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Protected by the interplay of on-site Coulomb interactions and spin-orbit coupling, Sr$_2$IrO$_4$ at high pressure is a rare example of a Mott insulator with a paramagnetic ground state. Here, using optical Raman scattering, we measure both…

Strongly Correlated Electrons · Physics 2021-11-29 Xiang Li , S. E. Cooper , A. Krishnadas , A. de la Torre , R. S. Perry , F. Baumberger , D. M. Silevitch , D. Hsieh , T. F. Rosenbaum , Yejun Feng

Continuous quantum phase transitions involving all-in-all-out (AIAO) antiferromagnetic order in strongly spin-orbit-coupled 5d compounds could give rise to various exotic electronic phases and strongly-coupled quantum critical phenomena.…

Strongly Correlated Electrons · Physics 2020-07-01 Yishu Wang , T. F. Rosenbaum , D. Prabhakaran , A. T. Boothroyd , Yejun Feng

The ability to control the magnetic state provides a powerful means to tune the underlying band topology, enabling transitions between distinct electronic phases and the emergence of novel quantum phenomena. In this work, we address the…

It was shown earlier that applying a magnetic field during the growth of Sr$_2$IrO$_4$, also known as "field-alteration", induces significant changes to its structural, magnetic, and transport properties. However, the microscopic nature of…

Strongly Correlated Electrons · Physics 2024-02-01 Nicholas Pellatz , Jungho Kim , Jong-Woo Kim , Itamar Kimchi , Gang Cao , Dmitry Reznik

Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

Strongly Correlated Electrons · Physics 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

We demonstrate via a muon spin rotation experiment that the electronic ground state of the iridium spinel compound, CuIr$_2$S$_4$, is not the presumed spin-singlet state but a novel paramagnetic state, showing a quasistatic spin glass-like…

Strongly Correlated Electrons · Physics 2014-02-27 K. M. Kojima , 2 R. Kadono , M. Miyazaki , M. Hiraishi , I. Yamauchi , A. Koda , Y. Tsuchiya , H. S. Suzuki , H. Kitazawa

For magnets with a fully frustrated inter-layer interaction, we argue that the quantum phase transitions from a paramagnetic to an antiferromagnetic ground state, driven by pressure or magnetic field, are asymptotically three-dimensional,…

Strongly Correlated Electrons · Physics 2007-11-08 Oliver Rösch , Matthias Vojta

We report magnetic properties of the layered itinerant system, Sr$_{1-x}$Ca$_x$Co$_2$P$_2$ in the magnetic field up to 70 T. As for the exchange-enhanced Pauli paramagnetic metal SrCo$_2$P$_2$, the magnetization curve shows two…

Strongly Correlated Electrons · Physics 2014-07-21 Masaki Imai , Chishiro Michioka , Hiroto Ohta , Akira Matsuo , Koichi Kindo , Hiroaki Ueda , Kazuyoshi Yoshimura

We report a study of the low-temperature high-pressure phase diagram of the intermetallic compound PrCu$_2$, by means of molecular-field calculations and $^{63,65}$Cu nuclear-quadrupole-resonance (NQR) measurements under pressure. The…

Strongly Correlated Electrons · Physics 2009-11-13 A. Sacchetti , M. Weller , H. R. Ott , Y. Onuki

We investigate the effect of pressure on the electronic and magnetic states of CdV$_2$O$_4$ by using ab initio electronic structure calculations. The Coulomb correlation and spin-orbit coupling play important role in deciding the…

Strongly Correlated Electrons · Physics 2012-08-06 Sudhir K. Pandey

We study magnetic properties of CrO$_2$ within the density functional theory plus dynamical mean-field theory (DFT+DMFT) approach in the paramagnetic phase. We consider the 3-orbital (per Cr site) model, containing only $t_{2g}$ states, the…

Strongly Correlated Electrons · Physics 2024-10-15 A. A. Katanin

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

The delicate balance between spin-orbit coupling, Coulomb repulsion and crystalline electric field interactions observed in Ir-based oxides is usually manifested as exotic magnetic behavior. Here we investigate the evolution of the exchange…

Conventional Paramagnetism - a state with finite magnetic moment per ion sans long range magnetic ordering, but with lowering temperature the moment on each ion picks up a particular direction, breaking rotational symmetry, and results into…

Strongly Correlated Electrons · Physics 2019-09-10 Birender Singh , Deepu Kumar , Kaustuv Manna , A. K. Bera , G. Aslan Cansever , A. Maljuk , S. Wurmehl , B. Büchner , Pradeep Kumar

The magnetic phase diagram of Sr$_{1-x}$Ca$_x$Co$_2$P$_2$ as a function of hydrostatic pressure and temperature is investigated by means of high pressure muon spin rotation, relaxation and resonance ($\mu^+$SR). The weak pressure dependence…

SrMoO4 was studied under compression up to 25 GPa by angle-dispersive x-ray diffraction. A phase transition was observed from the scheelite-structured ambient phase to a monoclinic fergusonite phase at 12.2(9) GPa with cell parameters a =…

Materials Science · Physics 2008-02-04 Daniel Errandonea , Ravhi S. Kumar , Xinghua Ma , Chaoyang Tu

Antiferromagnets exhibit rapid spin dynamics in a net zero magnetic background which enables novel spintronic applications and interrogation of many-body quantum phenomena. The layered antiferromagnet Sr$_2$IrO$_4$ hosts an exotic spin…

The anisotropic magnetic properties of Sr$_2$IrO$_4$ are investigated, using longitudinal and torque magnetometry. The critical scaling across $T_c$ of the longitudinal magnetization is the one expected for the 2D XY universality class.…

Strongly Correlated Electrons · Physics 2016-04-20 L. Fruchter , D. Colson , V. Brouet

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered…

The layered 5d transition metal oxide Sr2IrO4 has been shown to host a novel Jeff=1/2 Mott spin orbit insulating state with antiferromagnetic ordering, leading to comparisons with the layered cuprates. Here we study the effect of…

Strongly Correlated Electrons · Physics 2015-03-20 S. Calder , G. -X. Cao , M. D. Lumsden , J. W. Kim , Z. Gai , B. C. Sales , D. Mandrus , A. D. Christianson
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