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Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

Frequency combs, broadband light sources whose spectra consist of coherent, discrete modes, have become essential in many fields. Miniaturizing frequency combs would be a significant advance in these fields, enabling the deployment of…

We demonstrate a scheme, based on a cascade of lithium niobate intensity and phase modulators driven by specially tailored radio frequency waveforms to generate an optical frequency comb with very high spectral flatness. In this work we…

We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

Quantum Physics · Physics 2015-06-04 Fritz Keilmann , Sergiu Amarie

We perform dual-comb spectroscopy in two UV bands: 325-342 nm and 372-410 nm, corresponding to the 7th and 6th harmonics of a dual-comb 2.35-{\mu}m laser source, and simultaneously resolve ~500,000 and ~1,000,000 comb lines spaced by 80 MHz…

In this work we present the design and characterization of a dual comb photoacoustic spectroscopy (DCPAS) set-up for ammonia detection in the near infrared. The system consists of a dual electro-optic (EO) comb generator that generates a…

We present here a semiconductor injection laser operating in continuous wave with an emission covering more than one octave in frequency, and displaying homogeneous power distribution among the lasing modes. The gain medium is based on a…

Optics · Physics 2015-06-22 Markus Rösch , Giacomo Scalari , Mattias Beck , Jérôme Faist

We present detailed studies of the coherence properties of an ultra-broadband super-continuum, enabled by a new approach involving continuous wave laser sources to independently probe both the amplitude and phase noise quadratures across…

Optical frequency combs have recently been demonstrated in micro--resonators through nonlinear Kerr processes. Investigations in the past few years provided better understanding of micro--combs and showed that spectral span and mode locking…

Optics · Physics 2014-06-11 Ivan S. Grudinin , Nan Yu

Low noise and high repetition rate optical frequency combs are desirable for many applications from timekeeping to precision spectroscopy. For example, gigahertz repetition rate sources greatly increase the acquisition speed of spectra in a…

We report on the fabrication of high-Q, fused-quartz microresonators and the parametric generation of a frequency comb with 36 GHz line spacing using them. We have characterized the intrinsic stability of the comb in both the time and…

Optics · Physics 2011-11-18 Scott B. Papp , Scott A. Diddams

Globally, the long-haul transmission of ultra-high bandwidth data is enabled through coherent communications. Driven by the rapid pace of growth in interconnectivity over the last decade, long-haul data transmission has reached capacities…

Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…

Quantum Physics · Physics 2023-09-20 Haowei Shi , Zaijun Chen , Scott E. Fraser , Mengjie Yu , Zheshen Zhang , Quntao Zhuang

Terahertz quantum cascade laser sources based on intra-cavity difference frequency generation from mid-IR devices are an important asset for applications in rotational molecular spectroscopy and sensing, beingthe only electrically pumped…

A tunable diode laser spectrometer has been employed to examine the overtone absorption lines of $^{12}$CH$_4$ in the region around 12780 cm$^{-1}$ (780 nm) at room temperature. The spectrometer sources are commercially available tunable…

Chemical Physics · Physics 2022-02-10 A. Lucchesini

A four-wave-mixing, frequency-comb-based, hyperspectral imaging technique that is spectrally precise, potentially rapid, and can in principle be applied to any material, is demonstrated in a near-diffraction-limited microscopy application.

Optics · Physics 2021-07-21 Brad C. Smith , Bachana Lomsadze , Steven T. Cundiff

Gas samples relevant to health and environment typically contain a plethora of molecular species that span a huge concentration dynamic range. High-concentration molecules impose a strong absorption background that hinders robust…

Optics · Physics 2024-06-07 Qizhong Liang , Apoorva Bisht , Andrew Scheck , Peter G. Schunemann , Jun Ye

Frequency combs have revolutionized optical frequency metrology, allowing one to determine highly accurate transition frequencies of a wealth of molecular species. Despite a recognized scientific interest, these progresses have only…

Dual-comb spectroscopy (DCS) with few-GHz tooth spacing that provides the optimal trade-off between spectral resolution and refresh rate is a powerful tool for measuring and analyzing rapidly evolving transient events. Despite such an…

An experimental realization of high-precision direct frequency comb spectroscopy using counter-propagating femtosecond pulses on two-photon atomic transitions is presented. Doppler broadened background signal, hampering precision…

Atomic Physics · Physics 2013-07-11 Itan Barmes , Stefan Witte , Kjeld S. E. Eikema
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