Related papers: Nonadiabatic Sunlight-harvesting
Quantum coherence is highly involved in photochemical functioning of complex molecular systems. Co-existence and intermixing of electronic and/or vibrational coherences, while never unambiguously identified experimentally, has been proposed…
The strong-field induced generation of nonclassical states of light is not only a subject of fundamental research but also has potential usage in quantum information science and technology. The emerging field of strong-field quantum optics…
The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…
The nonlinearity exhibited by the kinetic inductance of a superconducting stripline couples stripline resonator modes together in a manner suitable for quantum non-demolition measurement of the number of photons in a given resonator mode.…
Coherence length is an important feature of a real light wave. From the Michelson interference of He-Ne laser beam, it is found that the coherence length of the beam decreases with the decrease of intensity when the laser beam passes…
We present a theory of vibrational modulation of two-dimensional coherent Fourier transformed electronic spectra. Based on an expansion of the system's energy gap correlation function in terms of Huang-Rhys factors, we explain the…
Effects of coupling between a molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using the nonequilibrium Green's function method.…
We discuss harmonic generation in the case of laser field-dressed Hamiltonians that are invariant under so-called dynamical symmetry operations. Examples for such systems are molecules which exhibit a discrete rotational symmetry of order N…
We show that a pulsed stimulus can be used to generate many-body quantum coherences in light-matter systems of general size. Specifically, we calculate the exact real-time evolution of a driven, generic out-of-equilibrium system comprising…
Strong light-matter coupling to form exciton- and vibropolaritons is increasingly touted as a powerful tool to alter the fundamental properties of organic materials. It is proposed that these states and their facile tunability can be used…
The influence of molecular vibrations on dissociative adsorption is studied by six-dimensional quantum dynamical calculations. For the system H_2 at Pd(100), which possesses non-activated pathways, it is shown that large vibrational effects…
We theoretically analyze the phase sensitivity of the Induced-Coherence (Mandel-Type) Interferometer, including the case where the sensitivity is "boosted" into the bright input regime with coherent-light seeding. We find scaling which…
We demonstrate and study the enhancement of intermediate-field two-photon absorption by shaped femtosecond pulses having spectral phases of antisymmetric nature. The intermediate-field regime corresponds to pulse intensities, where the…
In the context of nonlinear scattering, a continuous wave incident onto a nonlinear discrete molecular chain of coupled oscillators can be partially absorbed as a result of a 3-wave resonant interaction that couples two HF-waves of…
We investigate the non-linear response and energy absorption in bulk silicon irradiated by intense 12-fs near-infrared laser pulses. Depending on the laser intensity, we distinguish two regimes of non-linear absorption of the laser energy:…
The prospect of coherent dynamics and excitonic delocalization across several light-harvesting structures in photosynthetic membranes is of considerable interest, but challenging to explore experimentally. Here we demonstrate theoretically…
Vibrational polaritons are formed by strong coupling of molecular vibrations and photon modes in an optical cavity. Experiments have demonstrated that vibrational strong coupling can change molecular properties and even affect chemical…
The idea that excitonic state (electronic) coherences are of fundamental importance to natural photosynthesis gained popularity when, a decade ago, slowly dephasing quantum beats were observed in the two-dimensional electronic spectra of…
The time-development of photoexcitations in molecular aggregates exhibits specific dynamics of electronic states and vibrational wavefunction. We discuss the dynamical formation of entanglement between electronic and vibrational degrees of…
We study the stability and the modes of non -- isothermal coronal loop models with different intensity values of the equilibrium twisted magnetic field.We use an energy principle obtained via non -- equilibrium thermodynamic arguments. The…