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Using first-principles Density Functional Theory calculations, we showed that electronic and magnetic properties of bare and Ti adatom adsorbed single-layer silicene and germanene, which are charged or exerted by a perpendicular electric…

Mesoscale and Nanoscale Physics · Physics 2013-07-12 H. Hakan Gürel , V. Ongun Özçelik , S. Ciraci

We use first principles density functional theory to calculate the electronic structure of the phenylthiolate (S-C$_6$H$_5$) self-assembled monolayer (SAM) on Cu(111) and Au(111) substrates. We find significant lateral dispersion of the SAM…

Materials Science · Physics 2009-11-10 Vasili Perebeinos , Marshall Newton

We combine small angle scattering experiments and simulations to investigate the internal structure and interactions of composite Poly(N-isopropylacrylamide)-Poly(ethylene glycol) (PNIPAM-PEG) microgels. At low temperatures the…

It is often assumed that the hydrogen atoms in the thiol groups of a benzene-1,4-dithiol dissociate when Au-benzene-1,4-dithiol-Au junctions are formed. We demonstrate, by stability and transport properties calculations, that this…

The ability to create micro/nano patterns of organic self-assembled monolayers on semiconductor surfaces is crucial for fundamental studies and applications in a number of emerging fields in nanoscience. Here, we demonstrate the patterning…

Applied Physics · Physics 2020-01-06 Tianhan Liu , Timothy Keiper , Xiaolei Wang , Guang Yang , Daniel Hallinan , Jianhua Zhao , Peng Xiong

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes (PEs) on a charged planar substrate is investigated by means of Monte Carlo (MC) simulations. We study in detail the equilibrium structure of the first few PE…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina

Theoretical calculations based on density functional theory have made significant contributions to our understanding of metal oxides, their surfaces, and the binding of molecules at these surfaces. In this paper we investigate the binding…

Materials Science · Physics 2007-05-23 Oyvind Borck , Elsebeth Schroder

Effect of microstructures and interactions on segmental dynamics in polyethylene glycol (PEG) solution in water is probed with macro-scale oscillatory rheology and micro-scale diffusion of a fluorescent probe. PEG solution fluorescence…

Soft Condensed Matter · Physics 2020-07-07 Shipra Bhatt , Debjani Bagchi

The capacity and stability of constituent electrodes determine the performance of Li-ion batteries. In this study, density functional theory is employed to explore the potential application of recently synthesized two dimensional…

Mesoscale and Nanoscale Physics · Physics 2014-09-24 Shijun Zhao , Wei Kang

A recent report [Kiguchi {\it et al.}, Phys. Rev. B {\bf 68}, 115402 (2003)] that the (111) surface of 5 MgO layers grown epitaxially on Ag(111) becomes metallic to reduce the electric dipole moment raises a question of what will happen…

Materials Science · Physics 2009-11-10 Ryotaro Arita , Yoshiaki Tanida , Shiro Entani , Manabu Kiguchi , Koichiro Saiki , Hideo Aoki

The water/electrode interface under an applied bias potential is a challenging out-of-equilibrium phenomenon, which is difficult to accurately model at the atomic scale. In this study, we employ a combined approach of Density Functional…

Materials Science · Physics 2025-03-14 Graciele M. Arvelos , Marivi Fernández-Serra , Alexandre R. Rocha , Luana S. Pedroza

Dissipation mechanisms are experimentally studied on topological insulator surfaces of Bi2Te3, where common Joule dissipation was observed to be suppressed due to topologically protected surface states. Thus, a novel type of dissipation…

Mesoscale and Nanoscale Physics · Physics 2019-10-30 Dilek Yildiz , Marcin Kisiel , Urs Gysin , Oguzhan Gürlü , Ernst Meyer

The effect of the adsorption of a polypeptide on the lateral interaction of dimyristoylphosphatidylserine molecules in different phase states on the surface of a 10\,mM KCl aqueous solution has been studied. Changes in the surface pressure…

The surface conductivity is measured by a four-probe technique for pentacene and rubrene single-crystals laminated on polarized and nearly unpolarized molecular monolayers with application of perpendicular electric fields. The polarization…

Materials Science · Physics 2009-11-10 J. Takeya , T. Nishikawa , T. Takenobu , S. Kobayashi , C. Goldmann , C. Krellner , T. Shimoda , T. Mitani , Y Iwasa , B. Batlogg

We compute the electronic structure of two-dimensional (2D) materials decorated with self-assembled organic monolayers using density functional theory. We find that 2D materials are strongly impacted by near-field electrostatic effects…

Materials Science · Physics 2021-09-22 Qunfei Zhou , Bukuru Anaclet , Trevor Steiner , Michele Kotiuga , Pierre Darancet

The catalytic performance of multimetallic electrodes is often attributed to a beneficial combination of ligand, strain, and ensemble effects. Understanding the influence of the electrochemical environment on the stability of the alloy…

Chemical Physics · Physics 2021-12-08 Stephen E. Weitzner , Ismaila Dabo

Molecular adsorption at the surface of a 2D material poses numerous questions regarding the modification to the band structure and interfacial states, which of course deserve full attention. In line with this, first-principle density…

Materials Science · Physics 2020-03-27 Tanmay Das , Sesha Vempati

The thermoelectric properties of polythiophene (PT) coupled to the Au (111) electrodes are studied based on density functional theory combined with nonequilibrium Green function formalism. Specially, the effect of Li and Cl adsorbents on…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Zahra Golsanamlou , Meysam Bagheri Tagani , Hamid Rahimpour Soleimani

Using scanning tunneling microscopy together with the first-principles density functional theory calculations we study structural properties of the Si(111)5x2-Au surface covered by Ag adatoms. The STM topography data show that a…

Mesoscale and Nanoscale Physics · Physics 2014-10-09 A. Stepniak , M. Krawiec , M. Jalochowski

We used density functional theories (DFT) to investigate the properties of Au2O and Au2O3-x (x = 00.08) to reveal their remarkable functionalities. Hybrid functional theories accurately estimate the band gap (Eg) of oxides, and the present…

Materials Science · Physics 2026-01-27 Yukio Watanabe
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