors lies in their very large absorption cross…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Lucas V. Besteiro , Xiang-Tian Kong , Zhiming Wang , Gregory V. Hartland , Alexander O. Govorov

When a semiconductor absorbs light, the resulting electron-hole superposition amounts to a uncontrolled quantum ripple that eventually degenerates into diffusion. If the conformation of these excitonic superpositions could be engineered,…

Mesoscale and Nanoscale Physics · Physics 2017-05-31 Xiaoning Zang , Simone Montangero , Lincoln D. Carr , Mark T. Lusk

In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons (i.e., bound electron-hole pairs) in CsPbBr3 perovskite nanocrystals (NCs)…

Achieving electrical injection of exciton-polaritons, half-light, half-matter quasiparticles arising from the strong coupling between photonic and excitonic resonances, is a crucial milestone to scale up polaritonic devices such as optical…

Optics · Physics 2022-09-14 Yutao Wang , Jingyi Tian , Maciej Klein , Giorgio Adamo , Son Tung Ha , Cesare Soci

An indirect exciton is a bound state of an electron and a hole in spatially separated layers. Two-dimensional indirect excitons can be created optically in heterostructures containing double quantum wells or atomically thin semiconductors.…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 Chao Xu , J. R. Leonard , C. J. Dorow , L. V. Butov , M. M. Fogler , D. E. Nikonov , I. A. Young

Efficient generation of radiation in the mid- and far- infrared relies primarily on lasers and coherent nonlinear optical phenomena driven by lasers. This wavelength range lacks of luminescent devices because the spontaneous emission rate…

Charged optical excitations (trions) generated by charge carrier injection are crucial for emerging optoelectronic technologies as they can be produced and manipulated by electric fields. Trions and neutral excitons can be efficiently…

Atomic and Molecular Clusters · Physics 2021-12-23 Jiří Doležal , Sofia Canola , Pablo Merino , Martin Švec

We show that for the very same reason that excitons are bright, i.e. coupled to photons, they have a higher energy than dark excitons, even for electrons spatially separated from holes, such as in a double quantum well. Indeed, the same…

Strongly Correlated Electrons · Physics 2008-07-30 Monique Combescot , Michael N. Leuenberger

The statistical theory of multiple exciton generation in quantum dots which is based on the Fermi approach to the problem of multiple particle in nucleon-nucleon collisions is presented. Our estimates of the multiple exciton generation…

Mesoscale and Nanoscale Physics · Physics 2011-02-07 B. L. Oksengendler , N. N. Turaeva , S. S. Rashidova

Advances in nanotechnology provide techniques for the realisation of integrated quantum-optical circuits for on-chip quantum information processing(QIP). The indistinguishable single photons, required for such devices can be generated by…

Mesoscale and Nanoscale Physics · Physics 2014-04-16 M. N. Makhonin , J. E. Dixon , R. J. Coles , B. Royall , E. Clarke , M. S. Skolnick , A. M. Fox

Colloidal Quantum Dots (CQDs), major building blocks in modern opto-electronic devices, have so far been synthesized with only one emission center where the exciton resides. Recent development of coupled Colloidal Quantum Dots Molecules…

Mesoscale and Nanoscale Physics · Physics 2022-06-22 Yossef E. Panfil , Jiabin Cui , Somnath Koley , Uri Banin

Exciton many-body interaction bear great implication for application in advanced photonic devices and quantum science and technology such as quantum computing, but the fundamental understanding about exciton many-body interaction is very…

Materials Science · Physics 2020-09-17 Yiling Yu , Guoqing Li , Linyou Cao

Resolving the momentum degree of freedom of excitons - electron-hole pairs bound by the Coulomb attraction in a photoexcited semiconductor, has remained a largely elusive goal for decades. In atomically thin semiconductors, such a…