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Graphene as a zero-bandgap two-dimensional semiconductor with a linear electron band dispersion near the Dirac points has the potential to exhibit very interesting nonlinear optical properties. In particular, third harmonic generation of…

Applied Physics · Physics 2018-01-31 Parvin Navaeipour , Ibraheem Al-Naib , Marc M. Dignam

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

Optics · Physics 2022-03-03 Davis M. Welakuh , Prineha Narang

High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…

A key concept underlying the specific functionalities of metasurfaces, i.e. arrays of subwavelength nanoparticles, is the use of constituent components to shape the wavefront of the light, on-demand. Metasurfaces are versatile and novel…

The discovery of topological phases has introduced a new dimension to materials science. Three-dimensional (3D) topological insulators (TIs) are a remarkable class of matter that is insulating in the bulk while hosting conductive…

Breaking inversion symmetry in solids plays a central role in nonlinear optics because it can change material properties, such as producing even-order nonlinear optical (NLO) effects. Although a centrosymmetric diamond has been developed as…

Optics · Physics 2022-03-21 Aizitiaili Abulikemu , Yuta Kainuma , Toshu An , Muneaki Hase

Plasmonic enhancement of nonlinear optical processes confront severe limitations arising from the strong dispersion of metal susceptibilities and small interaction volumes that hamper desirable phase-matching-like conditions. Maximizing…

We demonstrate a nonlinear metamaterial which enhance higher order harmonics in microwave frequency regime. Nonlinearity in the structure is introduced by adding a varactor diode in the common slit of the double split ring resonator (DSRR)…

Applied Physics · Physics 2017-05-23 Sinhara R Silva , Khagendra Battarai , Alexander Shields , Jiangfeng Zhou

Metasurfaces consisting of hybrid metal/dielectric nanostructures carry advantages of both material platforms. The hybrid structures can not only tightly confine subwavelength electromagnetic fields but also lower the absorption losses.…

Optics · Physics 2022-11-23 Ajith P Ravishankar , Felix Vennberg , Anand Srinivasan

High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…

We explore the outcomes of detailed microscopic models by calculating second- and third-harmonic generation from thin film surfaces with discontinuous free-electron densities. These circumstances can occur in structures consisting of a…

Nanophotonics research has focused recently on the ability of non-linear optical processes to mediate and transform optical signals in a myriad of novel devices, including optical modulators, transducers, color filters, photodetectors,…

We report the observation of second harmonic generation with high conversion efficiency $\sim 0.005\%$ in the terahertz regime from thin films of the topological insulator Bi$_2$Se$_3$ that exhibit the linear photogalvanic effect, measured…

Strongly Correlated Electrons · Physics 2024-06-11 Jonathan Stensberg , Xingyue Han , Zhuoliang Ni , Xiong Yao , Xiaoyu Yuan , Debarghya Mallick , Akshat Gandhi , Seongshik Oh , Liang Wu

There is an active demand to develop efficient nanoscale nonlinear sources for applications in photonic circuitry, quantum optics and biosensing. To this end, plasmonic systems have been utilized to boost the nonlinear signal generation,…

Optics · Physics 2019-06-26 Feng Wang , Manoj Manjare , Robert Lemasters , Chentao Li , Hayk Harutyunyan

We theoretically investigate the resonance of third harmonic generation (THG) that has been observed at frequency being half of the superconducting gap in a multiband disordered superconductor NbN. The central question is whether the…

Superconductivity · Physics 2020-10-09 Naoto Tsuji , Yusuke Nomura

Metasurfaces have long served as a cornerstone technique to enhance nonlinear processes, enabling frequency conversion, efficient light manipulation and integrated photonic devices. However, traditional bulk materials often suffer from high…

We study polarization independent improved light trapping in commercial thin film hydrogenated amorphous silicon (a-Si:H) solar photovoltaic cells using a three-dimensional silver array of multi-resonant nano-disk structures embedded in a…

We demonstrate phase-matched second-harmonic generation (SHG) from three-dimensional metamaterials consisting of stacked metasurfaces. To achieve phase matching, we utilize a novel mechanism based on phase engineering of the metasurfaces at…

We demonstrate a simple and scalable approach to increase conversion efficiencies of nonlinear metasurfaces by incorporating them into multipass cells and by letting the pump beam to interact with the metasurfaces multiple times. We…

Tailoring optical nonlinear effects (e.g. harmonic generation, sum-frequency mixing, etc.) in the recently emerging all-dielectric platform is important for both the fundamental science and industrial development of high-efficiency,…

Optics · Physics 2022-06-02 Shuyuan Xiao , Meibao Qin , Junyi Duan , Feng Wu , Tingting Liu