English
Related papers

Related papers: Prospects for laser cooling of polyatomic molecule…

200 papers

In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…

Quantum Physics · Physics 2007-05-23 Christiane P. Koch , José P. Palao , Ronnie Kosloff , Françoise Masnou-Seeuws

A study of the intensity-borrowing mechanisms important to optical cycling transitions in laser-coolable polyatomic molecules arising from non-adiabatic coupling, contributions beyond the Franck-Condon approximation, and Fermi resonances is…

Chemical Physics · Physics 2023-07-19 Chaoqun Zhang , Nicholas R. Hutzler , Lan Cheng

We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…

Atomic Physics · Physics 2017-09-13 Chien-Yu Lien , Scott R. Williams , Brian Odom

We investigated the optical cycling effect of the $\mathrm{X}^2\Sigma(v=0,\ N=1^-) - \mathrm{A}^2\Pi_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in…

Atomic and Molecular Clusters · Physics 2025-07-08 Kikyeong Kwon , Seunghwan Roh , Youngju Cho , Yongwoong Lee , Eunmi Chae

Polyatomic molecules provide complex internal structures that are ideal for applications in quantum information science, quantum simulation, and precision searches for physics beyond the Standard Model. A key feature of polyatomic molecules…

Alkaline earth monoalkoxide free radicals (MORs) have molecular properties conducive to direct laser cooling to sub-millikelvin temperatures. Using dispersed laser induced fluorescence (DLIF) measurements from a pulsed supersonic molecular…

Atomic Physics · Physics 2019-05-22 Ivan Kozyryev , Timothy C. Steimle , Phelan Yu , Duc-Trung Nguyen , John M. Doyle

Laser cooling of large, complex molecules is a long-standing goal, instrumental for enabling new quantum technology and precision measurements. A primary consideration for the feasibility of laser cooling, which determines the efficiency…

Optomechanical crystals (OMCs) enable coherent interactions between optical photons and microwave acoustic phonons, and represent a platform for implementing quantum transduction between microwave and optical signals. Optical…

Aluminum monochloride (AlCl) has been proposed as an excellent candidate for laser cooling. Here we present absorption spectroscopy measurements on the $A^1\Pi \leftarrow X^1\Sigma^+$ transition in AlCl inside a cryogenic helium buffer-gas…

Atomic Physics · Physics 2021-07-14 J. R. Daniel , C. Wang , K. Rodriguez , T. Lewis , A. Teplukhin , B. Kendrick , C. Bardeen , B. Hemmerling

The paper considers methods of particle cooling mostly concentrating on cooling of high energy heavy particles in the high energy colliders. Presently, there are two major methods of the cooling the electron cooling and stochastic cooling.…

Accelerator Physics · Physics 2024-01-30 Valeri Lebedev

We propose a scheme for direct laser deceleration of molecules based on a vibrational transition-mediated bichromatic force (VBCF). By precisely engineering mid-infrared optical fields, we establish coherent absorption-stimulated emission…

Atomic Physics · Physics 2026-05-20 Meng-Yi Yu , Ya-Nan Lv , Cun-Feng Cheng , Shui-Ming Hu

Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the…

Atomic Physics · Physics 2015-06-18 A. M. Jayich , A. C. Vutha , M. T. Hummon , J. V. Porto , W. C. Campbell

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…

Atomic Physics · Physics 2017-07-27 F. Lindenfelser , M. Marinelli , V. Negnevitsky , S. Ragg , J. P. Home

We propose an alternative method to laser cooling. Our approach utilizes the extreme brightness of a supersonic atomic beam, and the adiabatic atomic coilgun to slow atoms in the beam or to bring them to rest. We show how internal-state…

We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires single-frequency vacuum-ultraviolet light, while multielectron atoms…

Atomic Physics · Physics 2015-06-26 D. Kielpinski

We theoretically investigate the laser cooling of fermionic barium monofluoride (137BaF) molecules, which are promising candidates for precision studies of weak parity violation and nuclear anapole moments. This molecular species features…

Atomic Physics · Physics 2022-06-07 Felix Kogel , Marian Rockenhäuser , Ralf Albrecht , Tim Langen

Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these…

Degenerate optomechanical parametric oscillators are optical resonators in which a mechanical degree of freedom is coupled to a cavity mode that is nonlinearly amplified via parametric down-conversion of an external pumping laser. Below a…

Heteronuclear alkali-metal dimers represent the class of molecules of choice for creating samples of ultracold molecules exhibiting an intrinsic large permanent electric dipole moment. Among them, the KCs molecule, with a permanent dipole…

Atomic Physics · Physics 2015-04-08 D. Borsalino , R. Vexiau , M. Aymar , E. Luc-Koenig , O. Dulieu , N. Bouloufa-Maafa

Optomechanical systems show tremendous promise for high sensitivity sensing of forces and modification of mechanical properties via light. For example, similar to neutral atoms and trapped ions, laser cooling of mechanical motion by…

Quantum Physics · Physics 2017-06-07 Xunnong Xu , Thomas Purdy , Jacob M. Taylor