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High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

The attosecond high harmonic pulses obtained from a long Ar-filled gas cell were characterized by two techniques - the reconstruction of attosecond beating by interference of two-photon transition (RABITT) and frequency-resolved optical…

The physics of high harmonics has led to the generation of attosecond pulses and to trains of attosecond pulses. Measurements that confirm the pulse duration are all performed in the far field. All pulse duration measurements tacitly assume…

Optics · Physics 2012-06-15 E. Frumker , G. G. Paulus , H. Niikura , A. Naumov , D. M. Villeneuve , P. B. Corkum

We demonstrate a novel algorithmic approach for the second-harmonic-generation (SHG) frequency-resolved optical gating (FROG) ultrashort-pulse-measurement technique that always converges and, for complex pulses, is also much faster. It…

Optics · Physics 2019-02-20 Rana Jafari , Travis Jones , Rick Trebino

Coherent control over electron dynamics in atoms and molecules using high-intensity circularly-polarized laser pulses gives rise to current loops, resulting in the emission of magnetic fields. We propose and demonstrate with ab-initio…

We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…

Optics · Physics 2009-07-09 Marcin Kacprowicz , Wojciech Wasilewski , Konrad Banaszek

High-harmonic generation from solids can be utilized as probe of ultrafast dynamics, but thus far only over extended sample areas, since its spatial resolution is diffraction-limited. Here we propose spatial polarization gating, that is…

We review the main research directions ongoing in the development of high-harmonic generation-based extreme ultraviolet sources for the synthesization and application of trains and isolated attosecond pulses to time-resolved spectroscopy. A…

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

Frequency-resolved optical gating (FROG) is a popular technique for complete characterization of ultrashort laser pulses. The acquired data in FROG, called FROG trace, is the Fourier magnitude of the product of the unknown pulse with a…

Signal Processing · Electrical Eng. & Systems 2020-01-08 Samuel Pinilla , Tamir Bendory , Yonina C. Eldar , Henry Arguello

By means of a metal opto-acoustic transducer we generate quasi-longitudinal and quasi-transverse picosecond strain pulses in a (311)-GaAs substrate and monitor their propagation by picosecond acoustic interferometry. By probing at the…

Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schr\"{o}dinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields.…

Atomic Physics · Physics 2015-10-28 Lukas Medišauskas , Jack Wragg , Hugo van der Haart , Misha Yu. Ivanov

We develop the two-electron attosecond streak camera under realistic conditions using a quasi-classical model. We assume extreme ultra-violet (XUV) attosecond pulses with a full width at half maximum (FWHM) of 24 attoseconds, centered at…

Atomic Physics · Physics 2015-06-05 H. Price , A. Staudte , P. B. Corkum , A. Emmanouilidou

A practical approach is proposed for efficiently generating ultrashort attosecond pulses (APs) from realistic solid-state materials, aiming to optimize pulse width effectively. By adjusting the photon energy while maintaining a constant…

Optics · Physics 2025-02-25 Xinyuan Zhang , Shiqi Hu , Mengxue Guan , Sheng Meng

Transient grating spectroscopy has become a mainstay among metal and semiconductor characterization techniques. Here we extend the technique towards the shortest achievable timescales by using tabletop high-harmonic generation of attosecond…

We study theoretically the effect of the giant resonance in Xe on the phase difference between the consecutive high order resonantly-enhanced harmonics and calculate the duration of the attosecond pulses produced by these harmonics. For…

Atomic Physics · Physics 2016-12-28 V. V. Strelkov

Multiphoton-ionized electrons are born into a strong light field that will determine their short-term future. By controlling the infrared beam, we enable atoms or molecules to generate extreme ultraviolet (XUV) pulses and synthesize…

Atomic Physics · Physics 2020-10-13 Dong Hyuk Ko , Graham G. Brown , Chunmei Zhang , P. B. Corkum

We propose a method for programmable shaping of the amplitude and phase of the XUV and x-ray attosecond pulses produced by high-order harmonic generation. It overcomes the bandwidth limitations of existing spectral filters and enables…

Optics · Physics 2015-06-17 Dane R. Austin , Jens Biegert

The generation of gigawatt-class isolated attosecond pulses (IAPs) is vital for attosecond pump-probe experiments. In such experiments, the temporal duration of IAPs must be determined quickly and accurately. In this study, we developed a…

Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…

Atomic Physics · Physics 2020-01-08 D. Hammerland , P. Zhang , S. Kuehn , P. Jojart , I. Seres , V. Zuba , Z. Varallyay , K. Osvay , T. T. Luu , H. J. Woerner