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Polymers with active segments constitute prospective future materials and are used as a model for some biological systems such as chromatin. The directions of the active forces are typically introduced with temporal or spatial correlations…

Soft Condensed Matter · Physics 2024-11-25 Adam H. T. P. Höfler , Iurii Chubak , Christos N. Likos , Jan Smrek

We study the dynamics of a single chain polymer confined to a two dimensional cell. We introduce a kinetically constrained lattice gas model that preserves the connectivity of the chain, and we use this kinetically constrained model to…

Statistical Mechanics · Physics 2011-11-09 Armin Rahmani , Claudio Castelnovo , Jeremy Schmit , Claudio Chamon

We consider a model of an extensible semiflexible filament moving in two dimensions on a motility assay of motor proteins represented explicitly as active harmonic linkers. Their heads bind stochastically to polymer segments within a…

Biological Physics · Physics 2021-08-31 Amir Shee , Nisha Gupta , Abhishek Chaudhuri , Debasish Chaudhuri

Linear polymers are represented as chains of hopping reptons and their motion is described as a stochastic process on a lattice. This admittedly crude approximation still catches essential physics of polymer motion, i.e. the universal…

Statistical Mechanics · Physics 2015-05-18 J. M. J. van Leeuwen , Andrzej Drzewinski

We show the presence of both a minimum and clear oscillations in the frequency dependence of the translocation time of a polymer described as a unidimensional Rouse chain driven by a spatially localized oscillating linear potential. The…

Soft Condensed Matter · Physics 2010-09-16 Alessandro Fiasconaro , Juan José Mazo , Fernando Falo

While the dynamics of dimers and polymer chains in a viscous solvent is well understood within the celebrated Rouse model, the effect of an external magnetic field on the dynamics of a charged chain is much less understood. Here we…

Statistical Mechanics · Physics 2022-07-01 Rushikesh Shinde , Jens Uwe Sommer , Hartmut Löwen , Abhinav Sharma

We perform numerical simulations of an active fully flexible self-avoiding polymer as a function of the quality of the embedding solvent described in terms of an effective monomer-monomer interaction. Specifically, by extracting the Flory…

Soft Condensed Matter · Physics 2020-10-19 S. Das , N. Kennedy , A. Cacciuto

We study the dynamics and conformations of a single active semiflexible polymer whose monomers experience a propulsion force perpendicular to the local tangent, with the end beads being different from the inner beads ("end-tailored"). Using…

Soft Condensed Matter · Physics 2022-02-18 K. R. Prathyusha , Falko Ziebert , Ramin Golestanian

Polymer thin films exhibit pronounced interfacial mobility gradients that modify chain relaxation, yet how these gradients govern chain-scale dynamics across depth remains incompletely understood. Using molecular dynamics simulations of…

Soft Condensed Matter · Physics 2026-02-27 Bao T. Ma , David S. Simmons

We study the dynamics of local bond orientation in regular hyperbranched polymers modeled by Vicsek fractals. The local dynamics is investigated through the temporal autocorrelation functions of single bonds and the corresponding relaxation…

Soft Condensed Matter · Physics 2016-07-26 Maxim Dolgushev , Denis A. Markelov , Florian Fürstenberg , Thomas Guérin

We investigate the influence of polymer-pore interactions on the translocation dynamics using Langevin dynamics simulations. An attractive interaction can greatly improve translocation probability. At the same time, it also increases…

Soft Condensed Matter · Physics 2007-10-01 Kaifu Luo , Tapio Ala-Nissila , See-chen Ying , Aniket Bhattacharya

We present a theoretical model for understanding the kinetics of a long polymer in solution. A Smoluchowski-like equation has been used to model the problem of polymer looping with a Dirac delta function sink of finite strength. The results…

Statistical Mechanics · Physics 2017-04-25 Moumita Ganguly , Anirudhha Chakraborty

Polymer-like structures are ubiquitous in nature and synthetic materials. Their configurational and migration properties are often affected by crowded environments leading to non-thermal fluctuations. Here, we study an ideal Rouse chain in…

Soft Condensed Matter · Physics 2024-03-12 Pietro Luigi Muzzeddu , Andrea Gambassi , Jens-Uwe Sommer , Abhinav Sharma

The competition between reptation and Rouse Dynamics is incorporated in the Rubinstein-Duke model for polymer motion by extending it with sideways motions, which cross barriers and create or annihilate hernias. Using the Density-Matrix…

Statistical Mechanics · Physics 2009-11-13 Andrzej Drzewinski , J. M. J. van Leeuwen

Molecular dynamics simulation of a generic polymer model is applied to study melts of polymers with different types of intrinsic stiffness. Important static observables of the single chain such as gyration radius or persistence length are…

Soft Condensed Matter · Physics 2017-09-13 Roland Faller , Alexander Kolb , Florian Müller-Plathe

Stress relaxation following deformation of an entangled polymeric liquid is thought to be affected by transient reforming of chain entanglements. In this work, we use single molecule techniques to study the relaxation of individual polymers…

Soft Condensed Matter · Physics 2018-07-04 Yuecheng Zhou , Charles M. Schroeder

The unfolding of a polymer below the $\theta$ point when pulled by an external force is studied both in d=2 on the lattice and in $d=3$ off lattice. A ground state analysis of finite length chains shows that the globule unfolds via multiple…

Statistical Mechanics · Physics 2009-11-07 D. Marenduzzo , A. Maritan , A. Rosa , F. Seno

The breakage of a polymer chain of segments, coupled by anharmonic bonds with applied constant external tensile force is studied by means of Molecular Dynamics simulation. We show that the mean life time of the chain becomes progressively…

Soft Condensed Matter · Physics 2015-05-27 J. Paturej , A. Milchev , V. G. Rostiashvili , T. A. Vilgis

An applied tension force changes the equilibrium conformations of a polymer chain tethered to a planar substrate and thus affects the adsorption transition as well as the coil-globule and crystallization transitions. Conversely, solvent…

Soft Condensed Matter · Physics 2015-06-22 Jutta Luettmer-Strathmann , Kurt Binder

A statistical mechanical description of flexible and semi-flexible polymer chains in a poor solvent is developed in the constant force and constant distance ensembles. We predict the existence of many intermediate states at low temperatures…

Soft Condensed Matter · Physics 2007-05-23 Sanjay Kumar , Iwan Jensen , Jesper L. Jacobsen , Anthony J. Guttmann