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We present a directly generated on-chip dual-comb source at THz frequencies. The multi-heterodyne beating signal of two free-running THz quantum cascade laser frequency combs is measured electrically using one of the combs as a detector,…

Dual-comb spectroscopy is a rapidly developing technique that enables moving parts-free, simultaneously broadband and high-resolution measurements with microseconds of acquisition time. However, for high sensitivity measurements and…

Instrumentation and Detectors · Physics 2019-08-14 Lukasz A. Sterczewski , Jonas Westberg , Gerard Wysocki

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

We present quantum cascade laser (QCL) frequency comb devices with engineered waveguides for managing the dispersion. The QCL waveguide consists of multiple sections with different waveguide widths. The narrow and wide sections of the…

Frequency combs have revolutionized time and frequency metrology and in recent years, new frequency comb lasers that are highly compact or even on-chip have been demonstrated in the mid-infrared and THz regions of the electromagnetic…

Optics · Physics 2019-07-17 Giacomo Scalari , Jérôme Faist , Nathalie Picqué

Dissipative Kerr-microresonator soliton combs (hereafter called soliton combs) are promising to realize chip scale integration of full soliton comb systems providing high precision, broad spectral coverage and a coherent link to the…

Optical frequency combs based on mode-locked lasers have revolutionised the field of metrology and precision spectroscopy by providing precisely calibrated optical frequencies and coherent pulse trains. Amplification of the pulsed output…

Atomic Physics · Physics 2014-01-17 Jonas Morgenweg , Itan Barmes , Kjeld S. E. Eikema

We present broadband dual frequency comb laser absorption measurements of 2% H$_2$O (natural isotopic abundance of 99.7% H$_2^{16}$O) in air from 6600-7650 cm$^{-1}$ (1307-1515 nm) with a spectral point spacing of 0.0068 cm$^{-1}$.…

Atmospheric and Oceanic Physics · Physics 2024-02-29 Scott C. Egbert , Keeyoon Sung , Sean C. Coburn , Brian J. Drouin , Gregory B. Rieker

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

Coherent anti-Stokes Raman scattering (CARS) spectroscopy with time-delayed ultrashort pulses and a single-pixel photodetector has shown great potential for spectroscopic imaging and transient studies in chemistry and biological research.…

Optics · Physics 2023-12-05 Tianjian Lv , Bing Han , Ming Yan , Zhaoyang Wen , Kun Huang , Kangwen Yang , Heping Zeng

We report on the first direct measurement of the emission character of quantum cascade laser based frequency combs, using intensity autocorrelation. The correlation technique is based on fast electro-optic sampling, with a bandwidth…

Instrumentation and Detectors · Physics 2017-09-20 Ileana-Cristina Benea-Chelmus , Markus Rösch , Giacomo Scalari , Mattias Beck , Jérôme Faist

Spectroscopy in the molecular fingerprint spectral region (6.5-20 $\mu$m) yields critical information on material structure for physical, chemical and biological sciences. Despite decades of interest and effort, this portion of the…

Two semiconductor optical frequency combs consuming less than 1 W of electrical power are used to demonstrate high-sensitivity mid-infrared dual-comb spectroscopy in the important 3-4 $\mu$m spectral region. The devices are 4 millimeters…

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

Optics · Physics 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

This paper investigates three spectroscopic techniques - Tunable Diode Laser Absorption Spectroscopy (TDLAS), Wavelength Modulation Spectroscopy (WMS), and Heterodyne Phase Sensitive Dispersion Spectroscopy (HPSDS) - to evaluate their…

Instrumentation and Detectors · Physics 2025-04-02 Iskander Gazizov , Davide Pinto , Harald Moser , Savda Sam , Pedro Martin-Mateos , Liam O'Faolain , Bernhard Lendl

Accurate absorption models for gases at high pressure and temperature support advanced optical combustion diagnostics and aid in the study of harsh planetary atmospheres. Developing and validating absorption models for these applications…

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…

Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…

Optics · Physics 2016-06-01 David Burghoff , Yang Yang , Qing Hu
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