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Utilizing hot carriers is the crucial approach for solar cell to exceed the thermodynamic detailed balance limit, yet effective extraction of hot carriers in absorber materials via most commonly used semiconductor acceptors has been a…

The full control of the fundamental photophysics of nanosystems at frequencies as high as few THz is key for tunable and ultrafast nano-photonic devices and metamaterials. Here we combine geometrical and ultrafast control of the optical…

The ability to extract material parameters of perovskite from quantitative experimental analysis is essential for rational design of photovoltaic and optoelectronic applications. However, the difficulty of this analysis increases…

The ultrafast dynamics of charge carriers in solids plays a pivotal role in emerging optoelectronics, photonics, energy harvesting, and quantum technology applications. However, the investigation and direct visualization of such…

Metal halide perovskites, a class of cost-effective semiconductor materials, are of great interest for modern and upcoming display technologies that prioritize the light-emitting diodes (LEDs) with high efficiency and excellent color…

The reversible phase transition between orthorhombic and cubic phases is demonstrated in all-inorganic perovskite CsPbIBr2 grown by a dual-source vapor-deposition method. The phase transition is actuated via heating and moisture exposure.…

Applied Physics · Physics 2018-12-24 Chen Zou , Jiajiu Zheng , Cheng Chang , Arka Majumdar , Lih Y. Lin

Using cross-correlation current noise spectroscopy, we have investigated carrier dynamics in methylammonium lead triiodide solar cells. This method provides a space selectivity for devices with planar multi-layered structure, effectively…

Applied Physics · Physics 2020-07-15 Kevin Davenport , Fei Zhang , Mark Hayward , Logan Draper , Kai Zhu , Andrey Rogachev

The behavior of hot carriers in metal-halide perovskites (MHPs) present a valuable foundation for understanding the details of carrier-phonon coupling in the materials as well as the prospective development of highly efficient hot carrier…

For opto-electronic and photo-voltaic applications of perovskites, it is essential to know the optical properties and intrinsic losses of the used materials. A systematic microscopic analysis is presented for the example of methylammonium…

Materials Science · Physics 2018-10-29 Lars C. Bannow , Jörg Hader , Jerome V. Moloney , Stephan W. Koch

Organometal halide perovskites are promising solar-cell materials for next-generation photovoltaic applications. The long carrier lifetime and diffusion length of these materials make them very attractive for use in light absorbers and…

Materials Science · Physics 2016-12-21 Fan Zheng , Liang Z. Tan , Shi Liu , Andrew M. Rappe

Perovskite solar cells (PSCs) are the fastest-growing photovoltaic (PV) technology in the solar cell community and have reached an efficiency close to that of commercial silicon (Si) solar cells. The organic-inorganic halide perovskite…

Materials Science · Physics 2024-11-28 Kashimul Hossain

Metal halide perovskites are attracting tremendous interest for a variety of optoelectronic applications. The ability to tune the perovskite bandgap by tweaking the chemical compositions opens up new applications as coloured emitters and as…

Research on organic thin-film transistors tends to focus on improvements in device performance, but very little is understood about the ultimate limits of these devices, the microscopic physical mechanisms responsible for their limitations,…

Materials Science · Physics 2013-02-15 Ignacio Gutiérrez Lezama , Alberto F. Morpurgo

Quantum wells made of two-dimensional organic-inorganic hybrid perovskites (2D-PKs) offer a high degree of flexibility in tailoring optoelectronic properties through carrier confinement and functional interlayers. Compared to their 3D…

The determination of minority-carrier lifetimes and surface recombination velocities is essential for the development of semiconductor technologies such as solar cells. The recent development of two-photon time-resolved microscopy allows…

Materials Science · Physics 2016-03-28 Benoit Gaury , Paul Haney

In recent years, hybrid organic-inorganic metal halides have been at the forefront of materials research. Typically, the functional (e.g., optoelectronic) properties of hybrid halides are derived from the inorganic structural part, whereas…

Halide perovskite optoelectronic devices suffer from chemical degradation and current-voltage hysteresis induced by migration of highly mobile charged defects. Atomic scale molecular dynamics simulations can capture the motion of these…

Materials Science · Physics 2025-05-20 Viren Tyagi , Mike Pols , Geert Brocks , Shuxia Tao

Unbalanced mobility and injection of charge carriers in metal-halide perovskite light-emitting devices pose severe limitations to the efficiency and response time of the electroluminescence. Modulation of gate bias in methylammonium lead…

Applied Physics · Physics 2023-04-25 Maciej Klein , Krzysztof Blecharz , Bryan Wei Hao Cheng , Annalisa Bruno , Cesare Soci

A critical issue hindering the potential applications of semiconductor mixed-halide perovskites is the phase segregation effect, wherein localized regions enriched with one type of halide anions would be formed upon continuous…

Materials Science · Physics 2024-07-09 Xueying Ma , Yuhui Ye , Yang Xiao , Shengnan Feng , Chunfeng Zhang , Keyu Xia , Fengrui Hu , Min Xiao , Xiaoyong Wang

Organic semiconductors are indispensable for today's display technologies in form of organic light emitting diodes (OLEDs) and further optoelectronic applications. However, organic materials do not reach the same charge carrier mobility as…

Soft Condensed Matter · Physics 2023-10-12 Patrick Reiser , Manuel Konrad , Artem Fediai , Salvador Léon , Wolfgang Wenzel , Pascal Friederich
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