Related papers: Ultrasensitive Doppler Raman spectroscopy using ra…
We present a rapid-scanning approach to fluorescence-detected two-dimensional electronic spectroscopy that combines acousto-optic phase-modulation with digital lock-in detection. The approach shifts the signal detection window to suppress…
Correlated rotational alignment spectroscopy correlates observables of ultrafast gas-phase spectroscopy with high-resolution, broad-band rotational Raman spectra. This article reviews the measurement principle of CRASY, existing…
Four-wave mixing processes are ubiquitous in ultrafast optics and the determination of the coefficients of the $\chi^{(3)}$ tensor is thus essential. We introduce a novel time-resolved ultrafast spectroscopic method to characterize the…
Resonant nonlinear-optical interference processes in four-level Doppler-broadened media are studied. Specific features of amplification and optical switching of short-wavelength radiation in a strongly-absorbing resonant gas under coherent…
Time-resolved optical filtering (TROF) measures the spectrogram or sonogram by a fast photodiode followed a tunable narrowband optical filter. For periodic signal and to match the sonogram, numerical TROF algorithm is used to find the…
It is proposed a few-atom Doppler-sensitive absorption spectroscopy scheme resolving the long-standing dilemma regarding the nature of an atomic quantum translational motion (superpositional or non-superpositional) and its measurement…
Spectroscopy is a powerful tool to probe physical, chemical, and biological systems. Recent advances in microfabrication have introduced novel, intriguing mesoscopic quantum systems including superconductor-semiconductor hybrid devices and…
Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…
Ultrasensitive detection of the frequency, phase, and amplitude of radio frequency (RF) electric fields is central to a variety of important applications, including radio communication, cosmology, dark matter searches, and high-fidelity…
Band-resolved frequency modulation spectroscopy is a common method to measure weak signals of radiative ensembles. When the optical depth of the medium is large, the signal drops exponentially and the technique becomes ineffective. In this…
We describe methods using frequency combs and optical resonators for recording two-dimensional (2D) ultrafast spectroscopy signals with high sensitivity. By coupling multiple frequency combs to higher-order modes of one or more optical…
We describe a new optical diagnostic for determining the composition of gases by measuring the motion of atoms and molecules trapped within very deep optical lattices. This non-resonant method is analogous to conventional Raman scattering,…
We introduce a phase imaging mechanism for scanning transmission electron microscopy that exploits the complementary intensity changes of transmitted disks at different scattering angles. For scanning transmission electron microscopy, this…
Optical stellar interferometers have demonstrated milli-arcsecond resolution with few apertures spaced hundreds of meters apart. To obtain rich direct images, many apertures will be needed, for a better sampling of the incoming wavefront.…
Phase-sensitive optical parametric amplification of squeezed states helps to overcome detection loss and noise and thus increase the robustness of sub-shot-noise sensing. Because such techniques, e.g., imaging and spectroscopy, operate with…
We innovatively propose a method to improve the performance of Rydberg atom sensors based on the repetition frequency of pulsed lasers, which is verified in experiments. Rydberg atoms excited by pulsed lasers are influenced significantly by…
Raman scattering underlies a broad range of spectroscopic and light-generation techniques, yet its conventional description, based on the Raman gain spectrum, accurately describes only long-pulse, steady-state dynamics. We present a…
We show that the modulation of the phases of the laser beams of ultra-short pulses leads to modulation of the two photon fluorescence intensity. The phase modulation technique when used in multi-photon microscopy can improve the signal to…
Spectral measurements in the infrared (IR) optical range provide unique fingerprints of materials which are useful for material analysis, environmental sensing, and health diagnostics. Current IR spectroscopy techniques require the use of…
We present a new technique using a frequency comb laser and optical cavities for performing ultrafast transient absorption spectroscopy with improved sensitivity. Resonantly enhancing the probe pulses, we demonstrate a sensitivity of…