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We report the results of a large-scale modelling study of radiation damage effects in the nuclear waste form zirconolite. We particularly focus on the effects of radiation damage in amorphous zirconolite and have developed a new way to…

Materials Science · Physics 2021-02-03 Aaron Diver , Oliver Dicks , Alin Elena , Ilian Todorov , Kostya Trachenko

The molecular structures of amorphous silica and crystalline quartz are used to predict their intrinsic strength and fracture toughness together with the theoretical strength of silicon dioxide. At the atomic scale, the amorphous silica is…

Materials Science · Physics 2024-10-15 Xiaozhi Hu

Using molecular dynamics simulations, with a realistic many-body embedded-atom potential, and a novel method to characterize local order, we study the structure of pure nickel during the rapid quench of the liquid and in the resulting…

Disordered Systems and Neural Networks · Physics 2016-08-15 Oscar Rodríguez de la Fuente , José M. Soler

The controlled generation and manipulation of atom-like defects in solids has a wide range of applications in quantum technology. Although various defect centres have displayed promise as either quantum sensors, single photon emitters or…

Mechanical shear deformations lead, in some cases, to effects similar to those resulting from ion irradiation. Here we characterize the effects of shear velocity and temperature on amorphous silicon (\aSi) modelled using classical molecular…

Materials Science · Physics 2015-05-19 Ali Kerrache , Normand Mousseau , Laurent J. Lewis

We report the density-functional calculations that systematically clarify the stable forms of carbon-related defects and their energy levels in amorphous SiO$_2$ using the melt-quench technique in molecular dynamics. Considering the…

Materials Science · Physics 2018-12-03 Yu-ichiro Matsushita , Atsushi Oshiyama

Identification of microscopic configuration of point defects acting as quantum bits is a key step in the advance of quantum information processing and sensing. Among the numerous candidates, silicon vacancy related centers in silicon…

Materials Science · Physics 2017-11-01 Viktor Ivády , Joel Davidsson , Nguyen Tien Son , Takeshi Ohshima , Igor A. Abrikosov , Adam Gali

The buckled structure of silicene leads to the possibility of new kinds of line defects that separate regions with reversed buckled phases. In the present work we show that these new grain boundaries have very low formation energies, one…

Materials Science · Physics 2013-12-13 Matheus P. Lima , A. Fazzio , Antonio J. R. da Silva

Silicon has long been synonymous with semiconductor technology. This unique role is due largely to the remarkable properties of the Si-SiO_2 interface, especially the (001)-oriented interface used in most devices. Although Si is crystalline…

Materials Science · Physics 2009-10-31 Yuhai Tu , J. Tersoff

We study the dynamic electrical response of a silicon-molecular monolayer-metal junctions and we observe two contributions in the admittance spectroscopy data. These contributions are related to dipolar relaxation and molecular organization…

Mesoscale and Nanoscale Physics · Physics 2010-07-27 Nicolas Clement , Stephane Pleutin , David Guerin , Dominique Vuillaume

Graphene, being one-atom thick, is extremely sensitive to the presence of adsorbed atoms and molecules and, more generally, to defects such as vacancies, holes and/or substitutional dopants. This property, apart from being directly usable…

Materials Science · Physics 2011-04-08 Rocco Martinazzo , Simone Casolo , Gian Franco Tantardini

In this paper we discuss the application of current it ab initio computer simulation techniques to hydrogenated amorphous silicon (a-Si:H). We begin by discussing thermal fluctuation in the number of coordination defects in the material,…

Materials Science · Physics 2009-11-13 D. A. Drabold , T. A. Abtew , F. Inam , Y. Pan

Use of amorphous silicon ($a$-Si) and hydrogenated amorphous silicon ($a$-Si:H) in photovoltaics has been limited by light-induced degradation (the Staebler-Wronski effect) and low hole mobilities, and voids have been implicated in both…

Materials Science · Physics 2020-02-19 Enrique Guerrero , David A. Strubbe

A free-energy functional that contains both the symmetry conserved and symmetry broken parts of the direct pair correlation function has been used to investigate the freezing of a system of hard spheres into crystalline and amorphous…

Soft Condensed Matter · Physics 2015-05-27 Swarn Lata Singh , Atul S. Bharadwaj , Yashwant Singh

The atomic structure of amorphous materials is believed to be well described by the continuous random network model. We present an algorithm for the generation of large, high-quality continuous random networks. The algorithm is a variation…

Materials Science · Physics 2007-05-23 R. L. C. Vink , G. T. Barkema , M. A. Stijnman , R. H. Bisseling

Multi-crystalline silicon is widely used for producing low-cost and high-efficiency solar cells. During crystal growth and device fabrication, silicon solar cells contain grain boundaries (GBs) which are preferential segregation sites for…

Materials Science · Physics 2020-11-24 Rita Maji , Eleonora Luppi , Nathalie Capron , Elena Degoli

We have investigated the response of amorphous silicon (a-Si), in particular crystallization, to external mechanical shear deformations using classical molecular dynamics (MD) simulations and the empirical Environment Dependent Inter-atomic…

Materials Science · Physics 2015-05-28 Ali Kerrache , Normand Mousseau , Laurent J. Lewis

The simulations of field-evaporation processes for silicon atoms on various Si(001) surfaces are implemented using the first-principles calculations based on the real-space finite-difference method. We find that the atoms which locate on…

Condensed Matter · Physics 2009-11-10 Tomoya Ono , Kikuji Hirose

Networks of silicon nanowires possess intriguing electronic properties surpassing the predictions based on quantum confinement of individual nanowires. Employing large-scale atomistic pseudopotential computations, as yet unexplored branched…

Mesoscale and Nanoscale Physics · Physics 2013-11-18 Ümit Keleş , Bartosz Liedke , Karl-Heinz Heinig , Ceyhun Bulutay

We present linear ensembles of dangling bond chains on a hydrogen terminated Si(100) surface, patterned in the closest spaced arrangement allowed by the surface lattice. Local density of states maps over a range of voltages extending…

Mesoscale and Nanoscale Physics · Physics 2016-07-21 John A. Wood , Mohammad Rashidi , Mohammad Koleini , Jason L. Pitters , Robert A. Wolkow
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