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Methylammonium lead triiodine (MAPbI$_3$) is a material representative of the hybrid organic-inorganic lead halide perovskites which attract currently great attention due to their photovoltaic efficiency and bright optoelectronic…

Materials Science · Physics 2022-06-08 E. Kirstein , D. R. Yakovlev , E. A. Zhukov , J. Höcker , V. Dyakonov , M. Bayer

Halide perovskite solar cells presented a unique opportunity to apply modern computational materials science techniques to an (initially) poorly understood new material. In this review, we recount the key understanding developed during the…

Mesoscale and Nanoscale Physics · Physics 2018-11-07 Jarvist Moore Frost

Organometallic halide perovskites have garnered considerable attention in recent times due to their promising optoelectronic attributes, particularly within the realm of solar photovoltaics (PV). How perovskite films form is of utmost…

We present the electronic transport properties of $\mathrm{BaZrS_3}$ (BZS) thin films grown epitaxially by gas-source molecular beam epitaxy (MBE). We observe n-type behavior in all samples, with carrier concentration ranging from $4 \times…

Materials Science · Physics 2025-06-04 Jack Van Sambeek , Jessica Dong , Anton V. Ievlev , Tao Cai , Ida Sadeghi , Rafael Jaramillo

Using transient fluorescent spectra at time-zero, we develop a density-resolved fluorescent spectroscopic method for investigating photoproducts in CH3NH3PbI3 perovskite and related photophysics. The density dependent dynamical co-existence…

Materials Science · Physics 2016-11-22 Wei Wang , Yu Li , Xiangyuan Wang , Yanping Lv , Shufeng Wang , Kai Wang , Yantao Shi , Lixin Xiao , Zhijian Chen , Qihuang Gong

The transport properties of organic light-emitting diodes in which the emissive layer is composed of conjugated polymers in the liquid-crystalline phase have been investigated. We have performed simulations of the current transient response…

Condensed Matter · Physics 2009-11-07 S. J. Martin , A. Kambili , A. B. Walker

We analyze the quantum transport properties of MAPbI3 within a tight-binding model. Charge carriers are strongly scattered by the Fr\"ohlich interaction with longitudinal optical phonon modes. This limits their mobilities at room…

With the rapid evolution of lead halide perovskite solar cells, there are considerable evidences that the mobile ions strongly impact their properties. However, except the activation energy, the other properties of ionic migration are…

Materials Science · Physics 2018-06-21 Ningbo Yi , Gang Li , Yuhan Wang , Shuai Wang , Kaiyang Wang , Qinghai Song , Shumin Xiao

Perovskite solar cells have potential to deliver terawatt-scale power via low-cost manufacturing. However, scaling is limited by slow, high-temperature annealing of the inorganic transport layers and the lack of reliable, large-area methods…

Materials Science · Physics 2022-01-25 Julia E. Huddy , Youxiong Ye , William J. Scheideler

The discovery of lead free all-inorganic alloyed double perovskites have revolutionized photovoltaic research, showing promising light emitting efficiency and its tunability. However, detailed studies regarding optical, exciton, polaron and…

Materials Science · Physics 2021-10-26 Manjari Jain , Manish Kumar , Preeti Bhumla , Saswata Bhattacharya

Efficient charge separation at the interfaces between the perovskite and with the carrier transport layers is crucial for perovskite solar cells to achieve high power conversion efficiency. We systematically investigate the hole injection…

Materials Science · Physics 2017-10-05 Kunie Ishioka , Bobby G. Barker , Masatoshi Yanagida , Yasuhiro Shirai , Kenjiro Miyano

Metal halide perovskites exhibit coupled electronic and ionic properties that determine their photovoltaic performance and operational stability. Understanding and quantifying ionic transport are therefore essential for advancing perovskite…

Two-dimensional (2D) halide perovskites (HPs) are promising materials for various optoelectronic applications, yet a comprehensive understanding of their dynamics is still elusive. Here, we offer insight into the dynamics of prototypical 2D…

Materials Science · Physics 2024-08-15 Erik Fransson , Julia Wiktor , Paul Erhart

Halide perovskites are semiconductors that exhibit sharp optical absorption edges and small Urbach energies allowing for efficient collection of sunlight in thin-film photovoltaic devices. However, halide perovskites also exhibit large…

Materials Science · Physics 2019-07-25 Christian Gehrmann , David A. Egger

Great success has been achieved in improving the photovoltaic energy conversion efficiency of the organic-inorganic perovskite-based solar cells, but with very limited knowledge on the thermal transport in hybrid perovskites, which would…

Materials Science · Physics 2016-03-02 Xin Qian , Xiaokun Gu , Ronggui Yang

Hot-carrier solar cells use the photon excess energy, that is, the energy exceeding the absorber bandgap, to do additional work. These devices have the potential to beat the upper limit for the photovoltaic power conversion efficiency set…

Materials Science · Physics 2025-02-21 Priya Viji , Constantin Tormann , Clemens Göhler , Martijn Kemerink

Halide perovskites have emerged as one of the most interesting materials for optoelectronic applications due to their favorable properties, such as defect-tolerance and long charge carrier lifetimes, which are attributed to their dynamic…

Materials Science · Physics 2023-11-20 Julia Wiktor , Erik Fransson , Dominik Kubicki , Paul Erhart

We use optical pump--THz probe spectroscopy at low temperatures to study the hot carrier response in thin Bi$_2$Se$_3$ films of several thicknesses, allowing us to separate the bulk from the surface transient response. We find that for…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 R. Valdés Aguilar , J. Qi , M. Brahlek , N. Bansal , A. Azad , J. Bowlan , S. Oh , A. J. Taylor , R. P. Prasankumar , D. A. Yarotski

Lead halide perovskites (LHPs) exhibit outstanding optoelectronic properties, making them highly promising for applications in various optoelectronics devices. However, rapid ion migration in LHPs not only undermines device stability but…

The organic-inorganic hybrid lead trihalide perovskites have been emerging as the most attractive photovoltaic material. As regulated by Shockley-Queisser theory, a formidable materials science challenge for the next level improvement…