Related papers: Prospects for laser cooling of polyatomic molecule…
Optical Bloch equations and rate equations serve as powerful tools to model light-matter interactions from textbook-like two-level atoms to the complex internal dynamics of molecules. A particular challenge in this context is posed by…
Molecular ions can be held in a chain of laser-cooled atomic ions by sympathetic cooling. This system is ideal for performing high-precision molecular spectroscopy with applications in astrochemistry and fundamental physics. Here we show…
Beam cooling enables an increase of peak and average luminosities and significantly expands the discovery potential of colliders; therefore, it is an indispensable component of any modern design. Optical Stochastic Cooling (OSC) is a…
Cooling and Entanglement in optomechanical systems coupled through radiation pressure and photothermal force is studied. To develop the photothermal model, we derive an expression for deformation constant of the force. Exploiting linearized…
Studying optical properties of organic materials is important due to the rapid development of organic light-emitting diodes, solar cells, and photon detectors. Here for the first time we have performed tight-binding calculations for singlet…
The translational motion of molecular ions can be effectively cooled sympathetically to temperatures below 100 mK in ion traps through Coulomb interactions with laser-cooled atomic ions. The distribution of internal rovibrational states,…
The coexistence and competition of superconductivity and magnetism can lead to a variety of rich physics and technological applications. Recent discovery of atomic-layer superconductors and self-assembly of magnetic molecules on solid…
Laser cooling on weak transitions is a useful technique for reaching ultracold temperatures in atoms with multiple valence electrons. However, for strongly magnetic atoms a conventional narrow-line magneto-optical trap (MOT) is destabilized…
Laser cycling of resonances can remove entropy from a system via spontaneously emitted photons, with electronic resonances providing the fastest cooling timescales because of their rapid relaxation rates. Although atoms are routinely laser…
We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasi-closed cycling transition is established to scatter $\sim 10^3$ photons per molecule, predominantly limited by interaction time. This…
We propose a general method to cool the translational motion of molecules. Our method is an extension of single photon atomic cooling which was successfully implemented in our laboratory. Requiring a single event of absorption followed by a…
We propose a scheme to directly laser cool Rydberg atoms by laser cooling the residual ion core within the Rydberg-electron orbit. The scheme is detailed for alkaline-earth-metal Rydberg atoms, whose ions can be easily laser cooled. We…
Since the advent of atom laser-cooling, trapping or cooling natural molecules has been a long standing and challenging goal. Here, we demonstrate a method for laser-trapping molecules that is radically novel in its configuration, in its…
Laser cooling of translational motion of small molecules is performed by addressing transitions that ensure spontaneous emission cannot cause net rotational excitation. This will not be possible once the rotational splitting becomes…
We propose to repeatedly load laser-cooled molecules into optical tweezers, and transfer them to storage states that are rotationally excited by two additional quanta. Collisional loss of molecules in these storage states is suppressed, and…
We present a high-resolution laser spectroscopic study of the $\tilde{A}\,^2B_2- \tilde{X}\,^2A_1$ and $\tilde{B}\,^2B_1- \tilde{X}\,^2A_1$ transitions of calcium (I) phenoxide, CaOPh (CaOC$_6$H$_5$). The rotationally resolved band systems…
Particle accelerators and storage rings have been transformative instruments of discovery, and, for many applications, innovations in particle-beam cooling have been a principal driver of that success1. Beam cooling reduces the spread in…
We explore the feasibility of optically forming long-range tetratomic and larger polyatomic molecules in their ground electronic state from ultracold pairs of polar molecules aligned by external fields. Depending on the relative orientation…
We proposed a general Zeeman slower scheme applicable to the majority of the laser-coolable molecules. Different from previous schemes, the key idea of our scheme lies in that the compensation of the detuning with the magnetic field is done…
The LiFr diatomic represents a promising candidate for indirect laser cooling that has not yet been investigated not theoretically or experimentally. The potential energy curves of the ground and low_lying excited states of the LiFr…