Related papers: Nonadiabatic Sunlight-harvesting
Using a mid-infrared quantum cascade laser and wavelength modulation absorption spectroscopy, we measure the frequencies of ro-vibrational transitions of N$_2$O in the 17 $\mu$m region with uncertainties below 5 MHz. These lines,…
We present a theoretical study of noise-induced quantum coherences in a model three-level V-type system interacting with incoherent radiation, an important prototype for a wide range of physical systems ranging from trapped ions to…
Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…
We investigate the generation of higher-order harmonics from a quantum optics perspective via the interaction of a semiconductor with a coherent pump field focusing on the regime where strong-field intraband excitations dominate. The…
Photoassociation, assembling molecules from atoms using laser light, is limited by the low density of atom pairs at sufficiently short interatomic separations. Here, we show that non-resonant light with intensities of the order of 10^10…
The equations governing the interaction between incoherent light and electron-acoustic waves are presented. The modulational instability properties of the system are studied, and the effect of partially coherent light is discussed. It is…
Effects of coupling between an molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using nonequilibrium Green's function method.…
Optical resonators have shown outstanding abilities to tailor chemical landscapes through enhanced light-matter interaction between confined optical modes and molecule vibrations. We propose a theoretical model to study cooperative…
The nonlinear absorption of laser radiation of relativistic intensities in the underdense plasma by a mechanism of stimulated bremsstrahlung of electrons on the ions/nuclei is investigated in the low frequency approximation. Coefficient of…
The semiconductor Bloch equations for a two-band model including inter- and intraband excitation are used to study the nonlinear absorption of single and multiple light pulses by direct-gap semiconductors. For a consistent analysis the…
We study collective dynamics of interacting centers of exciton-polariton condensation in presence of spatial inhomogeneity, as modeled by diatomic active oscillator lattices. The mode formalism is developed and employed to derive existence…
Photonic resonance modes can be spectrally coupled to the vibrational modes of molecules in the mid-infrared regime through interactions between localized electric fields and nearby molecules. According to recent studies, radiative loss…
We study the longitudinal stability of beam-plasma systems in the presence of a density inhomogeneity in the background plasma. Previous works have focused on the non-relativistic regime where hydrodynamical models are used to evolve…
Following the observation of coherent oscillations in non-linear spectra of photosynthetic pigment protein complexes, particularly phycobilliprotein such as PC645, coherent vibronic transport has been suggested as a design principle for…
The influence of fast vibrations on energy transfer and conversion in natural molecular aggregates is an issue of central interest. This article shows the important role of high-energy quantized vibrations and their non-equilibrium dynamics…
The extent of exciton coherence in protein-pigment complexes has significant implications for the initial light harvesting step in photosynthetic organisms. In this work we model the main antenna protein of photosystem II, namely light…
Larmor precession of the quasiparticle spin about a transverse magnetic field leads to the oscillations in the spontaneous photon echo signal due to the shuffling of the optical coherence between optically accessible (bright) and…
We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…
In this paper, the interaction of a 1064 nm continuum-wave laser with inductively-coupled plasma generated in a fluorescent light bulb has been studied both experimentally and theoretically. The absorption coefficients pertaining to the…
Vibrational density of states of a classical two-dimensional electron system obtained with a molecular-dynamics simulation is shown to have a peak in both solid and liquid phases. From an exact diagonalisation of the dynamical matrix, the…