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We demonstrate how the technique of ultrafast resonant x-ray scattering can be applied to imaging dynamics of electronic wave packets in crystals. We study scattering patterns from crystals with electron dynamics in valence bands taking…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Robin Santra

Future ultrafast x-ray light sources might image ultrafast coherent electron motion in real-space and in real-time. For a rigorous understanding of such an imaging experiment, we extend the theory of non-resonant x-ray scattering to the…

Atomic Physics · Physics 2015-06-19 Gopal Dixit , Jan Malte Slowik , Robin Santra

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

We present a concurrent Monte Carlo (MC) - molecular dynamics (MD) approach to modeling of matter response to excitation of its electronic system. The two methods are combined on-the-fly at each time step in one code, TREKIS-4. The MC model…

Other Condensed Matter · Physics 2023-02-17 N. Medvedev , F. Akhmetov , R. A. Rymzhanov , R. Voronkov , A. E. Volkov

High energy photons created from back-scattering of jets in quark gluon plasma are a valuable probe of the temperature of the plasma, and of the energy loss mechanism of quarks in the plasma. An unambiguous identification of these photons…

Nuclear Theory · Physics 2014-10-14 Somnath De , Rainer J. Fries , Dinesh K. Srivastava

We review the study of dissociative recombination and ro-vibrational excitation of diatomic and small polyatomic molecular ions initiating complex organic molecules formation. In particular, we show how Multichannel Quantum Defect Theory…

Photoabsorption by and fluorescence of the K{\alpha} transitions in highly charged iron ions are essential mechanisms for X-ray radiation transfer in astrophysical environments. We study photoabsorption due to the main K{\alpha} transitions…

Several nonlinear spectroscopy experiments which employ broadband x-ray pulses to probe the coupling between localized core and delocalized valence excitation are simulated for the amino acid cysteine at the K-edges of oxygen and nitrogen…

Chemical Physics · Physics 2015-06-15 Jason D. Biggs , Yu Zhang , Daniel Healion , Shaul Mukamel

Coherent diffractive imaging has enabled the structural analysis of individual free nanoparticles in a single shot and offers the tracking of their light induced dynamics with unprecedented spatial and temporal resolution. The retrieval of…

Optics · Physics 2020-05-07 Björn Kruse , Benjamin Liewehr , Christian Peltz , Thomas Fennel

MoS2 monolayers exhibit excellent light absorption and large thermoelectric power, which are, however, accompanied with very strong exciton binding energy - resulting in complex photoresponse characteristics. We study the electrical…

Mesoscale and Nanoscale Physics · Physics 2016-07-05 Sangeeth Kallatt , Govindarao Umesh , Navakanta Bhat , Kausik Majumdar

Vacuum-stimulated Raman transitions are driven between two magnetic substates of a rubidium-87 atom strongly coupled to an optical cavity. A magnetic field lifts the degeneracy of these states, and the atom is alternately exposed to laser…

Quantum Physics · Physics 2007-05-23 T. Wilk , S. C. Webster , H. P. Specht , G. Rempe , A. Kuhn

Polyatomic molecules in strong laser fields can undergo substantial nuclear motion within tens of femtoseconds. Ion imaging methods based on dissociation or Coulomb explosion therefore have difficulty faithfully recording the geometry…

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

A theoretical study of the intense-field single ionization of molecular hydrogen or deuterium oriented either parallel or perpendicular to a linear polarized laser pulse (400 nm) is performed for different internuclear separations and pulse…

Quantum Physics · Physics 2015-05-14 Yulian V. Vanne , Alejandro Saenz

High-intensity X-ray sources are invaluable tools, enabling experiments at the forefront of our understanding of materials science, chemistry, biology, and physics. Laser-plasma electron accelerators are sources of high-intensity X-rays, as…

Plasma Physics · Physics 2018-10-17 J. L. Martins , J. Vieira , J. Ferri , T. Fülöp

A new type of spectroscopy for high-resolution studies of spin waves that relies on resonant scattering of hard x-rays is introduced. The energy transfer in the scattering process is encoded in the precession of the polarization vector of…

Materials Science · Physics 2019-03-25 Ralf Röhlsberger

During reionization, a fraction of galactic Ly$\alpha$ emission is scattered in the intergalactic medium (IGM) and appears as a diffuse light extending megaparsecs from the source. We investigate how to probe the properties of the early…

Cosmology and Nongalactic Astrophysics · Physics 2022-06-08 Hyunbae Park , Hyo Jeong Kim , Kyungjin Ahn , Hyunmi Song , Intae Jung , Pierre Ocvirk , Paul R. Shapiro , Taha Dawoodbhoy , Jenny G. Sorce , Ilian T. Iliev

Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural phenomena such as light-induced phase transitions and chemical reactions. Whereas static electron densities in single molecules can be…

We calculate signals of real photon-photon scattering in the collision of three laser pulses. Taking goal parameters from the Station of Extreme Light at the upcoming Shanghai Coherent Light Source, we consider two scenarios: i) the…

High Energy Physics - Phenomenology · Physics 2018-08-14 B. King , H. Hu , B. Shen

We theoretically study multiphoton ionization of Mg in the circularly as well as the linearly polarized laser fields. Specifically two-, three-, and four-photon ionization cross sections from the ground and first excited states are…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima