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Eu(TTA)3 complexes are used as an emission source in the presence of high refractive index dielectric nanostructures. These nanostructures support Mie-type resonances that modify the local density of optical states. Specifically, the…

Whispering-gallery-mode microcavities are known to have high optical quality factor, making them suitable for nonlinear optical interactions. Here, third-harmonic generation is observed using a relatively small radius wedge silicon oxide…

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

We study third-harmonic generation (THG) in an excitonic insulator (EI) described in a two-band correlated electron model. Employing the perturbative expansion with respect to the external electric field, we derive the THG susceptibility…

Strongly Correlated Electrons · Physics 2021-12-28 Tetsuhiro Tanabe , Tatsuya Kaneko , Yukinori Ohta

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

Aluminum nitride and silicon nitride have recently emerged as important nonlinear optical materials in integrated photonics respectively for their quadratic and cubic optical nonlinearity. A composite aluminum nitride and silicon nitride…

Optics · Physics 2017-12-04 Joshua B. Surya , Xiang Guo , Chang-Ling Zou , Hong X. Tang

A one-dimensional photonic-crystal (PC) cavity with nanoholes is proposed for extremely enhancing the THz electric fields by utilizing the electromagnetic (EM) boundary conditions, where both slot effect (for the perpendicular component of…

Optics · Physics 2018-12-05 Qijing Lu , Xiaogang Chen , Chang-Ling Zou , Shusen Xie

Localized electromagnetic modes and negligible Ohmic losses dictate the growing interest in subwavelength all-dielectric nanoparticles. Although an exhaustive volume of study dealt with interaction of all-dielectric nanostructures with…

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component…

The search for miniaturized components for nonlinear optical processes needs a way to overcome the efficiency loss due to the effective size reduction of the active medium. We investigate here a combination of a nanosized nonlinear…

The generation of the localized surface plasmon resonance (LSPR) on the surface of plasmonic structures in the nanoscale has paved the way for advanced biosensing, surpassing the conventional detection limits. The electric field enhancement…

Optics · Physics 2023-12-12 Siddhartha Banerjee , Jolly Xavier

Strong second harmonic generation (SHG) in silicon nitride has been extensively studied-among others, in terms of laser-induced SHG enhancement in Si3N4 waveguides. This enhancement has been ascribed to the all-optical poling induced by the…

Immense optical field enhancement was predicted to occur for the Berreman mode in ultrathin films at frequencies in the vicinity of epsilon near zero (ENZ). Here, we report the first experimental proof of this prediction in the mid-infrared…

High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

Dielectric capacitors are widely used in pulsed power electronic devices due to their ultrahigh power densities and extremely fast charge/discharge speed. To achieve enhanced energy storage density, both maximum polarization (Pmax) and…

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì
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