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We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 A. V. Bragas , C. Aku-Leh , S. Costantino , Alka Ingale , J. Zhao , R. Merlin

The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of…

Using femtosecond pump-probe spectroscopy with pulse shaping techniques, one can generate and detect coherent phonons in chirality-specific semiconducting single-walled carbon nanotubes. The signals are resonantly enhanced when the pump…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 G. D. Sanders , C. J. Stanton , J. -H. Kim , K. -J. Yee , Y. -S. Lim , E. H. Haroz , L. G. Booshehri , J. Kono , R. Saito

1$T$-TaSe$_{2}$ is host to coexisting strongly-correlated phases including charge density waves (CDWs) and an unusual Mott transition at low temperature. Here, we investigate coherent phonon oscillations in 1$T$-TaSe$_{2}$ using a…

Strongly Correlated Electrons · Physics 2023-10-26 C. J. Sayers , H. Hedayat , A. Ceraso , F. Museur , M. Cattelan , L. S. Hart , L. S. Farrar , S. Dal Conte , G. Cerullo , C. Dallera , E. Da Como , E. Carpene

The excitation and detection of coherent phonons has given unique insights into condensed matter, in particular for materials with strong electron-phonon coupling. We report a study of coherent phonons in the layered charge density wave…

The interaction of excitons with lattice vibrations underlies the scattering from bright to dark excitons as well as the coherent modulation of the exciton energy. Unlike the former mechanism, which involves phonons with finite momentum,…

Mesoscale and Nanoscale Physics · Physics 2024-06-24 Enrico Perfetto , Kai Wu , Gianluca Stefanucci

We demonstrate the generation of coherent phonons in a quartz Bulk Acoustic Wave (BAW) resonator through the photoelastic properties of the crystal, via the coupling to a microwave cavity enhanced by a photonic lambda scheme. This is…

Density Functional Theory (DFT) calculations not only allow to predict the vibrational and optical properties of solids but also to understand and disentangle the mechanisms playing a key role in the generation of coherent optical phonons.…

Materials Science · Physics 2025-10-09 A. Levchuk , R. Busselez , G. Vaudel , P. Ruello , V. Juvé , B. Arnaud

The near-field interaction due to a strong electromagnetic field induced by resonant localized plasmons can result in a strong coupling of excitonic states or formation of hybrid exciton-plasmon modes in quantum confined structures. This…

Mesoscale and Nanoscale Physics · Physics 2019-04-01 Yuba Poudel , Gary N. Lim , Mojtaba Moazzezi , Zachariah Hennighausen , Yuri Rostovtsev , Francis DSouza , Swastik Kar , Arup Neogi

We report two new first-order Raman modes in the spectra of few-layer MoS$_2$ at 286~cm$^{-1}$ and 471~cm$^{-1}$ for excitation energies above 2.4~eV. These modes appear only in few-layer MoS$_2$; therefore their absence provides an easy…

Materials Science · Physics 2015-06-17 Nils Scheuschner , Roland Gillen , Matthias Staiger , Janina Maultzsch

Single-layer transition metal dichalcogenides are at the center of an ever increasing research effort both in terms of fundamental physics and applications. Exciton-phonon coupling plays a key role in determining the (opto)electronic…

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

The topologically nontrivial and chemically functional distorted octahedral (T') transition metal dichalcogenides (TMDCs) are a type of layered semimetal that has attracted significant recent attention. However, the properties of monolayer…

Materials Science · Physics 2016-12-14 Shao-Yu Chen , Carl H. Naylor , Thomas Goldstein , A. T. Charlie Johnson , Jun Yan

We present a novel and simple picture of the generation dynamics of coherent longitudinal optical (LO) phonons and LO-phonon-plasmon-coupled (LOPC) modes by the ultrafast infrared pump-pulses in gallium arsenide (GaAs) employing the…

Materials Science · Physics 2024-05-14 Itsuki Takagi , Yuma Konno , Yosuke Kayanuma , Kazutaka G. Nakamura

We report an observation of coherent phonons of $E_g^1$, $E_u^1$, $A_{1g}^1$, and $E_g^2$ symmetry generated in a single-crystal film of $Bi_2Se_3$ by an intense single-cycle THz pulse. The atomic vibrations reveal themselves through…

Coherent phonons, light-induced coherent lattice vibrations in solids, provide a powerful route to engineer structural and electronic degrees of freedom using light. In this manuscript, we formulate an ab initio theory of the displacive…

Materials Science · Physics 2024-07-25 C. Emeis , S. Jauernik , S. Dahiya , Y. Pan , C. E. Jensen , P. Hein , M. Bauer , F. Caruso

Multi-gigahertz mechanical vibrations stemming from interactions between light fields and matter, also known as acoustic phonons, have long been a subject of study. In recent years, specially designed functional devices have been developed…

Optics · Physics 2021-04-14 Mamoru Endo , Shota Kimura , Shuntaro Tani , Yohei Kobayashi

Time-resolved spectroscopies using intense THz pulses appear as a promising tool to address collective electronic excitations in condensed matter. In particular recent experiments showed the possibility to selectively excite collective…

Strongly Correlated Electrons · Physics 2019-11-18 Mattia Udina , Tommaso Cea , Lara Benfatto

Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…

Mesoscale and Nanoscale Physics · Physics 2021-11-29 Ziqi Li , Bo Peng , Miao-Ling Lin , Yu-Chen Leng , Bin Zhang , Chi Pang , Ping-Heng Tan , Bartomeu Monserrat , Feng Chen

We have investigated the dynamical properties of coherent phonons generated in antimony under high density photo excitation. Precise measurements and extended analysis of coherent phonon oscillations provide new insights into the process of…

Materials Science · Physics 2016-03-02 H. Kumagai , I. Matsubara , J. Nakahara , T. Mishina
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