Related papers: A Near-Ideal Molecule-Based Haldane Spin-Chain
Using the valence-bond-solid (VBS) approach and the Schwinger boson mean field approximation, we study the dependence of the Haldane gap of a spin-1 linear chain Heisenberg antiferromagnet on impurity doping with different spins. The…
We theoretically study quasi-two-dimensional nickel compounds, where the nickel ions assume Ni$^{2+}$ $d^8$ valence state and feature a low-spin $S=0$ ground state quasidegenerate with $S=1$ ionic excitations. Such a level structure is…
Recent inelastic neutron scattering studies by Pan et al., Nature Communications 8, 123 (2017), find evidence for spin excitations at energies above the quasi-particle gap in an iron-selenide high-Tc superconductor. The momenta of the spin…
We present an analytical calculation of the spin-wave spectrum of the Jahn-Teller system LaTiO3. The calculation includes all superexchange couplings between nearest-neighbor Ti ions allowed by the space-group symmetries: The isotropic…
Reversible control of spin-dependent thermoelectricity via mechanical strain provides a platform for next-generation energy harvesting and thermal logic circuits. Using first-principles and Boltzmann transport calculations, we demonstrate…
We have obtained an analytic expression for the $k$ dependence of excitation energy gap for an arbitrary double $S=1/2$ spin-chain by using the nonlocal unitary transformation and the variational method. It is checked to explain the gap…
We present a systematic inelastic neutron scattering and neutron diffraction study of the magnetic structure of the quasi-1D spin-1/2 magnet SrCo2V2O8, where the interchain coupling in the Neel-type antiferromagnetic ground state breaks the…
The recently discovered high-$T_c$ superconductivity in La$_{3}$Ni$_{2}$O$_{7}$ with $T_c \approx 80K$ provides another intriguing platform to explore the microscopic mechanism of unconventional superconductivity. In this work, we study a…
Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor…
We show how quasi-one-dimensional correlated insulating states arise at two-thirds filling in organometallic multinuclear coordination complexes described by layered decorated honeycomb lattices. The interplay of spin-orbit coupling and…
The frustrated spin-1/2 Ising-Heisenberg ladder with Heisenberg intra-rung and Ising inter-rung interactions is exactly solved in a longitudinal magnetic field by taking advantage of the local conservation of the total spin on each rung and…
Inelastic neutron scattering experiments on the Haldane-gap quantum antiferromagnet NDMAP are performed in magnetic fields below and above the critical field Hc at which the gap closes. Quasi-elastic neutron scattering is found for H>Hc…
Neutron scattering experiments reveal that a diagonal spin modulation, which is a one-dimensional modulation rotated away by 45$^\circ$ from that in the superconducting phase, occurs universally across the insulating spin-glass phase in…
We use extensive DMRG calculations to show that a classification of SU(n) spin chains with regard to the existence of spinon confinement and hence a Haldane gap obtained previously for valence bond solid models applies to SU(n) Heisenberg…
High-field electron paramagnetic resonance (HFEPR) spectra were collected at several frequencies for single crystal [Zn3.91Ni0.09(hmp)4(dmb)4Cl4] (1), where dmb is 3,3-dimethyl-1-butanol and hmp is the monoanion of 2-hydroxymethylpyridine.…
We present results of inelastic neutron scattering experiments performed for the compound Magnetic and neutron spectroscopic properties of the tetrameric nickel compound $[Mo_{12}O_{28}(\mu_2-OH)_9(\mu_3-OH)_3{Ni(H_2O)_3}_4] $\cdot$…
Heavy transition metal magnets with $J_{\rm eff}$ $=$ 1/2 electronic ground states have attracted recent interest due to their penchant for hosting new classes of quantum spin liquids and superconductors. Unfortunately, model systems with…
Detailed ${}^{31}$P nuclear magnetic resonance (NMR) measurements are presented on well-characterized single crystals of antiferromagnetic van der Waals Ni$_2$P$_2$S$_6$. An anomalous breakdown is observed in the proportionality of the NMR…
We calculate the excitation spectrum and spectral weights of the alternating antiferromagnetic-ferromagnetic spin-half Heisenberg chain with exchange couplings $J$ and $-|\lambda|J$ as a power series in $\lambda$. For small $|\lambda|$, the…
Improving matrix-product state techniques based on the purification of the density matrix, we are able to accurately calculate the finite-temperature dynamic response of the infinite spin-1 XXZ chain with single-ion anisotropy in the…