English
Related papers

Related papers: Oxygen Vacancy in ZnO-$w$ Phase: Pseudohybrid Hubb…

200 papers

Zinc-air batteries offer large specific energy densities, while relying on abundant and non-toxic materials. In this paper, we present the first multi-dimensional simulations of zinc-air batteries. We refine our existing theory-based model…

Chemical Physics · Physics 2019-06-25 Tobias Schmitt , Tobias Arlt , Ingo Manke , Arnulf Latz , Birger Horstmann

We present a first-principles study of the atomic, electronic, and magnetic properties of two-dimensional (2D), single and bilayer ZnO in honeycomb structure and its armchair and zigzag nanoribbons. In order to reveal the dimensionality…

Materials Science · Physics 2010-01-26 M. Topsakal , S. Cahangirov , E. Bekaroglu , S. Ciraci

Developing cost-effective and high-performance electrodes is critical for advancing hydrogen (H$_2$) production through electrochemical water splitting. In this study, we present a novel electrode design by depositing a $\beta$-MnO$_2$…

We present a first-principles study of the low-temperature rhombohedral phase of BaTiO$_3$ using Hubbard-corrected density-functional theory. By employing density-functional perturbation theory, we compute the onsite Hubbard $U$ for…

Materials Science · Physics 2023-12-29 G. Gebreyesus , Lorenzo Bastonero , Michele Kotiuga , Nicola Marzari , Iurii Timrov

Divalent tin oxides have attracted considerable attention as novel p-type oxide semiconductors, which are essential for realizing future oxide electronic devices. Recently, p-type Sn2Nb2O7 and SnNb2O6 were developed; however, enhanced hole…

Materials Science · Physics 2020-12-25 Akane Samizo , Makoto Minohara , Naoto Kikuchi , Kyoko K. Bando , Yoshihiro Aiura , Ko Mibu , Keishi Nishio

Energy band structures of metal-deficient hexagonal diborides M$_{0.75}$B$_2$ (M = Nb, Zr and Y) were calculated using the full-potential LMTO method. The metal vacancies change the density of states near the Fermi level and this effect is…

Superconductivity · Physics 2009-11-07 I. R. Shein , K. I. Shein , N. I. Medvedeva , A. L. Ivanovskii

Wide-bandgap oxides such as ZnO are favorable hosts for spin defect qubits due to their dilute nuclear spin background and potential for ultra-high purity. Yet, a deep-level defect qubit with robust optical and spin properties has not been…

Cubic hafnia (HfO$_2$) is of great interest for a number of applications in electronics because of its high dielectric constant. However, common defects in such applications degrade the properties of hafina. We have investigated the…

Materials Science · Physics 2019-07-31 Raghuveer Chimata , Hyeondeok Shin , Anouar Benali , Olle Heinonen

Search for efficient materials for application in the fields of optoelectronics and photovoltaics are active areas of research across the world. The potential of compounds such as K${_3}$Cu${_3}$P${_2}$ is not yet fully realized. Therefore,…

Materials Science · Physics 2022-03-25 Mwende Mbilo , George S. Manyali , Robinson J. Musembi

The formation and electronic properties of nitrogen-related defect complexes in $\beta-Ga_2O_3$ are investigated using first-principles calculations. Starting from the energetically favorable $N_{i9}-N_{OI}$ configuration, nitrogen atoms…

Materials Science · Physics 2026-05-13 Asiyeh Shokri , Yevgen Melikhov , Yevgen Syryanyy , Maryna Chernyshova , Iraida N. Demchenko

The effects of non-magnetic iso-valent defects inside the CuO2 plane(s) on superconducting transition temperature, Tc, dc charge transport, and the bulk magnetic susceptibility, \c{hi}(T), were investigated for the YBa2(Cu1-yZny)3O7-d…

Superconductivity · Physics 2013-02-15 S. H. Naqib , R. S. Islam

We discuss the applicability of the pseudopotential-like self-interaction correction (pSIC) to the study of defect energetics and electronic structure of In2O3. Our results predict that substitutional (at oxygen sites) and interstitial (at…

Materials Science · Physics 2016-06-24 Juan J. Meléndez , Małgorzata Wierzbowska

In the high-transition-temperature (high-Tc) superconductors the pseudogap phase becomes predominant when the density of doped holes is reduced1. Within this phase it has been unclear which electronic symmetries (if any) are broken, what…

We have investigated the effect of Zn substitution on the hole content, p, and the oxygen deficiency, d, for a series of high-quality crystalline c-axis oriented thin films and polycrystalline Y1-xCaxBa2(Cu1-yZny)3O7-delta compounds over a…

Superconductivity · Physics 2009-11-11 S. H. Naqib

Preparation of solid solutions represents an effective means to improve the photocatalytic properties of semiconductor-based materials. Nevertheless, the effects of site-occupancy disorder on the mixing stability and electronic properties…

Materials Science · Physics 2018-12-11 Joel Shenoy , Judy N. Hart , Ricardo Grau-Crespo , Neil L. Allan , Claudio Cazorla

The Emery model (aka the three-band Hubbard model) offers a simplified description of the copper-oxide planes that form the building blocks of high-temperature superconductors. By contrast with the even simpler one-band Hubbard model, it…

Strongly Correlated Electrons · Physics 2025-06-11 Louis-Bernard St-Cyr , David Sénéchal

Accurately modeling compounds with partially filled $d$ and $f$ shells remains a hard challenge for density-functional theory, due to large self-interaction errors stemming from local or semi-local exchange-correlation functionals. Hubbard…

Materials Science · Physics 2026-01-19 Kinga Warda , Eric Macke , Iurii Timrov , Lucio Colombi Ciacchi , Piotr M. Kowalski

In this work an overall electronic structure including the position and formation energies of various intrinsic defects are computed for anatase using Density Functional Theory aided by Hubbard correction (DFT+U). The intrinsic point…

We study the hole binding energy and pairing correlations in the three-band Hubbard model coupled to an apical oxygen phonon, by exact diagonalization and constrained-path Monte Carlo simulations. In the physically relevant charge-transfer…

Strongly Correlated Electrons · Physics 2011-03-02 Z. B. Huang , H. Q. Lin , E. Arrigoni

Colloidal zinc oxide (ZnO) nanoparticles are frequently used in the field of organic photovoltaics for the realization of solution-producible, electron-selective interfacial layers. Despite of the widespread use, there is a lack of detailed…

Applied Physics · Physics 2019-04-25 Sebastian Wilken , Jürgen Parisi , Holger Borchert