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Understanding the role of self-propulsion on the conformational properties of active filamentous objects has relevance in biology. In this context, we consider a flexible bead-spring model polymer for which along with both attractive and…

Soft Condensed Matter · Physics 2022-02-22 Subhajit Paul , Suman Majumder , Wolfhard Janke

Using molecular dynamic simulation, we study the stretching of an adsorbed homopolymer in a poor solvent with one end held at a distance $z_e$ from the substrate. We measure the vertical force $f$ on the end of the chain as a function of…

Soft Condensed Matter · Physics 2009-11-10 Franck Celestini , Thoma Frisch , Xabier Oyharcabal

Via molecular dynamics simulation with Langevin thermostat we study the structure and dynamics of a flexible bead-spring active polymer model after a quench from good to poor solvent conditions. The self propulsion is introduced via a…

Soft Condensed Matter · Physics 2021-03-18 Subhajit Paul , Suman Majumder , Wolfhard Janke

This study focuses on comparing the individual polymer chain dynamics in an entangled polymeric liquid under different shear and extension rates. Polymer chains under various shear rates and extension rates were simulated using a…

Chemical Physics · Physics 2021-01-15 Behrouz Behdani , Tong Mou , Cody Spratt , Slava Butcovich , Ryan Gettler , Joontaek Park

We consider the rupture dynamics of a homopolymer chain pulled at one end at a constant loading rate. Our model of the breakable polymer is related to the Rouse chain, with the only difference that the interaction between the monomers is…

Soft Condensed Matter · Physics 2009-10-29 S. Fugmann , I. M. Sokolov

We study the influence of some quenched disorder in the sequence of monomers on the entropic elasticity of long polymeric chains. Starting from the Kratky-Porod model, we show numerically that some randomness in the favoured angles between…

Statistical Mechanics · Physics 2009-10-30 D. Bensimon , D. Dohmi , M. Mezard

Dynamics of a discrete polymer in time-dependent external potentials is studied with the master equation approach. We consider both stochastic and deterministic switching mechanisms for the potential states and give the essential equations…

Statistical Mechanics · Physics 2008-06-25 Janne Kauttonen , Juha Merikoski , Otto Pulkkinen

We study flexible polymer macromolecules in a crowded (porous) environment, modelling them as self-attracting self-avoiding walks (SASAW) on site-diluted percolative lattices in space dimensions d=2, 3. The influence of stretching force on…

Soft Condensed Matter · Physics 2009-12-09 V. Blavatska , W. Janke

We consider how active forces modeled as non-thermal random noise affect the average dynamical properties of a Rouse polymer. As the power spectrum of the noise is not known we keep the analytical treatment as generic as possible and then…

Statistical Mechanics · Physics 2017-05-23 Dino Osmanovic , Yitzhak Rabin

We study dynamics of a Rouse polymer chain, which diffuses in a three-dimensional space under the constraint that one of its ends, referred to as the slip-link, may move only along a one-dimensional line containing randomly placed,…

Statistical Mechanics · Physics 2007-05-23 S. Nechaev , G. Oshanin , A. Blumen

We present large-scale molecular dynamics simulations for a coarse-grained model of polymer melts in equilibrium. From detailed Rouse mode analysis we show that the time-dependent relaxation of the autocorrelation function (ACF) of modes…

Soft Condensed Matter · Physics 2017-04-26 Hsiao-Ping Hsu , Kurt Kremer

Using extensive computer simulations, the behavior of the structural modes --- more precisely, the eigenmodes of a phantom Rouse polymer --- are characterized for a polymer in the three-dimensional repton model, and are used to study the…

Soft Condensed Matter · Physics 2015-03-18 Gerard T. Barkema , Debabrata Panja , J. M. J. van Leeuwen

By applying local primitive path and Rouse modes analysis we study the chains conformations, local dynamics and viscosity of a model polymer melt in a polymer-wall interface. We establish that the presence of a repulsive wall leads to…

Materials Science · Physics 2009-11-11 Mihail Vladkov , J. -L. Barrat

In this paper, we construct an effective model for the dynamics of an excluded-volume chain under confinement, by extending the formalism of Rouse modes. We make specific predictions about the behavior of the modes for a single polymer…

Soft Condensed Matter · Physics 2009-09-29 Joshua Kalb , Bulbul Chakraborty

This work investigates the effects of tangent polar activity on the conformational and dynamic properties of entangled polymer melts through Langevin molecular dynamics simulations. We examine systems composed of all self-propelled,…

Soft Condensed Matter · Physics 2024-11-19 Javier Oller-Iscar , Andrés R. Tejedor , Marisol Ripoll , Jorge Ramírez

The dynamics of a polymer ring enclosing a constant {\sl algebraic} area is studied. The constraint of a constant area is found to couple the dynamics of the two Cartesian components of the position vector of the polymer ring through the…

Soft Condensed Matter · Physics 2009-11-10 Arti Dua , Thomas A. Vilgis

The static and dynamic properties of a cyclic Rouse chain modified by the introduction of an effective, spherically symmetric, attracting potential of entropic nature is studied. It is shown that a relatively weak potential can lead to a…

Soft Condensed Matter · Physics 2025-02-26 Nail Fatkullin , Carlos Mattea , Kevin Lindt , Siegfried Stapf , Margarita Kruteva

Modeling of polymer chains has received a lot of attention in mathematics. In fact, probabilistic models that naturally arise in statistical mechanics have been widely studied by mathematicians for the very challenging and novel problems…

Probability · Mathematics 2007-05-23 Francesco Caravenna

Using molecular dynamics simulations we examine the dynamics of a family of model polymers with varying chain length and torsional potential barriers. We focus on features of the dynamics of polymers that are seen experimentally but absent…

Soft Condensed Matter · Physics 2019-06-11 Daniel Fragiadakis , C. Michael Roland

We study the translocation of a semiflexible polymer through a conical channel with attractive surface interactions and a driving force which varies spatially inside the channel. Using the results of the translocation dynamics of a flexible…

Soft Condensed Matter · Physics 2022-11-15 Andri Sharma , Rajeev Kapri , Abhishek Chaudhuri