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In frustrated Ising magnets, classical spin liquids (CSLs) with macroscopic ground-state degeneracy can survive against conventional magnetic order, as exemplified by systems on triangular, kagome and pyrochlore lattices at zero field. Here…

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani

Three-dimensionally (3D) frustrated magnets generally exist in the magnetic diamond and pyrochlore lattices, in which quantum fluctuations suppress magnetic orders and generate highly entangled ground states (GS). LiYbSe2 in a previously…

Strongly Correlated Electrons · Physics 2022-06-15 Ranuri S. Dissanayaka Mudiyanselage , Haozhe Wang , Olivia Vilella , Martin Mourigal , Gabriel Kotliar , Weiwei Xie

A decade ago, Alexei Kitaev proposed an exactly solvable $S$ = 1/2 model on a two-dimensional honeycomb lattice, where the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the ground state. It…

Strongly Correlated Electrons · Physics 2022-01-21 Hidenori Takagi , Tomohiro Takayama , George Jackeli , Giniyat Khaliullin , Stephen E. Nagler

The most fascinating feature of certain two-dimensional (2D) gapless quantum spin liquid (QSL) is that their spinon excitations behave like the fermionic carriers of a paramagnetic metal. The spinon Fermi surface is then expected to produce…

Strongly Correlated Electrons · Physics 2020-09-17 N. Li , Q. Huang , X. Y. Yue , W. J. Chu , Q. Chen , E. S. Choi , X. Zhao , H. D. Zhou , X. F. Sun

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

Strongly Correlated Electrons · Physics 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

Strongly Correlated Electrons · Physics 2024-08-21 Hidekazu Tanaka

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the…

Strongly Correlated Electrons · Physics 2024-05-30 S. Suetsugu , T. Asaba , Y. Kasahara , Y. Kohsaka , K. Totsuka , B. Li , Y. Zhao , Y. Li , M. Tokunaga , Y. Matsuda

Recent experiments suggest a quantum spin liquid ground state in the material PbCuTe$_2$O$_6$, where $S=1/2$ moments are coupled by antiferromagnetic Heisenberg interactions into a three dimensional structure of corner sharing triangles…

Strongly Correlated Electrons · Physics 2021-09-15 Li Ern Chern , Yong Baek Kim

Fifty years after Anderson's resonating valence-bond proposal, the spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) remains the ultimate platform to explore highly entangled quantum spin states in proximity to magnetic order.…

We investigate the ground-state and the finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a square lattice with frustrating nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by…

Strongly Correlated Electrons · Physics 2018-10-26 Kazuki Uematsu , Hikaru Kawamura

Triangular lattice antiferromagnets are prototypes for frustrated magnetism and may potentially realize novel quantum magnetic states such as a quantum spin liquid ground state. A recent work suggests NdTa$_7$O$_{19}$ with rare-earth…

We present a neutron diffraction study of NaYbO$_2$, a candidate quantum spin liquid compound hosting a geometrically frustrated triangular lattice of magnetic Yb$^{3+}$ ions. We observe diffuse magnetic scattering that persists to at least…

The ground state of the spin$-1/2$ kagome antiferromagnet remains uncertain despite decades of active research. Here we step aside from this debated question to address the ground-state nature of a related, and potentially just as rich,…

Strongly Correlated Electrons · Physics 2019-12-11 Tristan Lugan , L. D. C Jaubert , Arnaud Ralko

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated…

Ba3IrTi2O9 crystallizes in a hexagonal structure consisting of a layered triangular arrangement of Ir4+ (Jeff=1/2). Magnetic susceptibility and heat capacity data show no magnetic ordering down to 0.35K inspite of a strong magnetic coupling…

Strongly Correlated Electrons · Physics 2012-10-29 Tusharkanti Dey , A. V. Mahajan , P. Khuntia , M. Baenitz , B. Koteswararao , F. C. Chou

Recently several triangular-lattice magnets with delafossite structure have been found to display spin-liquid behavior down to the lowest temperatures. Remarkably, applying a magnetic field destroys the spin liquid which then gives way to…

Strongly Correlated Electrons · Physics 2024-07-09 Santanu Dey , Joseph Maciejko , Matthias Vojta

The quantum antiferromagnet on the pyrochlore lattice offers an archetypal frustrated system, which potentially realizes a quantum spin liquid characterized by the absence of standard spontaneous symmetry breaking even at zero temperature,…

Strongly Correlated Electrons · Physics 2023-11-21 Rico Pohle , Youhei Yamaji , Masatoshi Imada

Recently, a number of experiments indicate the possible presence of spin liquid phases in quantum magnets with spin-1/2 and spin-1 moments sitting on triangular-lattice-based structures in Ba3CuSb2O9 and Ba3NiSb2O9 respectively. In relation…

Strongly Correlated Electrons · Physics 2013-06-04 Kyusung Hwang , Tyler Dodds , Subhro Bhattacharjee , Yong Baek Kim
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