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We discuss the discovery by variational Monte Carlo (VMC) methods of a series of multinode quantum spin liquids (QSLs) in extended Kitaev models on the honeycomb lattice. Like the gapless Kitaev spin liquid with its two nodes at K and…

Strongly Correlated Electrons · Physics 2024-12-03 Jiucai Wang , B. Normand , Zheng-Xin Liu

Recently it was realized that the zigzag magnetic order in Kitaev materials can be stabilized by small negative off-diagonal interactions called the $\Gamma'$ terms. To fully understand the effect of the $\Gamma'$ interactions, we…

Strongly Correlated Electrons · Physics 2020-10-21 Jiucai Wang , Qirong Zhao , Xiaoqun Wang , Zheng-Xin Liu

The S=3/2 Kitaev honeycomb model (KHM) is a quantum spin liquid (QSL) state coupled to a static Z$_2$ gauge field. Employing an SO(6) Majorana representation of spin 3/2's, we find an exact representation of the conserved plaquette fluxes…

Strongly Correlated Electrons · Physics 2022-07-07 Hui-Ke Jin , W. M. H. Natori , F. Pollmann , J. Knolle

In addition to the Kitaev ($K$) interaction, candidate Kitaev materials also possess Heisenberg ($J$) and off-diagonal symmetric ($\Gamma$) couplings. We investigate the quantum ($S = 1/2$) $K$-$J$-$\Gamma$ model on the honeycomb lattice by…

Strongly Correlated Electrons · Physics 2019-11-14 Jiucai Wang , B. Normand , Zheng-Xin Liu

A family of spin-orbit coupled honeycomb Mott insulators offers a playground to search for quantum spin liquids (QSLs) via bond-dependent interactions. In candidate materials, a symmetric off-diagonal $\Gamma$ term, close cousin of Kitaev…

Strongly Correlated Electrons · Physics 2021-06-07 Qiang Luo , Jize Zhao , Hae-Young Kee , Xiaoqun Wang

Topological states of matter such as quantum spin liquids (QSLs) are of great interest because of their remarkable predicted properties including protection of quantum information and the emergence of Majorana fermions. Such QSLs, however,…

Motivated by the recent synthesis of two insulating Li$_2$IrO$_3$ polymorphs, where Ir$^{4+}$ $S_{eff}$=1/2 moments form 3D ("harmonic") honeycomb structures with threefold coordination, we study magnetic Hamiltonians on the resulting…

Strongly Correlated Electrons · Physics 2014-11-26 Itamar Kimchi , James G. Analytis , Ashvin Vishwanath

Anderson proposed structural topology in frustrated magnets hosting novel quantum spin liquids (QSLs). The QSL state is indeed exactly derived by fractionalizing the spin excitation into spinless Majorana fermions in a perfect two…

We propose a theoretical model for a gapless spin liquid phase that may have been observed in a recent experiment on $\mathrm{H_3Li Ir_2 O_6}$. Despite the insulating and non-magnetic nature of the material, the specific heat coefficient…

Strongly Correlated Electrons · Physics 2018-03-29 Kevin Slagle , Wonjune Choi , Li Ern Chern , Yong Baek Kim

The possible existence of a quantum spin liquid (QSL) phase, an exotic state of matter with long-range quantum entanglement and fractionalized excitations, in $\alpha$-RuCl$_3$ has sparked widespread interests in exploring QSLs in various…

Strongly Correlated Electrons · Physics 2023-04-04 Shun-Yao Yu , Han Li , Qi-Rong Zhao , Yuan Gao , Xiao-Yu Dong , Zheng-Xin Liu , Wei Li , Shou-Shu Gong

A decade ago, Alexei Kitaev proposed an exactly solvable $S$ = 1/2 model on a two-dimensional honeycomb lattice, where the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the ground state. It…

Strongly Correlated Electrons · Physics 2022-01-21 Hidenori Takagi , Tomohiro Takayama , George Jackeli , Giniyat Khaliullin , Stephen E. Nagler

We use the projective symmetry group analysis to classify the quantum spin liquids on the $S=1/2$ pyrochlore magnet with a breathing anisotropy. We find 40 $\mathbb{Z}_2$ spin liquids and 16 $U(1)$ spin liquids that respect the $F\bar{4}3m$…

Strongly Correlated Electrons · Physics 2022-11-17 Li Ern Chern , Yong Baek Kim , Claudio Castelnovo

The characterization of quantum spin liquid phases in Kitaev materials has been a subject of intensive studies over the recent years, both theoretically and experimentally. Most theoretical studies have focused on an isotropically…

Strongly Correlated Electrons · Physics 2024-08-01 Matthias Gohlke , Jose Carlos Pelayo , Takafumi Suzuki

Quantum spin liquids (QSLs) represent highly entangled states of matter in which frustration-induced quantum fluctuations suppress any symmetry-breaking phase transition down to absolute zero, giving rise to fractionalized excitations and…

Quantum spin liquids (QSLs) host emergent, fractionalized fermionic excitations that are charge-neutral. Identifying clear experimental signatures of these excitations remains a central challenge in the field of strongly correlated systems,…

Strongly Correlated Electrons · Physics 2025-12-04 Penghao Zhu , Archisman Panigrahi , Leonid Levitov , Nandini Trivedi

The pursuit of quantum spin liquid (QSL) in the Kitaev honeycomb magnets has drawn intensive attention recently. In particular, $\alpha$-RuCl$_3$ has been widely recognized as a promising candidate for the Kitaev QSL. Although the compound…

Strongly Correlated Electrons · Physics 2023-03-29 Han Li , Wei Li , Gang Su

Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

The $S=3/2$ Kitaev honeycomb model (KHM) is unique among the spin-$S$ Kitaev models due to a massive ground state quasi-degeneracy that hampered previous numerical and analytical studies. In a recent work~\cite{jin2022unveiling}, we showed…

Strongly Correlated Electrons · Physics 2023-08-15 Willian M. H. Natori , Hui-Ke Jin , Johannes Knolle

We report a $^{35}$Cl nuclear magnetic resonance study in the honeycomb lattice, $\alpha$-RuCl$_3$, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct…

Strongly Correlated Electrons · Physics 2017-07-26 S. -H. Baek , S. -H. Do , K. -Y. Choi , Y. S. Kwon , A. U. B. Wolter , S. Nishimoto , Jeroen van den Brink , B. Büchner

The main question we address is how to probe the fractionalized excitations of a quantum spin liquid (QSL), for example, in the Kitaev honeycomb model. By analyzing the energy spectrum and entanglement entropy, for antiferromagnetic…

Strongly Correlated Electrons · Physics 2019-05-08 David C. Ronquillo , Adu Vengal , Nandini Trivedi
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