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We use time-domain terahertz spectroscopy to measure the low energy conductivity and magnons in RuCl$_3$ under external magnetic field. At zero field, an oscillation with a frequency of 0.62 THz is clearly observed in time-domain spectrum…

Strongly Correlated Electrons · Physics 2018-09-19 L. Y. Shi , Y. Q. Liu , T. Lin , M. Y. Zhang , S. J. Zhang , L. Wang , Y. G. Shi , T. Dong , N. L. Wang

In the search for experimental realizations of bond-anisotropic Kitaev interactions and resulting spin-liquid phases, the layered magnet $\alpha$-RuCl$_3$ is a prime candidate. Its modelling typically involves Heisenberg, Kitaev, and…

Strongly Correlated Electrons · Physics 2020-06-01 Lukas Janssen , Stefan Koch , Matthias Vojta

Honeycomb lattice Kitaev magnets exhibit exotic magnetic properties governed by the Kitaev interaction. This study delves into $\alpha$-RuCl$_3$, a prototypical example described by effective Hamiltonians encompassing bond-dependent Kitaev…

Strongly Correlated Electrons · Physics 2025-05-29 Hamid Mosadeq , Mohammad-Hossein Zare

We investigated the spin excitations of magnetoelectric $\text{LiFePO}_4$ by THz absorption spectroscopy in magnetic fields up to 33$\,$T. By studying their selection rules, we found not only magnetic-dipole, but also electric-dipole active…

Three kinds of magnetic resonance signals were detected in crystals of the spin-gap magnet TlCuCl_3. First, we have observed the microwave absorption due to the excitation of the transitions between the singlet ground state and the excited…

Strongly Correlated Electrons · Physics 2007-05-23 V. N. Glazkov , A. I. Smirnov , H. Tanaka , A. Oosawa

Low-energy magnon excitations in magnetoelectric LiFePO$_4$ have been investigated by high-frequency high-field electron spin resonance spectroscopy in magnetic fields up to B = 58 T and frequencies up to f = 745 GHz. For magnetic fields…

Strongly Correlated Electrons · Physics 2021-05-06 J. Werner , C. Neef , C. Koo , A. Ponomaryov , S. Zvyagin , R. Klingeler

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

We study the spin-wave excitations in $\alpha$-RuCl$_3$ by the spin-wave theory. Starting from the five-orbital Hubbard model and the perturbation theory, we derive an effective isospin-$1/2$ model in the large Hubbard ($U$) limit. Based on…

Strongly Correlated Electrons · Physics 2017-09-07 Wei Wang , Zhao-Yang Dong , Shun-Li Yu , Jian-Xin Li

Low-energy magnetic excitations in the spin-1/2 chain compound (C$_6$H$_9$N$_2$)CuCl$_3$ [known as (6MAP)CuCl$_3$] are probed by means of tunable-frequency electron spin resonance. Two modes with asymmetric (with respect to the $h\nu=g\mu_B…

Strongly Correlated Electrons · Physics 2015-05-19 M. Ozerov , A. A. Zvyagin , E. Čižmár , J. Wosnitza , R. Feyerherm , F. Xiao , C. P. Landee , S. A. Zvyagin

We study the field-induced magnetization processes of extended Heisenberg-Kitaev models on the honeycomb lattice, taking into account off-diagonal and longer-range exchange interactions, using a combination of Monte-Carlo simulations,…

Strongly Correlated Electrons · Physics 2017-09-04 Lukas Janssen , Eric C. Andrade , Matthias Vojta

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

Layered {\alpha}-RuCl3 is a promising material to potentially realize the long-sought Kitaev quantum spin liquid with fractionalized excitations. While evidence of this exotic state has been reported under a modest in-plane magnetic field,…

We compute the rotational anisotropy of the free energy of $\alpha$-RuCl$_3$ in an external magnetic field. This quantity, known as the magnetotropic susceptibility, $k$, relates to the second derivative of the free energy with respect to…

Strongly Correlated Electrons · Physics 2023-12-07 Toshihiro Sato , B. J. Ramshaw , K. A. Modic , Fakher F. Assaad

An external magnetic field can induce a transition in $\alpha$-RuCl$_3$ from an ordered zigzag state to a disordered state that is possibly related to the Kitaev quantum spin liquid. Here we present new field dependent inelastic neutron…

Thermodynamics of the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ is studied for different directions of in-plane magnetic field using measurements of the magnetic Gr\"uneisen parameter $\Gamma_B$ and specific heat $C$. We identify two…

Strongly Correlated Electrons · Physics 2021-03-03 S. Bachus , D. A. S. Kaib , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valentí , P. Gegenwart

We argue that several empirical constraints strongly restrict parameters of the effective microscopic spin model describing $\alpha$-RuCl$_3$. In particular, such constraints dictate a substantial \emph{positive} off-diagonal anisotropic…

Strongly Correlated Electrons · Physics 2020-07-06 P. A. Maksimov , A. L. Chernyshev

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of $\alpha$-RuCl$_3$, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements…

We report on a study of the electronic and magnetic properties of the triangular antiferromagnetic $\{Cu_3\}$ single-molecule magnet, based on spin density functional theory. Our calculations show that the low-energy magnetic properties are…

Mesoscale and Nanoscale Physics · Physics 2010-08-09 M. Fhokrul Islam , Javier F. Nossa , Carlo M. Canali , Mark Pederson

We report high-field electron spin resonance studies of the altermagnetic material $\alpha$-MnTe. In magnetic fields applied parallel to the triangular Mn$^{2+}$ layers we observed a single resonance line, corresponding to an…

Strongly Correlated Electrons · Physics 2025-10-29 K. Yu. Povarov , J. Wosnitza , S. Rößler , M. Schmidt , A. A. Tsirlin , S. A. Zvyagin
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