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Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

Intense few-to-sub-femtosecond soft x-ray pulses can produce neutral, two-site excited double-core-hole states by promoting two core electrons to the same unoccupied molecular orbital. We theoretically investigate double nitrogen K-edge…

Chemical Physics · Physics 2023-06-28 Adam E. A. Fouda , Dimitris Koulentianos , Linda Young , Gilles Doumy , Phay J. Ho

Collective excitations contain rich information about photoinduced transient states in correlated systems. In a Mott insulator, charge degrees of freedom are frozen, but can be activated by photodoping. The energy-momentum distribution of…

Strongly Correlated Electrons · Physics 2020-04-23 Yao Wang , Yuan Chen , Chunjing Jia , Brian Moritz , Thomas P. Devereaux

We demonstrate that by coherent driving two uncoupled rings in same direction, the effective photon circulating time in the dual ring modulator is reduced, with increased modulation quality. The inter-ring detuning dependent photon…

Optics · Physics 2015-06-22 Tingyi Gu , Young-kai Chen , Chee Wei Wong , Po Dong

Photoionization of molecular species is, essentially, a multi-path interferometer with both experimentally controllable and intrinsic molecular characteristics. In this work, XUV photoionization of impulsively aligned molecular targets…

We study single, double and higher-order nonlinear Compton scattering where an electron interacts nonlinearly with a high-intensity laser and emits one, two or more photons. We study, in particular, how double Compton scattering is…

High Energy Physics - Phenomenology · Physics 2019-05-22 Victor Dinu , Greger Torgrimsson

We develop a new computational tool and framework for characterizing the scattering of photons by energy-nonconserving Hamiltonians into unidirectional (chiral) waveguides, for example, with coherent pulsed excitation. The temporal…

Quantum Physics · Physics 2018-05-30 Kevin A. Fischer , Rahul Trivedi , Vinay Ramasesh , Irfan Siddiqi , Jelena Vučković

The multiple scattering of an ultrashort laser pulse by a turbid dispersive medium (namely a cloud of bubbles in water) is investigated by means of Monte Carlo simulations. The theory of Gouesbet and Gr\'ehan [Part. Part. Syst. Charact. 17…

Computational Physics · Physics 2022-03-14 Geoffroy Chaussonnet , Loïc Mees , Miloš Šormaz , Patrick Jenny , Philippe M. Bardet

The perturbation of a semiconductor from the thermodynamic equilibrium often leads to the display of nonlinear dynamics and formation of spatiotemporal patterns due to the spontaneous generation of competing processes. Here, we describe the…

Materials Science · Physics 2019-09-16 Ebrahim Najafi , Amir Jafari , Bolin Liao , Ahmed Zewail

We discuss the high energy photodisintegrataion of light nuclei in which the energy of the absorbed photon is equally shared between two nucleons in the target. For these reactions we investigate the model in which photon absorption by a…

Nuclear Theory · Physics 2017-08-23 Misak M. Sargsian

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

The kinetic energy distribution of D$^+$ ions resulting from the interaction of a femtosecond laser pulse with D$_2$ molecules is calculated based on the rescattering model. From analyzing the molecular dynamics, it is shown that the…

Atomic Physics · Physics 2009-11-10 X. M. Tong , Z. X. Zhao , C. D. Lin

Quantum entangled photons provide a sensitive probe of many-body interactions and offer an unique experimental portal for quantifying many-body correlations in a material system. In this paper, we present a theoretical demonstration of how…

Quantum Physics · Physics 2020-03-18 Eric R. Bittner , Hao Li , Andrei Piryatinski , Ajay Ram Srimath Kandada , Carlos Silva

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

We grew SrTiO3 on SrTiO3 (001) by pulsed laser deposition, using x-ray scattering to monitor the growth in real time. The time-resolved small angle scattering exhibits a well-defined length scale associated with the spacing between unit…

Materials Science · Physics 2015-06-25 Aaron Fleet , Darren Dale , A. R. Woll , Y. Suzuki , J. D. Brock

The high flexibility of organic molecules offers great potential for designing the optical properties of light-active materials for the next generation of optoelectronic and photonic applications. However, despite successful implementations…

The advent of ultrafast pulsed X-ray free-electron lasers with very high brightness has enabled the determination of transient molecular structures of small and medium-sized organic molecules in excited states and undergoing chemical…

Chemical Physics · Physics 2025-10-07 Peter M. Weber , Brian Stankus , Adam Kirrander

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

Quantum Physics · Physics 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

The introduction of femto-chemistry has made it a primary goal to follow the nuclear and electronic evolution of a molecule in time and space as it undergoes a chemical reaction. Using Coulomb Explosion Imaging we have shot the first…

We solve the hydrodynamic-ballistic equations of motion for a one-dimensional time-dependent Thomas-Fermi model of Cl_2 exposed to an intense subpicosecond laser field, and observe simultaneous multielectron ionization and molecular…

Atomic Physics · Physics 2009-10-30 Miroslaw Brewczyk , Kazimierz Rzazewski , Charles W. Clark
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