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This paper clarifies the microscopic nature of the staggered scalar order, which is specific to even number of f electrons per site. In such systems, crystalline electric field (CEF) can make a singlet ground state. As exchange interaction…

Strongly Correlated Electrons · Physics 2015-05-20 Yoshio Kuramoto , Shintaro Hoshino , Junya Otsuki

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…

Crystal and magnetic structures of the mineral centennialite CaCu$_3$(OH)$_6$Cl$_2\cdot0.6$H$_2$O are investigated by means of synchrotron x-ray diffraction and neutron diffraction measurements complemented by density functional theory…

We investigate crystal structure and magnetic properties including spin relaxation and magnetocaloric effect in NASICON type NaFe$_2$PO$_4$(SO$_4$)$_2$ sample. The Rietveld refinement of x-ray and neutron diffraction patterns show a…

Strongly Correlated Electrons · Physics 2024-03-14 Manish Kr. Singh , A. K. Bera , Ajay Kumar , S. M. Yusuf , R. S. Dhaka

Origin of the non-magnetic phase transition in PrTi$_2$Al$_{20}$, reported earlier in the macroscopic study, has been asserted microscopically using elastic and inelastic neutron scattering techniques. It has been shown spectroscopically…

Strongly Correlated Electrons · Physics 2013-05-03 Taku J Sato , Soshi Ibuka , Yusuke Nambu , Teruo Yamazaki , Akito Sakai , Satoru Nakatsuji

Sr2IrO4 hosts a novel Jeff =1/2 Mott state and quasi-two-dimensional antiferromagnetic order, providing a unique avenue of exploring emergent states of matter and functions that are extraordinarily sensitive to any structural variations.…

Strongly Correlated Electrons · Physics 2023-09-19 H. W. Wang , L. Y. Zhang , N. Hu , B. You , Y. T. Chang , S. L. Yuan , C. L. Lu , J. M. Liu

In a cubic environment, the ground state of spin-orbit coupled $5d^2$ ions is a non-Kramers $E_g$ doublet, which hosts quadrupole and octupole moments. A series of $5d^2$ osmium double perovskites Ba$_2M$OsO$_6$ (M = Mg, Ca, Zn, Cd) have…

Strongly Correlated Electrons · Physics 2023-08-14 Ahmed Rayyan , Xiaoyu Liu , Hae-Young Kee

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

Strongly Correlated Electrons · Physics 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

FeVO$_4$ has been studied by heat capacity, magnetic susceptibility, electric polarization and single crystal neutron diffraction experiments. The triclinic crystal structure is made of \emph{S}-shaped clusters of six Fe$^{3+}$ ions, linked…

Superconductivity · Physics 2015-05-13 A. Daoud-Aladine , B. Kundys , C. Martin , P. G. Radaelli , P. J. Brown , C. Simon , L. C. Chapon

We have succeeded in growing single crystals of SmPt2Si2 and have performed electrical resistivity, magnetization and specific heat measurements. The magnetic susceptibility shows that SmPt2Si2 is an Ising magnet with the…

Strongly Correlated Electrons · Physics 2015-06-23 Kengo Fushiya , Tatsuma D. Matsuda , Ryuji Higashinaka , Kazuhiro Akiyama , Yuji Aoki

The clathrate compound Ce3Pd20Si6 is a heavy-fermion metal that exhibits magnetically hidden order at low temperatures. Reputedly, this exotic type of magnetic ground state, known as "phase II", could be associated with the ordering of Ce…

Strongly Correlated Electrons · Physics 2016-12-28 P. Y. Portnichenko , S. Paschen , A. Prokofiev , M. Vojta , A. S. Cameron , J. -M. Mignot , A. Ivanov , D. S. Inosov

We develop a comprehensive theory for magnetoelectricity in magnetically ordered quasi-2D systems whereby in thermal equilibrium an electric field can induce a magnetization $m$ and a magnetic field can induce a polarization. This effect…

Mesoscale and Nanoscale Physics · Physics 2020-10-16 R. Winkler , U. Zülicke

Different configurations of magnetic orders and cation distributions for NiFe2O4 are studied by the density functional based methods with the possible inclusion of the on-site Coulomb interaction U. The lowest energy state is an inverse…

Materials Science · Physics 2011-05-10 Ching Cheng

We investigate the phase diagram of TmB4, an Ising magnet on a frustrated Shastry-Sutherland lattice by neutron diffraction and magnetization experiments. At low temperature we find Neel order at low field, ferrimagnetic order at high field…

Strongly Correlated Electrons · Physics 2009-11-13 K. Siemensmeyer , E. Wulf , H. -J. Mikeska , K. Flachbart , S. Gabani , S. Matas , P. Priputen , A. Efdokimova , N. Shitsevalova

We investigated the magnetic phase diagram of single crystals of SrNdFeO$_{4}$ by measuring the magnetic properties, the specific heat and the dielectric permittivity. The system has two magnetically active ions, Fe$^{3+}$ and Nd$^{3+}$.…

Materials Science · Physics 2015-06-05 J. M. Hwang , E. S. Choi , H. D. Zhou , Y. Xin , J. Lu , P. Schlottmann

We present here a detailed investigation into the magnetic ordering of full Heusler alloy Ga$_2$MnCo using dc, ac magnetization measurements, neutron diffraction and neutron depolarization experiments. Crystal structure at room temperature…

Strongly Correlated Electrons · Physics 2018-05-21 Tamalika Samanta , P. A. Bhobe , A. Das , A. Kumar , A. K. Nigam

The low-temperature antiferromagnetic state of the Sm-ions in both nonsuperconducting SmFeAsO and superconducting SmFeAsO$_{0.9}$F$_{0.1}$ single crystals was studied by magnetic torque, magnetization, and magnetoresistance measurements in…

The tetragonal heavy fermion compound CeRh2As2 has intriguing low temperature symmetry breaking phases whose nature is unclear. The unconventional superconducting phase is complemented by other normal state phases which presumably involve…

Strongly Correlated Electrons · Physics 2024-09-04 Burkhard Schmidt , Peter Thalmeier

Neutron diffraction and nuclear quadrupole resonance (NQR) measurements were employed to investigate magnetic order in the non-ferroelectric phase preceding the low-temperature multiferroic state in FeTe2O5Br. Refnement of the neutron…

Strongly Correlated Electrons · Physics 2013-04-10 M. Pregelj , P. Jeglič , A. Zorko , O. Zaharko , T. Apih , A. Gradišek , M. Komelj , H. Berger , D. Arčon